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On the structure of water-alcohol and ammonia-alcohol protonated clusters.
Karpas, Z; Eiceman, G A; Harden, C S; Ewing, R G.
Afiliación
  • Karpas Z; Department of Chemistry, New Mexico State University, Department 3C, Box 30001, 88003-0001, Las Cruces, NM, USA.
J Am Soc Mass Spectrom ; 4(6): 507-12, 1993 Jun.
Article en En | MEDLINE | ID: mdl-24235010
Collision-induced dissociation (CID) of protonated ammonia-alcohol and water-alcohol heteroclusters was studied using a triple quadrupole mass spectrometer with a corona discharge atmospheric pressure ionization source. CID results suggested that the ammonia-alcohol clusters had NH: at the core of the cluster and that hydrogen-bonded alcohol molecules solvated this central ion. In contrast, CID results in water-alcohol clusters showed that water loss was strongly favored over alcohol loss and that there was a preference for the charge to reside on an alcohol molecule. The results also indicated that a loose chain of hydrogen-bonded molecules was formed in the water-alcohol clusters and that there appeared to be no rigid protonation site or a fixed central ion. (J Am Soc Mass.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: J Am Soc Mass Spectrom Año: 1993 Tipo del documento: Article País de afiliación: Estados Unidos Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: J Am Soc Mass Spectrom Año: 1993 Tipo del documento: Article País de afiliación: Estados Unidos Pais de publicación: Estados Unidos