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Validation of an analytical method for the determination of cadmium (Cd) in fish by atomic absorption spectrometry with electrothermal atomisation.
Costa, L C S M; Neto, A P N; Araújo, M Q; Melo, M C C; Furtado, D M S; Kikuchi, A N S.
Afiliación
  • Costa LC; Laboratory of Residues and Contaminants - National Laboratory of Ministry of Agriculture, Livestock and Food Supply (LANAGRO-PA), Av. Almirante Barroso, 1234 Zip Code: 66095-000, Brazil.
Article en En | MEDLINE | ID: mdl-22364191
The validation of an analytical method was carried out for the determination of cadmium (Cd) in fish. The method was based on sample digestion in a microwave oven and subsequent reading using an atomic absorption spectrometer with a graphite furnace. The factorial design of experiments was applied to assess method ruggedness using the methodology of Box et al. [Box GEP, Hunter WG, Hunter JS. 1978. Statistics for experiments: an introduction to design, data analysis and model building. New York (NY): Wiley], studying the influence of sample mass, volume and concentration of acid used for sample digestion and the volume of modifier used. To study the possible matrix effect in the determination of Cd, the standard addition method was also performed. The results were treated using the OLS method. For the normality test a homoskedastic distribution was observed for the developed method and the results were adjusted to the statistical model proposed. F-tests and Student's t-tests indicated that there was no matrix effect on the calibration curve between the concentration range 1.0-10.0 µg Cd l(-1). Parameters such as selectivity, precision, decision limit, detection capability and limit of quantification were established by the method of standard addition to blank samples. The limit of quantification was 6.8 µg kg(-1). Accuracy, which was evaluated by using a certified reference material, was 107.0%. The recovery of the spiked analyte was 93.69% for the concentration of 50 µg kg(-1). Precision was defined by the coefficient of variation observed (Horrat value), estimated in terms of repeatability and reproducibility, and the values were below the limit, which is 2.0. The validation procedure confirmed the suitability of the method.
Asunto(s)

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Espectrofotometría Atómica / Cadmio / Contaminación de Alimentos / Alimentos Marinos Tipo de estudio: Evaluation_studies / Prognostic_studies Límite: Animals País/Región como asunto: America do sul / Brasil Idioma: En Revista: Food Addit Contam Part A Chem Anal Control Expo Risk Assess Asunto de la revista: CIENCIAS DA NUTRICAO Año: 2012 Tipo del documento: Article País de afiliación: Brasil Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Espectrofotometría Atómica / Cadmio / Contaminación de Alimentos / Alimentos Marinos Tipo de estudio: Evaluation_studies / Prognostic_studies Límite: Animals País/Región como asunto: America do sul / Brasil Idioma: En Revista: Food Addit Contam Part A Chem Anal Control Expo Risk Assess Asunto de la revista: CIENCIAS DA NUTRICAO Año: 2012 Tipo del documento: Article País de afiliación: Brasil Pais de publicación: Reino Unido