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Assessment of urinary mephenytoin metrics to phenotype for CYP2C19 and CYP2B6 activity.
Klaassen, Tobias; Jetter, Alexander; Tomalik-Scharte, Dorota; Kasel, Dirk; Kirchheiner, Julia; Jaehde, Ulrich; Fuhr, Uwe.
Afiliación
  • Klaassen T; Department of Pharmacology, Clinical Pharmacology, Hospital of the University of Cologne, Gleueler Str. 24, 50931, Köln, Germany.
Eur J Clin Pharmacol ; 64(4): 387-98, 2008 Apr.
Article en En | MEDLINE | ID: mdl-18071681
OBJECTIVES: (S)-Mephenytoin is selectively metabolised to (S)-4'-hydroxymephenytoin by CYP2C19. The urinary excretion of 4'-hydroxymephenytoin reflects the activity of individual enzymes. We evaluated fractioned urinary collection and beta-glucuronidase pre-treatment in order to determine the optimal CYP2C19 metrics. We also assessed whether urinary excretion of N-desmethylmephenytoin (nirvanol) might be a useful CYP2B6 metric in in vivo studies. METHODS: A 50-mg dose of mephenytoin was administered to 52 volunteers as a component of phenotyping cocktails in four separate studies. Urine was collected up to 166 h post-dose. Urinary excretion of 4'-hydroxymephenytoin and nirvanol was quantified by liquid chromatography-tandem mass spectrometry, and common CYP2C19 and CYP2B6 genotypes were determined. RESULTS: Cumulative excretion of 4'-hydroxymephenytoin in urine with beta-glucuronidase treatment collected from before mephenytoin administration up to 12-16 h thereafter showed the greatest difference between CYP2C19 genotypes and the lowest intra-individual variability (7%). Renal elimination of nirvanol was highest for a *4/*4 individual and lowest for individuals carrying the *5/*5 and *1/*7 genotype, but lasted for several weeks, thus making its use in cross-over studies difficult. CONCLUSION: Cumulative urinary excretion of 4'-hydroxymephenytoin 0-12 h post-administration is a sensitive and reproducible metric of CYP2C19 activity, enabling the effect of a drug on CYP2C19 to be assessed in a small sample size of n=6 volunteers. While nirvanol excretion may reflect CYP2B6 activity in vivo, it is not useful for CYP2B6 phenotyping.
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Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Oxidorreductasas N-Desmetilantes / Hidrocarburo de Aril Hidroxilasas / Mefenitoína / Anticonvulsivantes Tipo de estudio: Clinical_trials Límite: Adult / Humans / Male / Middle aged Idioma: En Revista: Eur J Clin Pharmacol Año: 2008 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Alemania
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Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Oxidorreductasas N-Desmetilantes / Hidrocarburo de Aril Hidroxilasas / Mefenitoína / Anticonvulsivantes Tipo de estudio: Clinical_trials Límite: Adult / Humans / Male / Middle aged Idioma: En Revista: Eur J Clin Pharmacol Año: 2008 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Alemania