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Biotransformation of (-)-(1R,4S)-Menthone and (+)-(1S,4R)-Menthone by the Common Cutworm Spodoptera litura Larvae.
Marumoto, Shinsuke; Okuno, Yoshiharu; Hagiwara, Yuki; Miyazawa, Mitsuo.
Afiliación
  • Marumoto S; Joint Research Center, Kindai University (Former name: Kinki University).
  • Okuno Y; Department of Materials Science, Wakayama National College of Technology.
  • Hagiwara Y; Department of Applied Chemistry, Kindai University (Former name: Kinki University).
  • Miyazawa M; Graduate School of Materials Science, Nara Institute of Science and Technology.
J Oleo Sci ; 66(8): 883-888, 2017 Aug 01.
Article en En | MEDLINE | ID: mdl-28701651
Using biotransformation as a biocatalytic process has the advantage of being able to proceed under mild conditions and with high regio- and enantioselectivity. This study investigated the biotransformation of (-)-(1R,4S)-menthone (1) and (+)-(1S,4R)-menthone (2) by Spodoptera litura larvae. Compound 1 was converted to (-)-(1R,4S)-7-hydroxymenthone (1-1), (+)-(1R,3S,4S)-7-hydroxyneomenthol (1-2) and (-)-(1R,4S,8R)-p-menth-3-one-9-oic acid (1-3). The metabolism of substrate 2 generated three enantiomers of the above metabolites, designated as 2-1 to 2-3, respectively. The C-9 position of (-)-menthone and (+)-menthone was oxidized to carboxylic acid by S. litura, which is a metabolic pathway not observed in any other example of biocatalysis.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Spodoptera / Larva / Mentol Límite: Animals Idioma: En Revista: J Oleo Sci Asunto de la revista: BIOQUIMICA Año: 2017 Tipo del documento: Article Pais de publicación: Japón

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Spodoptera / Larva / Mentol Límite: Animals Idioma: En Revista: J Oleo Sci Asunto de la revista: BIOQUIMICA Año: 2017 Tipo del documento: Article Pais de publicación: Japón