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Facile synthesis of 2-O-iodoacetyl protected glycosyl iodides: useful precursors of 1-->2-linked 1,2-trans-glycosides.
Ko, Yoon-Joo; Shim, Seung-Bo; Shin, Jung-Hyu.
Afiliación
  • Ko YJ; National Center for Inter-University Research Facilities, Seoul National University, Seoul, 151-747, Korea.
Org Lett ; 11(3): 609-12, 2009 Feb 05.
Article en En | MEDLINE | ID: mdl-19175346
The preparation and utilization of novel iodide glycosyl donors, 2-O-iodoacetyl-glycopyranosyl iodides, is described. The mechanism for the reaction of iodine with carbohydrate cyclic ketene acetal was investigated through low-temperature NMR experiments. 2-O-Iodoacetyl-glycopyranosyl iodides can serve as effective glycosyl donors giving 2-O-iodoacetyl 1,2-trans-glycosides in high yields and excellent stereoselectivities. The 2-O-iodoacetyl group was removed selectively with thiourea to afford 2-hydroxy 1,2-trans-glycosides in high yield without affecting other protecting groups and anomeric configurations.
Asunto(s)

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Glicósidos / Hidrocarburos Yodados Idioma: En Revista: Org Lett Asunto de la revista: BIOQUIMICA Año: 2009 Tipo del documento: Article Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Glicósidos / Hidrocarburos Yodados Idioma: En Revista: Org Lett Asunto de la revista: BIOQUIMICA Año: 2009 Tipo del documento: Article Pais de publicación: Estados Unidos