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Photophysics and photochemistry of zinc phthalocyanine/bovine serum albumin adducts.
Alarcón, Emilio; Edwards, Ana Maria; Garcia, Angélica M; Muñoz, Marcelo; Aspée, Alexis; Borsarelli, Claudio D; Lissi, Eduardo A.
Afiliación
  • Alarcón E; Facultad de Química, Departamento de Química Física, Pontificia Universidad Católica de Chile, Avda. Vicuña Mackenna 4860, Casilla 306, (536), Santiago, Chile.
Photochem Photobiol Sci ; 8(2): 255-63, 2009 Feb.
Article en En | MEDLINE | ID: mdl-19247519
Zinc phthalocyanine (ZnPc) is a well known Type II (singlet oxygen mediated) hydrophobic photosensitizer with potential use in PDT. We have found that the presence of bovine serum albumin diminishes the aggregation degree of ZnPc in aqueous solution, indicating that albumins could be potentially useful carriers for this type of photosensitizer in PDT. In order to explore the photochemical and photophysical behavior of ZnPc associated to the protein, we have evaluated triplet excited state lifetime and yield, dye bleaching, oxygen consumption, formation of carbonyls and peroxides, and the spontaneous chemiluminescence emitted after photolysis. The results show that dye association to BSA modifies the photophysics and photochemistry of ZnPC. In particular the decreased yield of long lived triplets suggests singlet state and/or static triplet quenching of the bound dye by the host protein.
Asunto(s)

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Albúmina Sérica Bovina / Indoles Idioma: En Revista: Photochem Photobiol Sci Asunto de la revista: BIOLOGIA / QUIMICA Año: 2009 Tipo del documento: Article País de afiliación: Chile Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Albúmina Sérica Bovina / Indoles Idioma: En Revista: Photochem Photobiol Sci Asunto de la revista: BIOLOGIA / QUIMICA Año: 2009 Tipo del documento: Article País de afiliación: Chile Pais de publicación: Reino Unido