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Application of a rapid and integrated analysis system (RIAS) as a high-throughput processing tool for in vitro ADME samples by liquid chromatography/tandem mass spectrometry.
Luippold, Andreas H; Arnhold, Thomas; Jörg, Wolfgang; Krüger, Beate; Süssmuth, Roderich D.
Afiliación
  • Luippold AH; Department of Drug Discovery Support, Boehringer Ingelheim Pharma GmbH & Co KG, Biberach an der Riss, Germany. andreas.luippold@boehringer-ingelheim.de
J Biomol Screen ; 16(3): 370-7, 2011 Mar.
Article en En | MEDLINE | ID: mdl-21335598
Over the past decade, drug discovery programs have started to address the optimization of key ADME properties already at an early stage of the process. Hence, analytical chemists have been confronted with tremendously rising sample numbers and have had to develop methodologies accelerating quantitative liquid chromatography/tandem mass spectrometry (LC/MS/MS). This article focuses on the application of a generic and fully automated LC/MS/MS, named Rapid and Integrated Analysis System (RIAS), as a high-throughput platform for the rapid quantification of drug-like compounds in various in vitro ADME assays. Previous efforts were dedicated to the setup and feasibility study of a workflow-integrated platform combining a modified high-throughput liquid handling LC/MS/MS system controlled by a customized software interface and a customized data-processing and reporting tool. Herein the authors present an extension of this previously developed basic application to a broad set of ADME screening campaigns, covering CYP inhibition, Caco-2, and PAMPA assays. The platform is capable of switching automatically between various ADME assays, performs MS compound optimization if required, and provides a speed of 8 s from sample to sample, independently of the type of ADME assay. Quantification and peak review are adopted to the high-throughput environment and tested against a standard HPLC-ESI technology.
Asunto(s)

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Cromatografía Liquida / Evaluación Preclínica de Medicamentos / Espectrometría de Masas en Tándem / Ensayos Analíticos de Alto Rendimiento Límite: Humans Idioma: En Revista: J Biomol Screen Asunto de la revista: BIOLOGIA MOLECULAR Año: 2011 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Cromatografía Liquida / Evaluación Preclínica de Medicamentos / Espectrometría de Masas en Tándem / Ensayos Analíticos de Alto Rendimiento Límite: Humans Idioma: En Revista: J Biomol Screen Asunto de la revista: BIOLOGIA MOLECULAR Año: 2011 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Estados Unidos