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The atomic scale structure of CXV carbon: wide-angle x-ray scattering and modeling studies.
Hawelek, L; Brodka, A; Dore, J C; Honkimaki, V; Burian, A.
Afiliación
  • Hawelek L; A Chelkowski Institute of Physics, University of Silesia, ulica Uniwersytecka 4, 40-007 Katowice, Poland. Institute of Non-Ferrous Metals, ulica Sowinskiego 5, 44-100 Gliwice, Poland.
J Phys Condens Matter ; 25(45): 454203, 2013 Nov 13.
Article en En | MEDLINE | ID: mdl-24140935
The disordered structure of commercially available CXV activated carbon produced from finely powdered wood-based carbon has been studied using the wide-angle x-ray scattering technique, molecular dynamics and density functional theory simulations. The x-ray scattering data has been converted to the real space representation in the form of the pair correlation function via the Fourier transform. Geometry optimizations using classical molecular dynamics based on the reactive empirical bond order potential and density functional theory at the B3LYP/6-31g* level have been performed to generate nanoscale models of CXV carbon consistent with the experimental data. The final model of the structure comprises four chain-like and buckled graphitic layers containing a small percentage of four-fold coordinated atoms (sp(3) defects) in each layer. The presence of non-hexagonal rings in the atomic arrangement has been also considered.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: J Phys Condens Matter Asunto de la revista: BIOFISICA Año: 2013 Tipo del documento: Article País de afiliación: Polonia Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: J Phys Condens Matter Asunto de la revista: BIOFISICA Año: 2013 Tipo del documento: Article País de afiliación: Polonia Pais de publicación: Reino Unido