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One-Step Synthesis of Boron Nitride Quantum Dots: Simple Chemistry Meets Delicate Nanotechnology.
Liu, Bingping; Yan, Shihai; Song, Zhongqian; Liu, Mengli; Ji, Xuqiang; Yang, Wenrong; Liu, Jingquan.
Afiliación
  • Liu B; College of Materials Science and Engineering, Laboratory of Fiber Materials and Modern Textile, Growing Base for State Key Laboratory, Qingdao University, Qingdao, 266071, China.
  • Yan S; College of Chemistry and Pharmaceutical Sciences, Qingdao Agricultural University, 266109, China.
  • Song Z; College of Materials Science and Engineering, Laboratory of Fiber Materials and Modern Textile, Growing Base for State Key Laboratory, Qingdao University, Qingdao, 266071, China.
  • Liu M; College of Materials Science and Engineering, Laboratory of Fiber Materials and Modern Textile, Growing Base for State Key Laboratory, Qingdao University, Qingdao, 266071, China.
  • Ji X; College of Materials Science and Engineering, Laboratory of Fiber Materials and Modern Textile, Growing Base for State Key Laboratory, Qingdao University, Qingdao, 266071, China.
  • Yang W; Centre for Chemistry and Biotechnology, School of Life and Environmental Sciences, Deakin University, Geelong Waurn Ponds Campus, VIC 3216, Australia.
  • Liu J; College of Materials Science and Engineering, Laboratory of Fiber Materials and Modern Textile, Growing Base for State Key Laboratory, Qingdao University, Qingdao, 266071, China.
Chemistry ; 22(52): 18899-18907, 2016 Dec 23.
Article en En | MEDLINE | ID: mdl-27896863
Herein, a conceptually new and straightforward aqueous route is described for the synthesis of hydroxyl- and amino-functionalized boron nitride quantum dots (BNQDs) with quantum yields (QY) as high as 18.3 % by using a facile bottom-up approach, in which a mixture of boric acid and ammonia solution was hydrothermally treated in one pot at 200 °C for 12 h. The functionalized BNQDs, with excellent photoluminescence properties, could be easily dispersed in an aqueous medium and applied as fluorescent probes for the detection of ferrous (Fe2+ ) and ferric (Fe3+ ) ions with excellent selectivity and low detection limits. The mechanisms for the hydrothermal reaction and fluorescence quenching were also simulated by using density functional theory (DFT), which confirmed the feasibility and advantages of this strategy. It provides a scalable and eco-friendly method for preparation of BNQDs with good dispersability and could also be generalized to the synthesis of other 2D quantum dots and nanoplates.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Chemistry Asunto de la revista: QUIMICA Año: 2016 Tipo del documento: Article País de afiliación: China Pais de publicación: Alemania
Texto completo
Añadir a Mi BVS
Imprimir
XML
PubMed Links
Buscar en Google

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Chemistry Asunto de la revista: QUIMICA Año: 2016 Tipo del documento: Article País de afiliación: China Pais de publicación: Alemania