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Plasma polymer film designs through the eyes of ToF-SIMS.
Bernard, Laetitia; Rupper, Patrick; Faccio, Greta; Hegemann, Dirk; Scholder, Olivier; Heuberger, Manfred; Maniura-Weber, Katharina; Vandenbossche, Marianne.
Afiliación
  • Bernard L; Laboratory for Nanoscale Materials Science, Empa, Überlandstrasse 129, 8600 Dübendorf, Switzerland.
  • Rupper P; Laboratory for Advanced Fibers, Empa, Lerchenfeldstrasse 5, 9014 St. Gallen, Switzerland.
  • Faccio G; Laboratory for Biointerfaces, Empa, Lerchenfeldstrasse 5, 9014 St. Gallen, Switzerland.
  • Hegemann D; Laboratory for Advanced Fibers, Empa, Lerchenfeldstrasse 5, 9014 St. Gallen, Switzerland.
  • Scholder O; Laboratory for Nanoscale Materials Science, Empa, Überlandstrasse 129, 8600 Dübendorf, Switzerland.
  • Heuberger M; Laboratory for Advanced Fibers, Empa, Lerchenfeldstrasse 5, 9014 St. Gallen, Switzerland.
  • Maniura-Weber K; Laboratory for Biointerfaces, Empa, Lerchenfeldstrasse 5, 9014 St. Gallen, Switzerland.
  • Vandenbossche M; Laboratory for Advanced Fibers, Empa, Lerchenfeldstrasse 5, 9014 St. Gallen, Switzerland.
Biointerphases ; 13(3): 03B417, 2018 04 05.
Article en En | MEDLINE | ID: mdl-29621884
Time-of-flight secondary ion mass spectrometry (ToF-SIMS) is increasingly used for the detailed chemical characterization of complex organic materials. Of particular interest in biointerface materials, it provides the accurate molecular information on their surface, a prerequisite for the understanding of subsequent interaction with biomaterials. Plasma polymer films are promising biointerface materials, as tuning the deposition parameters allows the control over film stability and density of surface functional groups. However, the optimization of these film properties not only requires a detailed characterization of the film chemistry, but also that of the deposition mechanisms. Here, ToF-SIMS is used within its different operation modes to investigate those on several plasma polymer film designs. The detailed information on surface molecular chemistry, interface conformation, vertical and lateral chemical and cross-linking gradients is gathered and linked to the underlying deposition mechanisms. In combination with other techniques, the interpretation and understanding of the final functional property of the films in terms of protein adsorption and site-specific binding is achieved.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Biointerphases Asunto de la revista: BIOTECNOLOGIA / ENGENHARIA BIOMEDICA Año: 2018 Tipo del documento: Article País de afiliación: Suiza Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Biointerphases Asunto de la revista: BIOTECNOLOGIA / ENGENHARIA BIOMEDICA Año: 2018 Tipo del documento: Article País de afiliación: Suiza Pais de publicación: Estados Unidos