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1.
Sci Rep ; 13(1): 8552, 2023 May 26.
Artigo em Inglês | MEDLINE | ID: mdl-37237064

RESUMO

We studied the two-step crystallisation process of a magnetic active 2D-granular system placed on different lens concaveness and under the action of an alternating magnetic field which controls its effective temperature. We have observed that the two-step features of the crystallisation process are more evident as the depth of the parabolic potential increases. At the initial formation of the nucleus, as a first step, in the central region of the lens an amorphous aggregate is formed. In an ulterior second step, this disordered aggregate, due to the effective temperature and the perturbations caused by the impacts of free particles moving in the surrounding region, evolves to an ordered crystalline structure. The nucleus size is larger for deeper concaveness of the parabolic potential. However, if the depth of the parabolic potential exceeds a certain value, the reordering process of the second step does not occur. The crystal growth occurs similarly; small disordered groups of particles join the nucleus, forming an amorphous shell of particles which experiments a rearranging while the aggregate grows. In the explored range of the depths of the parabolic potential, crystallisation generally occurs quicker as the deeper parabolic potential is. Also, aggregates are more clearly round-shaped as parabolic potential depth increases. On the contrary, the structures are more branched for a smaller depth of the parabolic potential. We studied the structural changes and features in the system by using the sixth orientational order parameter and the packing fraction.

2.
Phys Rev E ; 107(2-1): 024902, 2023 Feb.
Artigo em Inglês | MEDLINE | ID: mdl-36932580

RESUMO

It has been shown that a nonvibrating magnetic granular system, when fed by an alternating magnetic field, behaves with most of the distinctive physical features of active matter systems. In this work, we focus on the simplest granular system composed of a single magnetized spherical particle allocated in a quasi-one-dimensional circular channel that receives energy from a magnetic field reservoir and transduces it into a running and tumbling motion. The theoretical analysis, based on the run-and-tumble model for a circle of radius R, forecasts the existence of a dynamical phase transition between an erratic motion (disordered phase) when the characteristic persistence length of the run-and-tumble motion, ℓ_{c}R/2. It is found that the limiting behaviors of these phases correspond to Brownian motion on the circle and a simple uniform circular motion, respectively. Furthermore, it is qualitatively shown that the smaller the magnetization of a particle, the larger the persistence length. It is so at least within the experimental limit of validity of our experiments. Our results show a very good agreement between theory and experiment.

3.
Sci Rep ; 11(1): 16531, 2021 Aug 16.
Artigo em Inglês | MEDLINE | ID: mdl-34400707

RESUMO

We study the crystallisation processes occurring in a nonvibrating two-dimensional magnetic granular system at various fixed values of the effective temperature. In this system, the energy loss due to dissipative effects is compensated by the continuous energy input coming into the system from a sinusoidal magnetic field. When this balance leads to high values of the effective temperature, no aggregates are formed, because particles' kinetic energy prevents them from aggregating. For lower effective temperatures, formation of small aggregates is observed. The smaller the values of the applied field's amplitude, the larger the number of these disordered aggregates. One also observes that when clusters form at a given effective temperature, the average effective diffusion coefficient decreases as time increases. For medium values of the effective temperature, formation of small crystals is observed. We find that the sixth bond-orientational order parameter and the number of bonds, when considering more than two, are very sensitive for exhibiting the order in the system, even when crystals are still very small.

4.
Phys Rev E ; 100(3-1): 032602, 2019 Sep.
Artigo em Inglês | MEDLINE | ID: mdl-31640009

RESUMO

We introduce a theoretical approach to describe structural correlations among charged permeable spheres at finite particle concentrations. This theory explicitly accounts for correlations among microions and between microions and macroions and allows for the proposal of an effective interaction among macroions that successfully captures structural correlations observed in poly-N-isopropyl acrylamide microgel systems. In our description the bare charge is fixed and independent of the microgel size, the microgel concentration, and the ionic strength, which contrasts with results obtained using linear response approximations, where the bare charge needs to be adapted to properly account for microgel correlations obtained at different conditions.

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