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Preparation and characterization of conducting mixed-valence 9,9'-dimethyl-3,3'-bicarbazyl rectangular nanowires.
Tokuda, Takuya; Murashiro, Katsuyuki; Kubo, Minako; Masu, Hyuma; Imanari, Mamoru; Seki, Hiroko; Aoki, Nobuyuki; Ochiai, Yuichi; Kanoh, Hirofumi; Hoshino, Katsuyoshi.
Afiliación
  • Tokuda T; Graduate School of Advanced Integrated Science, Chiba University, Chiba 263-8522, Japan.
Langmuir ; 28(47): 16430-5, 2012 Nov 27.
Article en En | MEDLINE | ID: mdl-23106296
The facile synthesis of an organic electric conducting nanowire is described. The simple oxidation of 9-methylcarbazole by iron(III) perchlorate in a methanol/acetonitrile mixture under atmospheric pressure and temperature produces abundant nanowires without using a template. The nanowire consists of 9,9'-dimethyl-3,3'-dicarbazyl and has a rectangular nanowire shape with an average diameter of 397 ± 50 nm and length of 17 ± 5 µm. The results of the elemental analysis, (1)H NMR, FT-IR, XPS, and ESR measurements revealed that the chemical composition of the nanowire is (dicarbazyl)(0.12)(dicarbazylium·ClO(4)(-))(0.88)·H(2)O. This result, combined with the UV-vis-NIR measurement, demonstrates that 9,9'-dimethyl-3,3'-dicarbazyl stacks in a mixed valence state. The nanowire is electroactive and has an electric conductivity of 3.0 × 10(-5) S cm(-1).

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Langmuir Asunto de la revista: QUIMICA Año: 2012 Tipo del documento: Article País de afiliación: Japón Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Langmuir Asunto de la revista: QUIMICA Año: 2012 Tipo del documento: Article País de afiliación: Japón Pais de publicación: Estados Unidos