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Facile and efficient fabrication of photoresponsive microgels via thiol-Michael addition.
Zhang, Hui-Juan; Xin, Yan; Yan, Qiang; Zhou, Li-Lin; Peng, Liao; Yuan, Jin-Ying.
Afiliación
  • Zhang HJ; Key Lab of Organic Optoelectronics & Molecular Engineering of Ministry of Education, Department of Chemistry, Tsinghua University, Beijing 100084, PR China.
Macromol Rapid Commun ; 33(22): 1952-7, 2012 Nov 23.
Article en En | MEDLINE | ID: mdl-22907724
A photoresponsive microgel is designed by the combination of a noncovalent assembly strategy with a covalent cross-linking method. End-functionalized poly(ethylene glycol) with azobenzene [(PEG-(Azo)(2))] was mixed with acrylate-modified ß-CD (ß-CD-MAA) to form photoresponsive inclusion complex through host-guest interaction. The above photoresponsive complex was cross-linked by thiol-functionalized PEG (PEG-dithiol) via Michael addition click reaction. The photoreversibility of resulted microgel was studied by TEM, UV-Vis spectroscopy, and (1)H NMR measurements. The characterization results indicated that the reversible size changes of the microgel could be achieved by alternative UV-Vis irradiations with good repeatability.
Asunto(s)

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Compuestos de Sulfhidrilo / Geles Idioma: En Revista: Macromol Rapid Commun Año: 2012 Tipo del documento: Article Pais de publicación: Alemania

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Compuestos de Sulfhidrilo / Geles Idioma: En Revista: Macromol Rapid Commun Año: 2012 Tipo del documento: Article Pais de publicación: Alemania