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Hyporheic Exchange Controls Fate of Trace Organic Compounds in an Urban Stream.
Schaper, Jonas L; Posselt, Malte; McCallum, James L; Banks, Eddie W; Hoehne, Anja; Meinikmann, Karin; Shanafield, Margaret A; Batelaan, Okke; Lewandowski, Joerg.
Afiliación
  • Schaper JL; Leibniz-Institute of Freshwater Ecology and Inland Fisheries , Department Ecohydrology , Müggelseedamm 310 , 12587 Berlin , Germany.
  • Posselt M; Technical University of Berlin , Chair of Water Quality Engineering , Strasse des 17. Juni 135 , 10623 Berlin , Germany.
  • McCallum JL; Department of Environmental Science and Analytical Chemistry (ACES) , Stockholm University , Stockholm 114 18 , Sweden.
  • Banks EW; National Centre for Groundwater Research and Training, College of Science and Engineering , Flinders University , GPO Box 2100, Adelaide 5001 , South Australia , Australia.
  • Hoehne A; National Centre for Groundwater Research and Training, College of Science and Engineering , Flinders University , GPO Box 2100, Adelaide 5001 , South Australia , Australia.
  • Meinikmann K; Technical University of Berlin , Chair of Water Quality Engineering , Strasse des 17. Juni 135 , 10623 Berlin , Germany.
  • Shanafield MA; Leibniz-Institute of Freshwater Ecology and Inland Fisheries , Department Ecohydrology , Müggelseedamm 310 , 12587 Berlin , Germany.
  • Batelaan O; National Centre for Groundwater Research and Training, College of Science and Engineering , Flinders University , GPO Box 2100, Adelaide 5001 , South Australia , Australia.
  • Lewandowski J; National Centre for Groundwater Research and Training, College of Science and Engineering , Flinders University , GPO Box 2100, Adelaide 5001 , South Australia , Australia.
Environ Sci Technol ; 52(21): 12285-12294, 2018 11 06.
Article en En | MEDLINE | ID: mdl-30293423
First-order half-lives for 26 trace organic compounds (TrOCs) were determined in the hyporheic zone (HZ) and along a 3 km reach of a first-order stream in South Australia during both dry and wet seasons. Two salt tracer experiments were conducted and evaluated using a transient storage model to characterize seasonal differences in stream residence time and transient storage. Lagrangian and time-integrated surface water sampling were conducted to calculate half-lives in the surface water. Half-lives in the HZ were calculated using porewater samples obtained from a modified mini-point sampler and hyporheic residence times measured via active heat-pulse sensing. Half of the investigated TrOCs (e.g., oxazepam, olmesartan, candesartan) were not significantly removed along both the investigated river stretch and the sampled hyporheic flow paths. The remaining TrOCs (e.g., metformin, guanylurea, valsartan) were found to be significantly removed in the HZ and along the river stretch with relative removals in the HZ correlating to reach-scale relative removals. Using the modeled transport parameters, it was estimated that wet season reach-scale removal of TrOCs was predominately caused by removal in the HZ when the intensity of hyporheic exchange was also higher. Factors that increase HZ exchange are thus likely to promote in-stream reactivity of TrOCs.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Agua Subterránea Tipo de estudio: Prognostic_studies País/Región como asunto: Oceania Idioma: En Revista: Environ Sci Technol Año: 2018 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Estados Unidos
Texto completo
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Agua Subterránea Tipo de estudio: Prognostic_studies País/Región como asunto: Oceania Idioma: En Revista: Environ Sci Technol Año: 2018 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Estados Unidos