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Mechanism of formation of the C-terminal beta-hairpin of the B3 domain of the immunoglobulin binding protein G from Streptococcus. II. Interplay of local backbone conformational dynamics and long-range hydrophobic interactions in hairpin formation.
Skwierawska, Agnieszka; Zmudzinska, Wioletta; Oldziej, Stanislaw; Liwo, Adam; Scheraga, Harold A.
Afiliación
  • Skwierawska A; Medical University of Gdansk, Poland.
Proteins ; 76(3): 637-54, 2009 Aug 15.
Article en En | MEDLINE | ID: mdl-19241469
Two peptides, corresponding to the turn region of the C-terminal beta-hairpin of the B3 domain of the immunoglobulin binding protein G from Streptococcus, consisting of residues 51-56 [IG(51-56)] and 50-57 [IG(50-57)], respectively, were studied by circular dichroism and NMR spectroscopy at various temperatures and by differential scanning calorimetry. Our results show that the part of the sequence corresponding to the beta-turn in the native structure (DDATKT) of the B3 domain forms bent conformations similar to those observed in the native protein. The formation of a turn is observed for both peptides in a broad range of temperatures (T = 283-323 K), which confirms the conclusion drawn from our previous studies of longer sequences from the C-terminal beta-hairpin of the B3 domain of the immunoglobulin binding protein G (16, 14, and 12 residues), that the DDATKT sequence forms a nucleation site for formation of the beta-hairpin structure of peptides corresponding to the C-terminal part of all the B domains of the immunoglobulin binding protein G. We also show and discuss the role of long-range hydrophobic interactions as well as local conformational properties of polypeptide chains in the mechanism of formation of the beta-hairpin structure.
Asunto(s)

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Péptidos / Inmunoglobulinas / Proteínas del Tejido Nervioso Idioma: En Revista: Proteins Asunto de la revista: BIOQUIMICA Año: 2009 Tipo del documento: Article País de afiliación: Polonia Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Péptidos / Inmunoglobulinas / Proteínas del Tejido Nervioso Idioma: En Revista: Proteins Asunto de la revista: BIOQUIMICA Año: 2009 Tipo del documento: Article País de afiliación: Polonia Pais de publicación: Estados Unidos