RESUMEN
This work responds to the growing global demand for food, which requires improvements in agricultural production and sustainable management of natural resources. The focus is on soil erosion as a critical element in preserving agricultural productivity. From this perspective, the levels of radionuclides and chemical elements present in the soil, quantified through Gamma-Rays Spectrometry (GRS) and Energy Dispersive X-ray Fluorescence (EDXRF), were used to investigate soil redistribution over time. 27 soil samples ranging from 0 to 30 cm in depth were collected in an agricultural plot located in southern Brazil. Quantitative analysis indicated high mean concentrations of Fe (161 ± 7 gkg-1), Al (110 ± 17 gkg-1), Ca (2.6 ± 0.5 gkg-1), Mn (2.4 ± 0.3 gkg-1) and K (543 ± 165 mgkg-1) in comparison with the other detected elements. The quantification of 137Cs provided a mean inventory of 27 ± 17 Bqm-2. Using the proportional model, an estimated gross erosion rate of 28.2 tonha-1year-1 and a net soil deposition of 6.6 tonha-1year-1 were calculated. Therefore, a net soil loss of 21.6 tonha-1year-1 was experienced within the agricultural plot studied. The data set combination of both techniques with Principal Component Analysis (PCA) revealed correlations between the variables studied and the soil erosion dynamics. The PCA showed a tendency to separate the samples according to their sampling depth. Moreover, 137Cs behavior in soil proved to be similar to the behavior of elements found in fertilizers, like K. On the other hand, the individual influence of 137Cs was not enough to cause significant changes in the samples distribution in the scores plot, highlighting EDXRF as a promising technique to complement soil erosion studies.
Asunto(s)
Rayos gamma , Monitoreo de Radiación , Contaminantes Radiactivos del Suelo , Suelo , Contaminantes Radiactivos del Suelo/análisis , Suelo/química , Brasil , Monitoreo de Radiación/métodos , Radioisótopos de Cesio/análisis , Espectrometría gamma , Espectrometría por Rayos X/métodos , Agricultura/métodos , Rayos XRESUMEN
Brazil is the fourth largest cement consumer in the world and the largest producer in Latin America, around 1.3% of global production. The main inputs in the manufacture of cement are limestone and clay. Few studies have been carried out in the country on the risk of these materials used in civil construction. Therefore, the objective of this present work is to evaluate the radiological danger that they can present to society. Gamma spectrometry analysis on 16 samples of different brands of cement used as construction material in Rio de Janeiro (Brazil) was performed in this study, using an HPGe detector and the Genie 2000 data acquisition software. Samples were set to count for an accumulation time of 14,400 s (4 h) and all measurements were corrected to eliminate background and backscattering. Activity concentrations are determined for 226Ra was from (41.2 ± 1.6 to 174.9 ± 3.9) Bq kg-1, 232Th was from (15.7 ± 0.5 to 43.1 ± 0.7) Bq kg-1 and 40K was from (82.6 ± 7.2 to 254 ± 17) Bq kg-1. To assess radiological health risks: mean values of Radium Activity Equivalent 150.0 ± 3.4 Bq kg-1, Annual Gonadal Dose Equivalent 468 ± 11 µSv year-1 and Lifetime Excess Cancer Risk (ELCR) 2.42 ± 0.06 were calculated. Total Absorbed Dose Rates ranged from 72.2 ± 1.7 to 225.1 ± 5.2 nGy h-1. The damage to collective health was also estimated from the annual effective dose rates with an estimated total cost of damage to health of US$ 130 million. Values are generally within global limits reported by UNSCEAR.
Asunto(s)
Monitoreo de Radiación , Radiactividad , Radio (Elemento) , Contaminantes Radiactivos del Suelo , Radioisótopos de Potasio/análisis , Torio/análisis , Monitoreo de Radiación/métodos , Brasil , Materiales de Construcción/análisis , Radio (Elemento)/análisis , Contaminantes Radiactivos del Suelo/análisis , Espectrometría gammaRESUMEN
Argentina is a Latin American country which encounters soil degradation problems. The most productive regions have implemented conservative land practices (no-till). However, agricultural frontier has been displaced to marginal lands with arid and semiarid climates, with the consequent disappearance in many areas of native forest and land degradation. In this work, the fallout of gamma-emitting radionuclides, 137Cs and 7Be, was jointly used to assess changes in soil erosion in a recently converted semiarid ecosystem into agricultural land. 137Cs was utilized to estimate the erosion over the past 60 years, whereas 7Be was employed to estimate the erosion after the conversion of the area to cultivated land and soil tillage. For 137Cs the Proportional Model (PM), the Mass Balance Model II (MBMII) and the MODERN model were used, for 7Be the Profile Distribution Model (PDM) and the MODERN model were used. 137Cs indicates mean erosional rates of 8.2, 10.5 and 6.5â Mg ha-1 a-1, using MBMII, PM and MODERN, respectively, and that a soil layer between 0.5 and 0.8â mm was annually lost by erosion. By applying a 7Be tracer, we measured erosion rates of 2.4 and 3.3â Mg ha-1 (with PDM and Modern, respectively), indicating the loss of the upper 0.2â mm of soil. This erosion can be attributed to a few heavy rainfalls that occurred within the past 90 days. The results suggest that current land management practices have led to an increase in soil erosion. This could be attributed to the fact that the soil remains bare after crop harvest, which may compromise its conservation and future productivity.
Asunto(s)
Radioisótopos de Cesio , Erosión del Suelo , Contaminantes Radiactivos del Suelo , Ecosistema , Argentina , Contaminantes Radiactivos del Suelo/análisis , Agricultura/métodos , Suelo , Conservación de los Recursos NaturalesRESUMEN
Humans are constantly exposed to radioactivity present in rocks, soils, and water, mainly from materials in the Earth's crust that contain chemical elements belonging to the radioactive series of uranium and thorium. An important anthropogenic source of these natural radioisotopes to the environment is fertilizers, widely used to increase agricultural productivity. Exposure to ionizing radiation can become a public health problem worldwide, since it is related to the development of different cancers in humans. The present study aimed to survey research on the radioactive content in different types of mineral phosphate fertilizers used around the world through a comprehensive review of the Scopus and Web of Science databases. About 80 scientific articles fit the purpose of this review. The concentration activity values found varied widely from one country to another, and there is no specific legislation that determines the maximum allowed limits of radioisotopes in these agricultural inputs. In addition, there are still uncertainties regarding the impact of natural radioactivity from fertilizers on human health, highlighting the need for further investigations on the subject.
Asunto(s)
Radiactividad , Radio (Elemento) , Contaminantes Radiactivos del Suelo , Uranio , Humanos , Fertilizantes/análisis , Fosfatos , Radioisótopos , Minerales , Uranio/análisis , Torio/análisis , Contaminantes Radiactivos del Suelo/análisis , Radioisótopos de Potasio , Radio (Elemento)/análisisRESUMEN
The Uruguayan east coast has several mineral resources, which include black sand ores in the Barra de Valizas-Aguas Dulces area. Cancer in Uruguay shows non-homogeneous geographical distribution, with the highest standardized mortality ratio (SMR) in the northeast and east region, which includes the aforementioned area and the town of Barra de Valizas. The activity concentration of natural radionuclides (226Ra, 232Th and 40 K) in Barra de Valizas´soil was determined by gamma spectrometry in order to evaluate the radiological hazard for inhabitants and tourists. The outdoor annual effective dose (AEDE), excess lifetime cancer risk (ELCR), and annual gonadal dose equivalent (AGDE) were evaluated for inhabitants with a life expectancy of 77.7 years, a 0.2 and 0.5 occupancy factor, and using the conversion coefficients recommended by United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR). The annual effective dose was also evaluated for both summer and fortnight tourists. The radiological hazard indices for Barra de Valizas inhabitants are higher than the worldwide mean and recommended values. This may contribute to Rocha's higher SRM value, although a direct correlation cannot be assured with the epidemiological information currently available. Social, medical and anthropological studies will be carried out in future to provide data and verify this correlation.
Asunto(s)
Neoplasias , Monitoreo de Radiación , Radio (Elemento) , Contaminantes Radiactivos del Suelo , Humanos , Uruguay/epidemiología , Contaminantes Radiactivos del Suelo/análisis , Monitoreo de Radiación/métodos , Radioisótopos/análisis , Radio (Elemento)/análisisRESUMEN
Atmospheric nuclear tests (1945-1980) have led to radioactive fallout across the globe. French tests in Polynesia (1966-1974) may influence the signature of fallout in South America in addition to those conducted by USA and former USSR until 1963 in the Northern hemisphere. Here, we compiled the 240Pu/239Pu atom ratios reported for soils of South America and conducted additional measurements to examine their latitudinal distributions across this continent. Significantly lower ratio values were found in the 20-45° latitudinal band (0.04 to 0.13) compared to the rest of the continent (up to 0.20) and attributed to the contribution of the French atmospheric tests to the ultra-trace plutonium levels found in these soils. Based on sediment cores collected in lakes of Chile and Uruguay, we show the added value of measuring 240Pu/239Pu atom ratios to refine the age models of environmental archives in this region of the world.
Asunto(s)
Plutonio , Monitoreo de Radiación , Contaminantes Radiactivos del Suelo , Contaminantes Radiactivos del Agua , Chile , Plutonio/análisis , Radioisótopos/análisis , Suelo , Contaminantes Radiactivos del Suelo/análisis , Contaminantes Radiactivos del Agua/análisisRESUMEN
Climate, soil type and geology that can influence the activity concentrations of natural radionuclides in soils. For this, 41 samples were collected in the first 25 cm of soil from the state of Alagoas, Northeast Brazil. This sample collection represents the mains soils classifications, parental rocks, and rainfall variability in this locality. The samples of soils were processed and analyzed by means of gamma-ray spectrometry for the 40K, 226Ra and 228Ra. The non-parametric Mann-Whitney U test was applied to perform the statistical inference on the differences in activity concentration for each soil class studied. There was a significant difference in the 40K activity distributions between the combination for most soil types. The results for 226Ra show no significant difference. However, Planosols differ significantly from Yellow Acrisols and Regosols for 228Ra. The strong relationship of the 40K concentration with the rock classes was shown. On the other hand, an association of the activity concentration of 226Ra and 228Ra with the rock type was not evidenced. There was a negative correlation between the 40K activity concentration and the rainfall index. 226/228Ra concentrations showed no correlation with the rainfall index.
Asunto(s)
Monitoreo de Radiación , Contaminantes Radiactivos del Suelo , Brasil , Monitoreo de Radiación/métodos , Radioisótopos/análisis , Suelo/química , Contaminantes Radiactivos del Suelo/análisis , Espectrometría gammaRESUMEN
In this work we critically assess the soil-to-plant transfer factors (TF) for 137Cs and 40K in edible fleshy organs of tropical plants that are often components of the human diet. Radionuclide concentrations in soil and plants were obtained from previous investigations developed in Brazil, after the Goiânia radiological accident occurred in 1987. Transfer factors were determined in specific plant compartments (main root, main stem, bark, old and new branches, twig, old and new leaves, mature and green edible organs) of tropical species such as lemon (Citrus aurantifolia), orange (Citrus sinensis), guava (Psidium guajava), chili pepper (Capsicum frutescens), pomegranate (Punica granatum), papaya (Carica papaya), banana (Musa paradisíaca), and manioc (Manihot esculenta). For 137Cs, soil-to-fruit transfer factor ranged from 0.80 × 10-2 (banana) to 3.65 × 10-1 (pomegranate); for 40K, this factor was from 4.42 × 10-1 (orange) to 1.74 (chili pepper). Considering all the plant compartments analysed, the transfer factors for 40K are between 24.5 (guava) and 90.5 (papaya) times higher than for 137Cs. For both radionuclides, considerable differences in soil-to-plant transfer were found when new growing parts of the plant (green edible organ, leaf, and twig) are considered with respect to those older parts (mature edible organ, old leaf and branches). Considering all the species analyzed, the relationship TF(40K)/TF(137Cs) does not seem to follow a characteristic pattern. However, if we compare the value of this relationship for two organs of the same plant, the result is approximately constant, regardless of the species considered. This confirms earlier evidence that both radionuclides are similarly distributed in the different organs of the studied species. The differences in the transfer factors according to the ripening status of edible organs must be particularly considered when estimating the dose from ingestion of fruits and their derivatives in dose assessment models.
Asunto(s)
Plantas/metabolismo , Monitoreo de Radiación , Contaminantes Radiactivos del Suelo , Brasil , Radioisótopos de Cesio/análisis , Suelo , Contaminantes Radiactivos del Suelo/análisis , Clima TropicalRESUMEN
Cesium 137 is present in worldwide. To evaluate its deposition in the Brazilian state of Alagoas a total of 41 samples were collected by the Geological Survey of Brazil, then processed and analyzed by gamma-ray spectrometry with hyperpure germanium detectors. The activity concentration varied from (0.3 ± 0.1) Bq/kg to (1.1 ± 0.4) Bq/kg. The present study shows that the Borborema Plateau acts as a natural barrier to rainfall, favoring the deposition of 137Cs on the local soil.
Asunto(s)
Radioisótopos de Cesio/análisis , Contaminantes Radiactivos del Suelo/análisis , Brasil , Geología , Monitoreo de Radiación/métodosRESUMEN
ABSTRACT: The Chernobyl and Fukushima Dai-ichi Nuclear Power Plant accidents have demonstrated that radiocesium deposited on the ground was one of most important pathway contributions to the air dose rate. Cesium-134 contributes more significantly in the first period of 2-3 y. However, 137Cs external exposure may remain relevant for decades. The contribution to the air dose rate attributable to these radionuclides is maximum at the deposition time and then usually decreases over time. The dose rate temporal reduction is a consequence of both the radionuclide physical decay and the radionuclide downward mobility in soil. In this investigation, this decreasing behavior of the air dose rate is approached using an empirical attenuation function, and its coefficients are computed in terms of the effective diffusion coefficient and downward migration rates of radiocesium in soil. The methodology is tested for different hypothetical scenarios and in real situations, including areas affected by the two major accidents at nuclear power plants.
Asunto(s)
Aire/análisis , Radioisótopos de Cesio/análisis , Dosis de Radiación , Contaminantes Radiactivos del Suelo/análisis , Suelo/química , Rayos gamma , Monitoreo de Radiación , Factores de TiempoRESUMEN
Thorium is a radionuclide highly widespread in the earth's crust with a relevant contribution to the exposure to radiation of living organisms. Natural concentrations of thorium in the soil can be altered due to human activities such as mining, agriculture, and cattle industry. Mining and related industry have been operating for centuries in Zacatecas State, Mexico, leaving mining waste dumps that can release trace elements to the topsoil. There are not enough previous studies of thorium concentration in this area. Thirty-three soil samples from different locations from Zacatecas State were analyzed, using alpha-spectrometry and ICP-MS, to estimate the reference value for thorium in surface soil in order to provide regulatory agencies with a tool to verify possible disturbances due to anthropogenic activities. Geoaccumulation indexes and enrichment factors did not reveal significant alterations in topsoil thorium concentration. The average concentration was 13.6 ± 7.6 mg kg-1, which is consistent with the estimated average concentration in the earth crust and is then proposed as average basal concentration for this region. A slight disequilibrium has been found between the natural isotopes of thorium due to the semi-arid nature of the areas and climatic factors.
Asunto(s)
Contaminantes Radiactivos del Suelo , Torio , Animales , Bovinos , México , Minería , Suelo , Contaminantes Radiactivos del Suelo/análisis , Torio/análisisRESUMEN
To investigate whether and in which extension the levels of natural radionuclides in soils vary with parent rock, soil type, and climatic condition factors, a large-scale survey was carried out to cover the semiarid and tropical wet climate regions of the territory of Pernambuco state (Brazil). The radionuclide concentrations were analyzed by gamma spectrometry. The median values of the activity concentrations of 226Ra (20), 228Ra (38) and 40K (458) (Bq kg-1) in the soils agreed with the values reported worldwide. The concentrations of 40K in the soils from the semiarid region were higher than those in the soils from the tropical region, whereas the radium isotope levels were higher in soils from the tropical region. The less-developed soils from the semiarid region, such as Leptosols and Neosols, had the highest 40K levels, unlike the more developed soils (Acrisols and Ferrosols) from the tropical wet area, which showed the lowest contents of 40K and the highest content of radium isotopes. The low 40K contents in well-developed soils may be attributed to the leaching of 40K by the high rainfall rates of the tropical area. In contrast, the rainfall scarcity and high potential evaporation rates of the semiarid environment may be responsible for 40K accumulation in soils. The highest Ra isotope concentrations in the well-drained soils from the tropical climate may be ascribed to the presence of heavy minerals and adsorption on Fe oxyhydroxides, which are very common in those soils. The more developed the soil the lower the K concentration, regardless of the climate. For Ra, the differences are more significant for well-drained soils, and in this case, the tropical climate, with its high rainfall rate, makes the difference. As a conclusion, climate and soil formation time showed high and contrasting influence on the 40K and radium isotope contents in soils. Less developed soils from semiarid had the highest content of 40K, whereas the more developed soils from tropical areas had the highest content of radium.
Asunto(s)
Contaminantes Radiactivos del Suelo/análisis , Brasil , Clima , Monitoreo de Radiación , Radioisótopos , SueloRESUMEN
On 11 March 2011, a 9.0 magnitude earthquake struck the Tohoku region of Japan. The earthquake caused a 15 m tsunami that bombarded the east coast of the island nation. Among the losses was the damage to the Fukushima Daiichi nuclear reactor that lost onsite power and was unable to cool the reactor cores. The reactors melted down and released a plume of radionuclides into the environment. Radiocesiums (Cs and Cs) are the long-lived radionuclides of concern that were deposited along the plume and were distributed on the soil. Radiological decay models are typically used to determine the reduction in external radiation dose over time. However, these radiological decay models do not take into account physical removal by wind and water erosion, or sedimentation in soil outside expected depths. Thirty-five fixed dose-rate monitors were used to record dose rates at 1 mo intervals from the time of installation in Fukushima Prefecture in April 2012 until December 2018 and were used to estimate the effective half-life for radiocesium contamination based on external radiation dose rates. The effective half-life of cesium in the environment was calculated to be 3.2 ± 0.5 y, compared to a theoretical half-life of 7.8 y.
Asunto(s)
Radioisótopos de Cesio/análisis , Accidente Nuclear de Fukushima , Modelos Teóricos , Monitoreo de Radiación/métodos , Contaminantes Radiactivos del Suelo/análisis , Contaminantes Radiactivos del Agua/análisis , Semivida , Humanos , Ceniza Radiactiva/análisisRESUMEN
Natural radioactivity is a public health concern worldwide. Its deleterious effects are largely associated with emitting ionizing particles which generate innumerable toxicological consequences to human being. The present study aimed to describe the research state of the art on natural radioactivity in Brazil through a systematic review limited to articles published in the twenty-first century in the PubMed, SciELO, Lilacs, and Google Scholar databases. A total of 55 research articles were considered for this purpose. Based on the collected sample types, the radiation analysis in most of the scientific reports was performed on solid samples (soil/sediment/rocks), followed by water and air. In fact, most of the available information came from geological studies. A wide range of concentrations and a variety of radionuclides have been assessed, with radium being the most cited. Most of the studies described radiation levels above the international guidelines, and consider the Brazilian territory as a high natural background radiation region (HNBR). In comparison with other HNBR areas, the scientific information about the related risks to human health is still scarce. There is uncertainty about the real impact of natural radioactivity on human health, as there is a lack of scientific information for most of the country about this issue. The analysis and comparison of the available information highlights the potential risks linked to natural radioactivity and the need to incorporate suitable environmental management policies about this issue.
Asunto(s)
Radiación de Fondo , Monitoreo de Radiación , Contaminantes Radiactivos del Suelo/análisis , Brasil , Geología , Humanos , Radiactividad , Radioisótopos/análisis , Radio (Elemento)/análisis , SueloRESUMEN
Unsupported 210Pb (Pbexc) is generated in air and is subsequently deposited on soil surface. The Pbexc can be used for sediment dating, soil erosion/sedimentation and air mass studies. In many cases, 210Pb activity determination (gamma ray 46.5â¯keV) cannot be performed due to the lack of efficiency calibration curve, especially when radioactive patron source is not available. This work presents an alternative methodology to obtain the 210Pb activity values, based on the activity definition and the attenuation coefficient determinations and assuming that soil samples coming from depth higher than 25â¯cm only contain 210Pb generated in the soil (Pbexc free, i.e., for those soil layers the 210Pb activity is equal to the 226Ra activity, at secular equilibrium). The proposed methodology was evaluated using soils from La Plata region, Argentina. The same soil samples were also analyzed in a second laboratory by the conventional methodology. The obtained results indicated that the proposed procedure can be used as a good alternative in cases where a calibration sample is not available.
Asunto(s)
Radioisótopos de Plomo/análisis , Monitoreo de Radiación/métodos , Contaminantes Radiactivos del Suelo/análisis , Argentina , SueloRESUMEN
The radiometric monitoring carried out in the present study allowed the discovery of anomalous granite outcrops in natural radionuclides in the rural area of São Mamede in the state of Paraíba, Brazil. The characterisation study made it possible to determine maximum specific concentrations of approximately 199 kBq kg-1 of 238U, 85 kBq kg-1 of 226Ra, 26 kBq kg-1 of 232Th and 24 kBq kg-1 of 40K. Models for environmental dosimetry were applied, which resulted in obtaining the following quantities: radium equivalent (Raeq), indices of external (Hex), internal (Hin) and representative (Iyr) damage, and the effective outdoor dose (HE). The maximum results presented were approximately 123 kBq kg-1, 332, 562, 832, and 68 mSv y-1, respectively. Consequently, it was possible to define the region as of high radioactive background due to isolated rocky outcrops located in the rural area of the mentioned municipality.
Asunto(s)
Radiación de Fondo , Radioisótopos de Potasio/análisis , Monitoreo de Radiación/métodos , Radio (Elemento)/análisis , Contaminantes Radiactivos del Suelo/análisis , Torio/análisis , Uranio/análisis , BrasilRESUMEN
Inhaled radon and its progenies induce health concern due to high activity-concentration in selected thermal spas of Boyacá region. Hydrogeothermal water sources in a high risk seismic area, are studied to determine by water bubbling method radon concentration values; their occurrence is between few hundreds and 2000â¯Bqâ¯dm-3. Deposits, existing in this area, reach at the surface soil gas radon concentration up to 210â¯kBqâ¯m-3. Maintenance workers, health tourists and visitor's possible detrimental health effects, are discussed in relation to radon balneotherapy beneficial aspects.
Asunto(s)
Balneología , Manantiales de Aguas Termales/análisis , Radón/análisis , Contaminantes Radiactivos del Agua/análisis , Colombia , Humanos , Turismo Médico , Exposición Profesional/efectos adversos , Exposición Profesional/análisis , Monitoreo de Radiación , Radón/efectos adversos , Contaminantes Radiactivos del Suelo/efectos adversos , Contaminantes Radiactivos del Suelo/análisis , Contaminantes Radiactivos del Agua/efectos adversosRESUMEN
The natural radioactivity and the associated radiation hazards of soils from the Cumanayagua Granitoide-Granitic massif in the central south of Cuba have been studied. Mass activities of the natural radionuclides 238U, 232Th and 40K varied in the ranges 10.4-33, 4.6-21.7 and 381-1201 Bq kg-1, respectively. The radium equivalent activity (91.4 ± 22.1 Bq kg-1), absorbed dose rate (45.6 ± 11.1 nGy h-1), annual effective dose rate (56.1 ± 13.7 µSv y-1) and the external hazard index (0.25 ± 0.06) have been calculated and compared with the internationally approved values. According to these results, the area can be regarded as an area with normal natural background radiation and may not pose radiological risks to the inhabitants owing to harmful effects of ionizing radiation from the natural radionuclides in soils. This study provides background radioactivity concentrations in Cumanayagua Granitoide area and generate a baseline data for radiological mapping of Cuba in the future.
Asunto(s)
Materiales de Construcción/análisis , Sedimentos Geológicos/análisis , Radioisótopos de Potasio/análisis , Dióxido de Silicio/química , Contaminantes Radiactivos del Suelo/análisis , Suelo/química , Torio/análisis , Uranio/análisis , Radiación de Fondo , Cuba , Humanos , Dosis de Radiación , Monitoreo de RadiaciónRESUMEN
Present study area, which is located in the Central Range Fault (CRF) in the island of Trinidad, can provide solution to that problem as this strike-slip fault system is reported to be active in present time (during Holocene, most current geological epoch) with a movement of geodetic rate of 12⯱â¯3â¯mm/yr. Most recent work, with improved GPS time series analysis indicated that as creeping fault rather than locked fault. Moreover, the selected fault system is accompanied by mud volcanoes, which can amplify the level of radiation activity by slight but significant anomalies as described by some researchers from other areas. Furthermore, being one of the first environmental radiation study in the Caribbean Islands, this study is significant. With the aim to achieve a continuous monitoring of radiological data to assess the activity along CRF for possible earthquake forecasting, objectives of this preliminary investigation are to delineate CRFZ using radiation survey and to investigate the potential of using this survey to detect tectonic activities in this zone. As a pilot study, radiation measurements were carried out with the help of a portable Geiger Muller counter in 52 locations along the 25â¯km long section of CRF between Naved Dam and Pointe-a-Pierre. Radiation measurements were taken both at 1â¯m level above the surface and at nearly 1â¯m below the ground. Results from this pilot study showed that lithology was not the lone contributor to terrestrial radiation levels, as CRFZ and associated fissure plane have good control also (â¼3-5 times higher than the average background level). Although present study was not able to indicate the possibility of earthquakes in recent times (as previously stated), however, elevated radiation values in the vicinity of CRF, associated fissures (possibly interconnected fractures) and active mud volcanoes indicate possible activity in the study area. However, detail and periodic radiological studies are required before concluding that CRF is a creep fault rather than a locked fault.
Asunto(s)
Monitoreo de Radiación , Contaminantes Radiactivos del Suelo/análisis , Terremotos , Trinidad y Tobago , Erupciones VolcánicasRESUMEN
236U, 239Pu and 240Pu are present in soils mainly as a result of the local- and global-fallout from the atmospheric nuclear weapons tests carried out mainly in the 1950's and 1960's. In this work we provide new data on the presence of 236U and 239,240Pu in surface soils (i.e. up to 5â¯cm depth) from Chile and Africa. The results were obtained by low-energy Accelerator Mass Spectrometry (AMS). In the case of the Chilean samples, 236U/239Pu atom ratios show a high variability and are in general higher than the reported value for the global fallout in the Northern Hemisphere, ranging from 0.2 to 1.5. The 236U atomic concentrations range from 3.5â¯×â¯106 to 9.1â¯×â¯106 atoms/g, and are at least two orders of magnitude lower than the reported values in the Northern Hemisphere. The measured 240Pu/239Pu atom ratio in soils from South-Africa and Mozambique are of about 0.17, in agreement with the expected one for global-fallout at those coordinates. To best knowledge of the authors the present work is the first publication on 236U concentrations and 236U/239Pu atom ratios in soils from South-America and Africa.