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Role of the Mg/Al atomic ratio in hydrotalcite-supported Pd/Sn catalysts for nitrate adsorption and hydrogenation reduction.
Wan, Dongjin; Liu, Huijuan; Zhao, Xu; Qu, Jiuhui; Xiao, Shuhu; Hou, Yining.
Afiliación
  • Wan D; State Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China. dongjin1096@yahoo.com.cn
J Colloid Interface Sci ; 332(1): 151-7, 2009 Apr 01.
Article en En | MEDLINE | ID: mdl-19144356
Hydrotalcite-supported Pd/Sn catalysts with different Mg/Al atomic ratios (2, 3, 4, and 5) for nitrate adsorption and hydrogenation reduction were successfully synthesized by a coprecipitation method. The results showed that different atomic ratios of Mg/Al resulted in different interlayer spacings and zeta-potentials of the catalysts, which thus influenced its adsorption capacity. With the increase of Mg/Al atomic ratio, the interlayer spacing rose and zeta-potential decreased. The adsorption properties of the catalysts were mainly affected by interlayer spacing when Mg/Al atomic ratios increased from 2 to 4. However, when Mg/Al atomic ratios further increased from 4 to 5, there was a negative impact on the adsorption properties of zeta-potential. Also, the adsorption capacity of the catalysts for nitrate followed the order: Mg/Al=2

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: J Colloid Interface Sci Año: 2009 Tipo del documento: Article País de afiliación: China Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: J Colloid Interface Sci Año: 2009 Tipo del documento: Article País de afiliación: China Pais de publicación: Estados Unidos