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Asymmetric silica encapsulation toward colloidal Janus nanoparticles: a concave nanoreactor for template-synthesis of an electocatalytic hollow Pt nanodendrite.
Koo, Jung Hun; Kim, Daun; Kim, Jin Goo; Jeong, Hwakyeung; Kim, Jongwon; Lee, In Su.
Afiliación
  • Koo JH; Department of Chemistry, Pohang University of Science and Technology (POSTECH), Gyeogbuk 790-784, Korea. insulee97@postech.ac.kr.
Nanoscale ; 8(30): 14593-9, 2016 Aug 14.
Article en En | MEDLINE | ID: mdl-27432650
A novel reverse microemulsion strategy was developed to asymmetrically encapsulate metal-oxide nanoparticles in silica by exploiting the self-catalytic growth of aminosilane-containing silica at a single surface site. This strategy produced various colloidal Janus nanoparticles, including Au/Fe3O4@asy-SiO2, which were converted to an Au-containing silica nanosphere, Au@con-SiO2, by reductive Fe3O4 dissolution. The use of Au@con-SiO2 as a metal-growing nanoreactor allowed the templated synthesis of various noble-metal nanocrystals, including a hollow dendritic Pt nanoshell which exhibits significantly better electrocatalytic activities for the oxygen reduction reaction than commercial Pt/C catalysts.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Nanoscale Año: 2016 Tipo del documento: Article Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Nanoscale Año: 2016 Tipo del documento: Article Pais de publicación: Reino Unido