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1.
ACS Nano ; 16(4): 6676-6686, 2022 Apr 26.
Artículo en Inglés | MEDLINE | ID: mdl-35293217

RESUMEN

Currently, graphene films are expected to achieve real applications in various fields. However, the conventional synthesis methods still have intrinsic limitations, especially not being applicable on a surface with high curvature. Herein, an ultrafast synthesis method was developed for graphene and turbostratic graphite growth by a single subsecond pulse of microwaves generated by a household magnetron. We succeeded in growing high-quality around 10-layered turbostratic graphite in 0.16 s directly on the surface of an atomic force microscope probe and maintaining a tip curvature radius of less than 30 nm. The thus-produced probes showed high conductivity and tip durability. Moreover, turbostratic graphite film was also demonstrated to grow on the surface of dielectric Si flat substrates in a full coverage. Graphene can also grow on metallic Ni tips by this method. Our microwave ultrafast method can be used to grow high-quality graphene in a facile, efficient, and economical way.

2.
Adv Mater ; 33(30): e2101673, 2021 Jul.
Artículo en Inglés | MEDLINE | ID: mdl-34106491

RESUMEN

Whilst quantum computing has recently taken great leaps ahead, the development of quantum memories has decidedly lagged behind. Quantum memories are essential devices in the quantum technology palette and are needed for intermediate storage of quantum bit states and as quantum repeaters in long-distance quantum communication. Current quantum memories operate at cryogenic, mostly sub-Kelvin temperatures and require extensive and costly peripheral hardware. It is demonstrated that ensembles of weakly coupled molecular spins show long coherence times and can be used to store microwave pulses of arbitrary phase. These studies exploit strong coupling of the spin ensemble to special 3D microwave resonators. Most importantly, these systems operate at room temperature.

3.
Appl Phys B ; 123(1): 12, 2017.
Artículo en Inglés | MEDLINE | ID: mdl-32214686

RESUMEN

Elitzur and Vaidman have proposed a measurement scheme that, based on the quantum superposition principle, allows one to detect the presence of an object-in a dramatic scenario, a bomb-without interacting with it. It was pointed out by Ghirardi that this interaction-free measurement scheme can be put in direct relation with falsification tests of the macro-realistic worldview. Here we have implemented the "bomb test" with a single atom trapped in a spin-dependent optical lattice to show explicitly a violation of the Leggett-Garg inequality-a quantitative criterion fulfilled by macro-realistic physical theories. To perform interaction-free measurements, we have implemented a novel measurement method that correlates spin and position of the atom. This method, which quantum mechanically entangles spin and position, finds general application for spin measurements, thereby avoiding the shortcomings inherent in the widely used push-out technique. Allowing decoherence to dominate the evolution of our system causes a transition from quantum to classical behavior in fulfillment of the Leggett-Garg inequality.

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