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A chromatographic approach to analyze dansyl amino acid-HP-beta-CD association using macrocyclic antibiotic as the stationary phase.
André, C; Thomassin, M; Truong, T T; Robert, J F; Guillaume, Y C.
Afiliación
  • André C; Laboratoire de Chimie Analytique, Faculté de Médecine et de Pharmacie, Place Saint-Jacques, 25030 Besançon cedex, France.
J Chromatogr Sci ; 41(6): 311-6, 2003 Jul.
Article en En | MEDLINE | ID: mdl-12935303
The retention mechanism for a series of D,L-dansyl amino acids in high-performance liquid chromatography is investigated using a teicoplanin stationary phase and hydroxypropyl-beta-cyclodextrin (HP-beta-CD) as the mobile phase additive (0-16mM). A theoretical treatment is developed to determine the HP-beta-CD influence on the equilibrium between the teicoplanin phase and the aqueous medium, respectively. From the experimental data, the association constants of the D,L-dansyl amino acids-HP-beta-CD inclusion complexes are determined and discussed in relation to the enantiomer structure. A thermodynamic study confirms that both the retention and complexation mechanisms are independent of the dansyl amino acid molecular structure and its absolute carbon configuration.
Asunto(s)
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Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Compuestos de Dansilo / Aminoácidos / Antibacterianos Tipo de estudio: Risk_factors_studies Idioma: En Revista: J Chromatogr Sci Año: 2003 Tipo del documento: Article País de afiliación: Francia Pais de publicación: Estados Unidos
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Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Compuestos de Dansilo / Aminoácidos / Antibacterianos Tipo de estudio: Risk_factors_studies Idioma: En Revista: J Chromatogr Sci Año: 2003 Tipo del documento: Article País de afiliación: Francia Pais de publicación: Estados Unidos