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Tunable Self-Assembly and Morphology-Dependent Photoconductivity of a Donor-Acceptor-Structured Diruthenium Complex.
Sun, Meng-Jia; Zhang, Xinliang; Zhong, Yu-Wu; Zhan, Chuanlang; Yao, Jiannian.
Afiliación
  • Sun MJ; Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Photochemistry, Institute of Chemistry, Chinese Academy of Sciences , Beijing 100190, China.
  • Zhang X; University of Chinese Academy of Sciences , Beijing 100049, China.
  • Zhong YW; Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Photochemistry, Institute of Chemistry, Chinese Academy of Sciences , Beijing 100190, China.
  • Zhan C; University of Chinese Academy of Sciences , Beijing 100049, China.
  • Yao J; Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Photochemistry, Institute of Chemistry, Chinese Academy of Sciences , Beijing 100190, China.
Inorg Chem ; 55(24): 13007-13013, 2016 Dec 19.
Article en En | MEDLINE | ID: mdl-27989151
A donor-acceptor-structured diruthenium complex, 1(PF6)4, that contains an electron-deficient bridging ligand and electron-rich distal diarylamines modified with long aliphatic chains has been synthesized. By varying the solvent environments and assembly conditions, we obtained three different self-assembled nanostructures of 1(PF6)4, including zero-dimensional nanospheres, one-dimensional nanofibers, and thin films with interconnected nanowire networks. These structures were investigated by scanning electron microscopy, transmission electron microscopy, dynamic light scattering, X-ray diffraction, and atomic force microscopy (AFM) analysis. Conductive AFM analysis shows that the nanowire networks exhibit a high conductivity of 0.023 S/cm and an enhanced photoconductivity of 0.59 S/cm under visible light irradiation.
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Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Inorg Chem Año: 2016 Tipo del documento: Article País de afiliación: China Pais de publicación: Estados Unidos
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PubMed Links

Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Inorg Chem Año: 2016 Tipo del documento: Article País de afiliación: China Pais de publicación: Estados Unidos