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1.
ACS Appl Mater Interfaces ; 14(2): 3000-3007, 2022 Jan 19.
Artículo en Inglés | MEDLINE | ID: mdl-34990111

RESUMEN

Fabric-based wearable electronics are showing advantages in emerging applications in wearable devices, Internet of everything, and artificial intelligence. Compared to the one with organic materials, devices based on inorganic semiconductors (e.g., GaN) commonly show advantages of superior characteristics and high stability. Upon the transfer of GaN-based heterogeneous films from their rigid substrates onto flexible/fabric substrates, changes in strain would influence the device performance. Here, we demonstrate the transfer of InGaN/GaN multiple quantum well (MQW) films onto flexible/fabric substrates with an effective lift-off technique. The physical properties of the InGaN/GaN MQWs film are characterized by atomic force microscopy and high-resolution X-ray diffraction, indicating that the transferred film does not suffer from huge damage. Excellent flexible properties are observed in the film transferred on fabric, and the photoluminescence (PL) intensity is enhanced by the piezo-phototronic effect, which shows an increase of about 10% by applying an external strain with increasing the film curvature to 6.25 mm-1. Moreover, energy band diagrams of the GaN/InGaN/GaN heterojunction at different strains are illustrated to clarify the internal modulation mechanism by the piezo-phototronic effect. This work would facilitate the guidance of constructing high-performance devices on fabrics and also push forward the rapid development of flexible and wearable electronics.

2.
Adv Mater ; 33(32): e2101263, 2021 Aug.
Artículo en Inglés | MEDLINE | ID: mdl-34176170

RESUMEN

2D hybrid perovskites are very attractive for optoelectronic applications because of their numerous exceptional properties. The emerging 2D perovskite ferroelectrics, in which are the coupling of spontaneous polarization and piezoelectric effects, as well as photoexcitation and semiconductor behaviors, have great appeal in the field of piezo-phototronics that enable to effectively improve the performance of optoelectronic devices via modulating the electro-optical processes. However, current studies on 2D perovskite ferroelectrics focus on bulk ceramics that cannot endure irregular mechanical deformation and limit their application in flexible optoelectronics and piezo-phototronics. Herein, we synthesize ferroelectric EA4 Pb3 Br10 single-crystalline thin-films (SCFs) for integration into flexible photodetectors. The in-plane multiaxial ferroelectricity is evident within the EA4 Pb3 Br10 SCFs through systematic characterizations. Flexible photodetectors based on EA4 Pb3 Br10 SCFs are achieved with an impressive photodetection performance. More importantly, optoelectronic EA4 Pb3 Br10 SCFs incorporated with in-plane ferroelectric polarization and effective piezoelectric coefficient show great promise for the observation of piezo-phototronic effect, which is capable of greatly enhancing the photodetector performance. Under external strains, the responsivity of the flexible photodetectors can be modulated by piezo-phototronic effect with a remarkable enhancement up to 284%. Our findings shed light on the piezo-phototronic devices and offer a promising avenue to broaden functionalities of hybrid perovskite ferroelectrics.

3.
ACS Nano ; 9(3): 3143-50, 2015 Mar 24.
Artículo en Inglés | MEDLINE | ID: mdl-25712580

RESUMEN

A high-resolution dynamic tactile/pressure display is indispensable to the comprehensive perception of force/mechanical stimulations such as electronic skin, biomechanical imaging/analysis, or personalized signatures. Here, we present a dynamic pressure sensor array based on pressure/strain tuned photoluminescence imaging without the need for electricity. Each sensor is a nanopillar that consists of InGaN/GaN multiple quantum wells. Its photoluminescence intensity can be modulated dramatically and linearly by small strain (0-0.15%) owing to the piezo-phototronic effect. The sensor array has a high pixel density of 6350 dpi and exceptional small standard deviation of photoluminescence. High-quality tactile/pressure sensing distribution can be real-time recorded by parallel photoluminescence imaging without any cross-talk. The sensor array can be inexpensively fabricated over large areas by semiconductor product lines. The proposed dynamic all-optical pressure imaging with excellent resolution, high sensitivity, good uniformity, and ultrafast response time offers a suitable way for smart sensing, micro/nano-opto-electromechanical systems.


Asunto(s)
Electricidad , Nanotecnología/instrumentación , Imagen Óptica , Fenómenos Ópticos , Fotones , Presión , Semiconductores , Galio , Indio
4.
Adv Mater ; 27(9): 1553-60, 2015 Mar 04.
Artículo en Inglés | MEDLINE | ID: mdl-25589428

RESUMEN

An optical-fiber-nanowire hybridized UV-visible photodetector (PD) is reported. The PD is designed to allow direct integration in optical communication systems without requiring the use of couplers via fiber-welding technology. The PD works in two modes: axial and off-axial illumination mode. By using the piezo-phototronic effect, the performance of the PD is enhanced/optimized by up to 718% in sensitivity and 2067% in photoresponsivity.

5.
Adv Mater ; 26(42): 7209-16, 2014 Nov 12.
Artículo en Inglés | MEDLINE | ID: mdl-25205535

RESUMEN

Two-dimensional finite-element simulation of the piezo-phototronic effect in p-n-junction-based devices is carried out for the first time. A charge channel can be induced at the p-n junction interface when strain is applied, given the n-side is a piezoelectric semiconductor and the p-type side is non-piezoelectric semiconductor. This provides the first simulated evidence supporting the previously suggested mechanism responsible for the experimentally observed gigantic change of light-emission efficiency in piezo-phototronic light-emitting devices.

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