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The structure of human 15-lipoxygenase-2 with a substrate mimic.
Kobe, Matthew J; Neau, David B; Mitchell, Caitlin E; Bartlett, Sue G; Newcomer, Marcia E.
Afiliación
  • Kobe MJ; From the Department of Biological Sciences, Louisiana State University, Baton Rouge, Louisiana 70803 and.
J Biol Chem ; 289(12): 8562-9, 2014 Mar 21.
Article en En | MEDLINE | ID: mdl-24497644
Atherosclerosis is associated with chronic inflammation occurring over decades. The enzyme 15-lipoxygenase-2 (15-LOX-2) is highly expressed in large atherosclerotic plaques, and its activity has been linked to the progression of macrophages to the lipid-laden foam cells present in atherosclerotic plaques. We report here the crystal structure of human 15-LOX-2 in complex with an inhibitor that appears to bind as a substrate mimic. 15-LOX-2 contains a long loop, composed of hydrophobic amino acids, which projects from the amino-terminal membrane-binding domain. The loop is flanked by two Ca(2+)-binding sites that confer Ca(2+)-dependent membrane binding. A comparison of the human 15-LOX-2 and 5-LOX structures reveals similarities at the active sites, as well striking differences that can be exploited for design of isoform-selective inhibitors.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Araquidonato 15-Lipooxigenasa Límite: Humans Idioma: En Revista: J Biol Chem Año: 2014 Tipo del documento: Article Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Araquidonato 15-Lipooxigenasa Límite: Humans Idioma: En Revista: J Biol Chem Año: 2014 Tipo del documento: Article Pais de publicación: Estados Unidos