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Two-dimensional Mo(SCN)2: a novel MoS2-variant.
Kaltsas, Dimitrios; Tsetseris, Leonidas.
Afiliación
  • Kaltsas D; Department of Physics, National Technical University of Athens, GR-15780 Athens, Greece.
J Phys Condens Matter ; 29(8): 085702, 2017 Mar 01.
Article en En | MEDLINE | ID: mdl-28060778
Transition metal dichalcogenides (TMDC) are currently among the most studied two-dimensional (2D) materials. Based on first-principles calculations we propose a new family of 2D materials which resemble TMDC's, but contain more complex chemical groups instead of elemental chalcogen atoms. In particular, we identify various stable 2D polymorphs of molybdenum di-thiocyanate, Mo(SCN)2, with structures akin to those of MoS2. The most stable Mo(SCN)2 polymorphs are semiconductors with small energy band gaps, whereas a higher-energy structure is metallic. Since the calculated formation energies of MoS2 and Mo(SCN)2 are comparable, the synthesis of the latter should be feasible.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: J Phys Condens Matter Asunto de la revista: BIOFISICA Año: 2017 Tipo del documento: Article País de afiliación: Grecia Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: J Phys Condens Matter Asunto de la revista: BIOFISICA Año: 2017 Tipo del documento: Article País de afiliación: Grecia Pais de publicación: Reino Unido