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Synthesis and cardiac electrophysiological activity of aryl-substituted derivatives of the class III antiarrhythmic agent sematilide. Potential class I/III agents.
Phillips, G B; Morgan, T K; Nickisch, K; Lind, J M; Gomez, R P; Wohl, R A; Argentieri, T M; Sullivan, M E.
Afiliación
  • Phillips GB; Department of Medicinal Chemistry, Berlex Laboratories, Inc., Cedar Knolls, New Jersey 07927.
J Med Chem ; 33(2): 627-33, 1990 Feb.
Article en En | MEDLINE | ID: mdl-2299628
Twelve novel derivatives of the selective class III antiarrhythmic agent sematilide were prepared in an attempt to incorporate both class I and class III electrophysiological properties into a single molecule. Electrophysiological activity was determined by standard microelectrode techniques in canine cardiac Purkinje fibers. Initial assessment of class I efficacy was carried out in a ouabain-induced arrhythmia model in guinea pigs. All of the compounds prolonged action potential duration in Purkinje fibers (class III activity), and three were active against ouabain-induced arrhythmias (class I activity). Selected compounds were evaluated further in dogs for efficacy against arrhythmias occurring 24 h following coronary ligation (automatic arrhythmias) and induced by using programmed electrical stimulation techniques (reentrant arrhythmias). The most effective compounds from the series are 3g and -j, which were effective in both canine models. Molecular modeling and structure-activity relationships are discussed.
Asunto(s)
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Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Arritmias Cardíacas / Procainamida / Antiarrítmicos Límite: Animals Idioma: En Revista: J Med Chem Asunto de la revista: QUIMICA Año: 1990 Tipo del documento: Article Pais de publicación: Estados Unidos
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Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Arritmias Cardíacas / Procainamida / Antiarrítmicos Límite: Animals Idioma: En Revista: J Med Chem Asunto de la revista: QUIMICA Año: 1990 Tipo del documento: Article Pais de publicación: Estados Unidos