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Does Topology Dictate the Incidence of the Twist-Bend Phase? Insights Gained from Novel Unsymmetrical Bimesogens.
Mandle, Richard J; Goodby, John W.
Afiliación
  • Mandle RJ; Department of Chemistry, University of York, York, YO10 5DD, UK.
  • Goodby JW; Department of Chemistry, University of York, York, YO10 5DD, UK.
Chemistry ; 22(51): 18456-18464, 2016 Dec 19.
Article en En | MEDLINE | ID: mdl-27706844
We prepared a significant number of unsymmetrical liquid-crystalline dimers that exhibit the twist-bend nematic phase; a state of matter that exhibits spontaneous breaking of mirror symmetry and, for some materials, a microsecond electrooptic response. A number of novel unsymmetrical bimesogens were synthesized and in comparing their thermal behaviour to previous literature examples, we have uncovered an unexpected relationship between the thermal stability of the nematic and NTB phases. This relationship demonstrates that molecular shape dictates the incidence of this fascinating phase of matter and leads us to speculate as to the existence of "twist-bend nematic phases" on length scales beyond those of the molecule.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Tipo de estudio: Incidence_studies / Risk_factors_studies Idioma: En Revista: Chemistry Asunto de la revista: QUIMICA Año: 2016 Tipo del documento: Article Pais de publicación: Alemania

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Tipo de estudio: Incidence_studies / Risk_factors_studies Idioma: En Revista: Chemistry Asunto de la revista: QUIMICA Año: 2016 Tipo del documento: Article Pais de publicación: Alemania