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Geometry of guanidinium groups in arginines.
Malinska, Maura; Dauter, Miroslawa; Dauter, Zbigniew.
Afiliación
  • Malinska M; Synchrotron Radiation Research Section, Macromolecular Crystallography Laboratory, National Cancer Institute, Argonne National Laboratory, Argonne, Illinois, 60439.
  • Dauter M; Faculty of Chemistry, University of Warsaw, Warsaw, 02-093, Poland.
  • Dauter Z; Leidos Biomedical Research, Inc., Basic Science Program, Argonne National Laboratory, Argonne, Illinois, 60439.
Protein Sci ; 25(9): 1753-6, 2016 09.
Article en En | MEDLINE | ID: mdl-27326702
The restraints in common usage today have been obtained based on small molecule X-ray crystal structures available 25 years ago and recent reports have shown that the values of bond lengths and valence angles can be, in fact, significantly different from those stored in libraries, for example for the peptide bond or the histidine ring geometry. We showed that almost 50% of outliers found in protein validation reports released in the Protein Data Bank on 23 March 2016 come from geometry of guanidine groups in arginines. Therefore, structures of small molecules and atomic resolution protein crystal structures have been used to derive new target values for the geometry of this group. The most significant difference was found for NE-CZ-NH1 and NE-CZ-NH2 angles, showing that the guanidinium group is not symmetric. The NE-CZ-NH1 angle is larger, 121.5(10)˚, than NE-CZ-NH2, 119.2(10)˚, due to the repulsive interaction between NH1 and CD1 atom.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Arginina / Guanidina Idioma: En Revista: Protein Sci Asunto de la revista: BIOQUIMICA Año: 2016 Tipo del documento: Article Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Arginina / Guanidina Idioma: En Revista: Protein Sci Asunto de la revista: BIOQUIMICA Año: 2016 Tipo del documento: Article Pais de publicación: Estados Unidos