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Preclinical activity of multiple-target gold(III)-dithiocarbamato peptidomimetics in prostate cancer cells and xenografts.
Celegato, Marta; Fregona, Dolores; Mongiat, Maurizio; Ronconi, Luca; Borghese, Cinzia; Canzonieri, Vincenzo; Casagrande, Naike; Nardon, Chiara; Colombatti, Alfonso; Aldinucci, Donatella.
Afiliación
  • Celegato M; Centro di Riferimento Oncologico, IRCCS, National Cancer Institute, Experimental Oncology 2, Via F. Gallini 2, Aviano (PN), 33081, Italy.
Future Med Chem ; 6(11): 1249-63, 2014 Jul.
Article en En | MEDLINE | ID: mdl-25162999
BACKGROUND: Recently, novel gold(III)-dithiocarbamato peptidomimetics, designed to target peptide transporters upregulated in several tumor cells have shown promise as anticancer agents. RESULTS: The biological behavior of the most promising derivatives AuD8 and AuD9 was studied in PC3 and DU145 prostate cancer cells. They exert higher cytotoxicity in vitro than the reference drug cisplatin and induce apoptosis, promoting mitochondrial membrane permeabilization and stimulating reactive oxygen species generation. Moreover, they inhibit both selenoenzyme thioredoxin reductase and proteasome activity. Additionally, AuD8 effectively reduces tumor growth in prostate tumor-bearing nude mice with minimal systemic toxicity. CONCLUSION: Altogether, our results provide insights into the anticancer activity of these gold(III)-dithiocarbamato peptidomimetics and support their potential as new agents for prostate cancer treatment.
Asunto(s)

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Neoplasias de la Próstata / Tiocarbamatos / Compuestos de Oro / Peptidomiméticos Límite: Animals / Humans / Male Idioma: En Revista: Future Med Chem Año: 2014 Tipo del documento: Article País de afiliación: Italia Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Neoplasias de la Próstata / Tiocarbamatos / Compuestos de Oro / Peptidomiméticos Límite: Animals / Humans / Male Idioma: En Revista: Future Med Chem Año: 2014 Tipo del documento: Article País de afiliación: Italia Pais de publicación: Reino Unido