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Molecular field theory for biaxial nematics formed from liquid crystal dimers and inhibited by the twist-bend nematic.
To, T B T; Sluckin, T J; Luckhurst, G R.
Afiliación
  • To TBT; Mathematical Sciences, University of Southampton, Southampton, SO17 1BJ, UK. tungto@if.uff.br.
Phys Chem Chem Phys ; 19(43): 29321-29332, 2017 Nov 08.
Article en En | MEDLINE | ID: mdl-29072729
Liquid crystal dimers with odd spacers are good candidates as materials for biaxial nematic phases (NB). The dimers are flexible molecules sustaining biaxial conformations, and couplings between the conformational and orientational distributions could be expected to stabilise NB. We apply a molecular field theory for flexible molecules developed elsewhere to study a simple system made up of dimers composed of two cylindrically symmetric mesogenic groups. Our model allows for two idealised conformations: one linear and one bent at a tetrahedral angle. For a restricted set of chain lengths, the model predicts a first-order reentrant phase transition from the NB phase into a low temperature uniaxial nematic phase (NU). However the formation of the biaxial nematic could be blocked by the appearance of a twist-bent nematic.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Tipo de estudio: Prognostic_studies Idioma: En Revista: Phys Chem Chem Phys Asunto de la revista: BIOFISICA / QUIMICA Año: 2017 Tipo del documento: Article Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Tipo de estudio: Prognostic_studies Idioma: En Revista: Phys Chem Chem Phys Asunto de la revista: BIOFISICA / QUIMICA Año: 2017 Tipo del documento: Article Pais de publicación: Reino Unido