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First-principles study of diffusion of Li, Na, K and Ag in ZnO.
Huang, Gui-Yang; Wang, Chong-Yu; Wang, Jian-Tao.
Afiliación
  • Huang GY; Department of Physics, Tsinghua University, Beijing 100084, People's Republic of China.
J Phys Condens Matter ; 21(34): 345802, 2009 Aug 26.
Article en En | MEDLINE | ID: mdl-21715789
Based on ab initio total energy calculations, Li, Na and Ag interstitials are found to be stable with at least a 1.56 eV energy barrier to transform to a zinc substitutional site in ZnO, whereas K interstitial has a relatively small energy barrier at 0.79 eV. The isolated dopant substitutional defects (Li(Zn), Na(Zn), K(Zn) and Ag(Zn)) are found to be rather stable, with at least a 3.4 eV energy barrier to transform to an interstitial site. All of the dopant interstitials (Li(i), Na(i), K(i) and Ag(i)) are fast diffusers. The diffusion of Li interstitial is isotropic, whereas the diffusion of Na, K and Ag interstitials is highly anisotropic. Fundamental processes of the vacancy-assisted mechanisms are systematically investigated and specific values of the energy barriers are obtained.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: J Phys Condens Matter Asunto de la revista: BIOFISICA Año: 2009 Tipo del documento: Article Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: J Phys Condens Matter Asunto de la revista: BIOFISICA Año: 2009 Tipo del documento: Article Pais de publicación: Reino Unido