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Exploring the coordination modes of pyrrolyl ligands in bis(imido) uranium(VI) complexes.
Swartz, Douglas L; Spencer, Liam P; Scott, Brian L; Odom, Aaron L; Boncella, James M.
Afiliación
  • Swartz DL; Kutztown University, Department of Chemistry, Kutztown, PA 19530, USA. swartz@kutztown.edu
Dalton Trans ; 39(29): 6841-6, 2010 Aug 07.
Article en En | MEDLINE | ID: mdl-20485773
The preparation of a family of bis(imido) uranium(VI) complexes stabilized by mono- and bidentate pyrrolyl ancillary ligands is described. X-ray crystallographic studies of dipyrrolylmethane (dpm) derivatives show that the pyrrolyl coordination mode in these uranium(VI) ions is unexpected in comparison to analogous transition metal and lanthanide chemistry. The ability of the coordinated pyrrolyl moieties to undergo pyrrolyl isomerization has also been explored and demonstrates reactivity that is unique from structurally similar uranium(VI)-bis(cyclopentadienyl) derivatives.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Dalton Trans Asunto de la revista: QUIMICA Año: 2010 Tipo del documento: Article País de afiliación: Estados Unidos Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Dalton Trans Asunto de la revista: QUIMICA Año: 2010 Tipo del documento: Article País de afiliación: Estados Unidos Pais de publicación: Reino Unido