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UK-78,282, a novel piperidine compound that potently blocks the Kv1.3 voltage-gated potassium channel and inhibits human T cell activation.
Hanson, D C; Nguyen, A; Mather, R J; Rauer, H; Koch, K; Burgess, L E; Rizzi, J P; Donovan, C B; Bruns, M J; Canniff, P C; Cunningham, A C; Verdries, K A; Mena, E; Kath, J C; Gutman, G A; Cahalan, M D; Grissmer, S; Chandy, K G.
Afiliación
  • Hanson DC; Pfizer Inc., Central Research Division, Groton, Connecticut 06340, USA.
Br J Pharmacol ; 126(8): 1707-16, 1999 Apr.
Article en En | MEDLINE | ID: mdl-10372812
1. UK-78,282, a novel piperidine blocker of the T lymphocyte voltage-gated K+ channel, Kv1.3, was discovered by screening a large compound file using a high-throughput 86Rb efflux assay. This compound blocks Kv1.3 with a IC50 of approximately 200 nM and 1:1 stoichiometry. A closely related compound, CP-190,325, containing a benzyl moiety in place of the benzhydryl in UK-78,282, is significantly less potent. 2 Three lines of evidence indicate that UK-78,282 inhibits Kv1.3 in a use-dependent manner by preferentially blocking and binding to the C-type inactivated state of the channel. Increasing the fraction of inactivated channels by holding the membrane potential at - 50 mV enhances the channel's sensitivity to UK-78,282. Decreasing the number of inactivated channels by exposure to approximately 160 mM external K+ decreases the sensitivity to UK-78,282. Mutations that alter the rate of C-type inactivation also change the channel's sensitivity to UK-78,282 and there is a direct correlation between tau(h) and IC50 values. 3. Competition experiments suggest that UK-78,282 binds to residues at the inner surface of the channel overlapping the site of action of verapamil. Internal tetraethylammonium and external charybdotoxin do not compete UK-78,282's action on the channel. 4. UK-78,282 displays marked selectivity for Kv1.3 over several other closely related K+ channels, the only exception being the rapidly inactivating voltage-gated K+ channel, Kv1.4. 5. UK-78,282 effectively suppresses human T-lymphocyte activation.
Asunto(s)

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Piperidinas / Compuestos de Bencidrilo / Activación de Linfocitos / Linfocitos T / Bloqueadores de los Canales de Potasio / Inmunosupresores Límite: Animals / Humans Idioma: En Revista: Br J Pharmacol Año: 1999 Tipo del documento: Article País de afiliación: Estados Unidos Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Piperidinas / Compuestos de Bencidrilo / Activación de Linfocitos / Linfocitos T / Bloqueadores de los Canales de Potasio / Inmunosupresores Límite: Animals / Humans Idioma: En Revista: Br J Pharmacol Año: 1999 Tipo del documento: Article País de afiliación: Estados Unidos Pais de publicación: Reino Unido