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Bottom-Up Construction of Mesoporous Nanotubes from 78-Component Self-Assembled Nanobarrels.
Zhang, Guang-Lu; Zhou, Li-Peng; Yuan, Da-Qiang; Sun, Qing-Fu.
Afiliación
  • Zhang GL; State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, Fujian (P.R. China).
  • Zhou LP; University of Chinese Academy of Sciences, Beijing 100049 (P.R. China).
  • Yuan DQ; State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, Fujian (P.R. China).
  • Sun QF; State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, Fujian (P.R. China).
Angew Chem Int Ed Engl ; 54(34): 9844-8, 2015 Aug 17.
Article en En | MEDLINE | ID: mdl-26129827
Segmental and continuous hexagonal-packed mesoporous metal-organic nanotubes (MMONTs) with outside diameters of up to 4.5 nm and channel sizes of 2.4 nm were hierarchically constructed by a rational multicomponent self-assembly process involving starting from [L2Pd2(NO3)2] (L=o-phenanthroline or 2,2'-bipyridine) and 4-pyridinyl-3-pyrazole. An unprecedented crystallization-driven cross-linking between discrete nanobarrel building units by spontaneous loss of the capping ligands to form infinite nanotubes was observed. Such a barrel-to-tube transformation provides new possibilities for the fabrication of MMONTs using the solution bottom-up approach.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Angew Chem Int Ed Engl Año: 2015 Tipo del documento: Article Pais de publicación: Alemania
Texto completo
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Imprimir
XML
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Angew Chem Int Ed Engl Año: 2015 Tipo del documento: Article Pais de publicación: Alemania