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Pair distribution function computed tomography.
Jacques, Simon D M; Di Michiel, Marco; Kimber, Simon A J; Yang, Xiaohao; Cernik, Robert J; Beale, Andrew M; Billinge, Simon J L.
Afiliación
  • Jacques SD; 1] School of Materials, University of Manchester, Manchester M13 9PL, UK [2] Research Complex at Harwell, Rutherford Appleton Laboratory, Harwell, Didcot, Oxfordshire, OX11 0QX, UK.
Nat Commun ; 4: 2536, 2013.
Article en En | MEDLINE | ID: mdl-24077398
An emerging theme of modern composites and devices is the coupling of nanostructural properties of materials with their targeted arrangement at the microscale. Of the imaging techniques developed that provide insight into such designer materials and devices, those based on diffraction are particularly useful. However, to date, these have been heavily restrictive, providing information only on materials that exhibit high crystallographic ordering. Here we describe a method that uses a combination of X-ray atomic pair distribution function analysis and computed tomography to overcome this limitation. It allows the structure of nanocrystalline and amorphous materials to be identified, quantified and mapped. We demonstrate the method with a phantom object and subsequently apply it to resolving, in situ, the physicochemical states of a heterogeneous catalyst system. The method may have potential impact across a range of disciplines from materials science, biomaterials, geology, environmental science, palaeontology and cultural heritage to health.
Asunto(s)

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Difracción de Rayos X / Tomografía Computarizada por Rayos X / Nanoestructuras Idioma: En Revista: Nat Commun Asunto de la revista: BIOLOGIA / CIENCIA Año: 2013 Tipo del documento: Article Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Difracción de Rayos X / Tomografía Computarizada por Rayos X / Nanoestructuras Idioma: En Revista: Nat Commun Asunto de la revista: BIOLOGIA / CIENCIA Año: 2013 Tipo del documento: Article Pais de publicación: Reino Unido