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Enhanced Photophosphorylation of a Chloroplast-Entrapping Long-Lived Photoacid.
Xu, Youqian; Fei, Jinbo; Li, Guangle; Yuan, Tingting; Li, Yue; Wang, Chenlei; Li, Xianbao; Li, Junbai.
Afiliación
  • Xu Y; Beijing National Laboratory for Molecular Sciences (BNLMS) CAS Key Lab of Colloid, Interface and Chemical Thermodynamics, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China.
  • Fei J; University of Chinese Academic of Sciences, Beijing, 100049, China.
  • Li G; Beijing National Laboratory for Molecular Sciences (BNLMS) CAS Key Lab of Colloid, Interface and Chemical Thermodynamics, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China.
  • Yuan T; Beijing National Laboratory for Molecular Sciences (BNLMS) CAS Key Lab of Colloid, Interface and Chemical Thermodynamics, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China.
  • Li Y; University of Chinese Academic of Sciences, Beijing, 100049, China.
  • Wang C; Beijing National Laboratory for Molecular Sciences (BNLMS) CAS Key Lab of Colloid, Interface and Chemical Thermodynamics, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China.
  • Li X; University of Chinese Academic of Sciences, Beijing, 100049, China.
  • Li J; Beijing National Laboratory for Molecular Sciences (BNLMS) CAS Key Lab of Colloid, Interface and Chemical Thermodynamics, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China.
Angew Chem Int Ed Engl ; 56(42): 12903-12907, 2017 10 09.
Article en En | MEDLINE | ID: mdl-28834071
Enhancing solar energy conversion efficiency is very important for developing renewable energy, protecting the environment, and producing agricultural products. Efficient enhancement of photophosphorylation is demonstrated by coupling artificial photoacid generators (PAGs) with chloroplasts. The encapsulation of small molecular long-lived PAGs in the thylakoid lumen is improved greatly by ultrasonication. Under visible-light irradiation, a fast intramolecular photoreaction of the PAG occurs and produces many protons, remarkably enhancing the proton gradient in situ. Consequently, compared to pure chloroplasts, the assembled natural-artificial hybrid demonstrates approximately 3.9 times greater adenosine triphosphate (ATP) production. This work will provide new opportunities for constructing enhanced solar energy conversion systems.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Adenosina Trifosfato / Cloroplastos Idioma: En Revista: Angew Chem Int Ed Engl Año: 2017 Tipo del documento: Article País de afiliación: China Pais de publicación: Alemania
Texto completo
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XML
PubMed Links
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Adenosina Trifosfato / Cloroplastos Idioma: En Revista: Angew Chem Int Ed Engl Año: 2017 Tipo del documento: Article País de afiliación: China Pais de publicación: Alemania