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J Chromatogr A ; 1470: 104-110, 2016 Oct 28.
Artículo en Inglés | MEDLINE | ID: mdl-27693015

RESUMEN

Silica gel containing silver ions was prepared and characterized. Silica was organofunctionalized with 3-mercaptopropyl group by using grafting reaction followed by silver ions adsorption (silver covalently bonded to mercaptopropyl silca gel, Ag-MPSG). The organofunctionalization and silver coordination were observed by transmission infrared spectroscopy and elemental analyses (CHN and EDS). The textural characteristics were studied by N2 adsorption-desorption isotherms. Additionally, optical properties were studied by diffuse reflectance spectroscopy. The Ag-MPSG material was employed as stationary phase for the first time for fractionation of a heavy gas oil sample resulting in a fraction that is richer in polycyclic aromatic sulfur heterocycles (PASH). The fractions were analyzed by comprehensive two-dimensional gas chromatography with time-of-flight mass spectrometric detector and Ag-MPSG material provided similar fractionation performance when compared to conventional material [palladium covalently bonded to mercaptopropyl silca gel, Pd(II)-MPSG] usually employed for the same purpose and as the cost of silver is less than the one of palladium, the cost of the fractionation phase was reduced.


Asunto(s)
Aceites Combustibles/análisis , Paladio/química , Gel de Sílice/química , Plata/química , Tiofenos/aislamiento & purificación , Fraccionamiento Químico , Cromatografía de Gases y Espectrometría de Masas , Compuestos de Sulfhidrilo/química
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