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Capillary gas chromatography-mass spectrometry of all 93 acyclic octenes and their identification in fluid catalytic cracked gasoline.
Soják, Ladislav; Addová, Gabriela; Kubinec, Róbert; Kraus, Angelika; Bohác, Andrej.
Afiliación
  • Soják L; Institute of Chemistry, Faculty of Natural Sciences, Comenius University, Mlynská Dolina, Bratislava 84215, Slovak Republic. sojak@fns.uniba.sk
J Chromatogr A ; 1025(2): 237-53, 2004 Feb 06.
Article en En | MEDLINE | ID: mdl-14763808
The Kováts retention indices of all 93 acyclic octenes on polydimethylsiloxane and squalane as stationary phases as well as their mass spectra were measured. The means of gas chromatography-mass spectrometry (GC-MS) were used for confirmation of GC identification as well as for mass spectrometric deconvolution of the majority of gas chromatographic unseparated isomeric octene peaks. The distinction between corresponding E and Z acyclic octenes, that is either difficult or even impossible by means of GC-MS, was obtained on the basis of larger temperature coefficients of retention indices for Z isomeric octenes than for corresponding E isomers. The retention data expressed as homomorphy factors were correlated with the degree of branching, position of double bond, and position of alkyl group with respect to the double bond of acyclic octenes, and the structure-retention relationships were formulated. The 81 acyclic octenes were identified in FCC gasoline.
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Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Alquenos / Cromatografía de Gases y Espectrometría de Masas Tipo de estudio: Diagnostic_studies / Prognostic_studies Idioma: En Revista: J Chromatogr A Año: 2004 Tipo del documento: Article Pais de publicación: Países Bajos
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Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Alquenos / Cromatografía de Gases y Espectrometría de Masas Tipo de estudio: Diagnostic_studies / Prognostic_studies Idioma: En Revista: J Chromatogr A Año: 2004 Tipo del documento: Article Pais de publicación: Países Bajos