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Radical formation on a conserved tyrosine residue is crucial for DyP activity.
Strittmatter, Eric; Wachter, Sabrina; Liers, Christiane; Ullrich, René; Hofrichter, Martin; Plattner, Dietmar A; Piontek, Klaus.
Afiliación
  • Strittmatter E; Institute of Organic Chemistry, Albert-Ludwigs-University, Albertstrasse 21, 79104 Freiburg, Germany.
Arch Biochem Biophys ; 537(2): 161-7, 2013 Sep 15.
Article en En | MEDLINE | ID: mdl-23876237
Dye-decolorizing peroxidases (DyPs) are able to cleave bulky anthraquinone dyes. The recently published crystal structure of AauDyPI reveals that a direct oxidation in the distal heme cavity can be excluded for most DyP substrates. It is shown that a surface-exposed tyrosine residue acts as a substrate interaction site for bulky substrates. This amino acid is conserved in eucaryotic DyPs but is missing in the structurally related chlorite dismutases (Clds). Dye-decolorizing peroxidases of procaryotic origin equally possess a conserved tyrosine in the same region of the polypeptide albeit not at the homologous position.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Peroxidasas / Tirosina / Antraquinonas / Colorantes Idioma: En Revista: Arch Biochem Biophys Año: 2013 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Peroxidasas / Tirosina / Antraquinonas / Colorantes Idioma: En Revista: Arch Biochem Biophys Año: 2013 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Estados Unidos