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We theoretically show the asymmetric spin wave transmission in a coupled waveguide-skyrmion structure, where the skyrmion acts as an effective nanocavity allowing the whispering gallery modes for magnons. The asymmetry originates from the chiral spin wave mode localized in the circular skyrmion wall. By inputting two-tone excitations and mixing them in the skyrmion wall, we observe a unidirectional output magnon frequency comb propagating in the waveguide with a record number of teeth (>50). This coupled waveguide-cavity structure turns out to be a universal paradigm for generating asymmetric magnon frequency combs, where the cavity can be generalized to other magnetic structures that support the whispering gallery mode of magnons. Our results advance the understanding of the nonlinear interaction between magnons and magnetic textures and open a new pathway to exploring the asymmetric spin wave transmission and to steering the magnon frequency comb.

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Since their inception, frequency combs generated in microresonators, known as microcombs, have sparked significant scientific interests. Among the various applications leveraging microcombs, soliton microcombs are often preferred due to their inherent mode-locking capability. However, this choice introduces additional system complexity because an initialization process is required. Meanwhile, despite the theoretical understanding of the dynamics of other comb states, their practical potential, particularly in applications like sensing where simplicity is valued, remains largely untapped. Here, we demonstrate controllable generation of sub-combs that bypasses the need for accessing bistable regime. And in a graphene-sensitized microresonator, the sub-comb heterodynes produce stable, accurate microwave signals for high-precision gas detection. By exploring the formation dynamics of sub-combs, we achieved 2 MHz harmonic comb-to-comb beat notes with a signal-to-noise ratio (SNR) greater than 50 dB and phase noise as low as - 82 dBc/Hz at 1 MHz offset. The graphene sensitization on the intracavity probes results in exceptional frequency responsiveness to the adsorption of gas molecules on the graphene of microcavity surface, enabling detect limits down to the parts per billion (ppb) level. This synergy between graphene and sub-comb formation dynamics in a microcavity structure showcases the feasibility of utilizing microcombs in an incoherent state prior to soliton locking. It may mark a significant step toward the development of easy-to-operate, systemically simple, compact, and high-performance photonic sensors.

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The portable Raman spectrometer boasts portability, rapid analysis, and high flexibility. It stands as a crucial and powerful technical tool for analyzing the chemical composition of samples, whether biological or non-biological, across diverse fields. To improve the resolution of grating spectrometers and ensure a wide spectral range, many spectrometer systems have been designed with double-grating structures. However, the impact of external forces, such as installation deviations and inevitable collisions, may cause differences between the actual state of the internal spectrometer components and their theoretical values. Therefore, spectrometers must be calibrated to establish the relationship between the wavelength and the pixel positions. The characteristic peaks of commonly used calibration substances are primarily distributed in the 200-2000 cm-1 range. The distribution of characteristic peaks in other wavenumber ranges is sparse, especially for spectrometers with double-channel spectral structures and wide spectral ranges. This uneven distribution of spectral peaks generates significant errors in the polynomial fitting results used to calibrate spectrometers. Therefore, to satisfy the calibration requirements of a dual-channel portable Raman spectrometer with a wide spectral range, this study designed a calibration method based on an optical frequency comb, which generates dense and uniform comb-like spectral signals at equal intervals. The method was verified experimentally and compared to the traditional calibration method of using a mercury-argon lamp. The results showed that the error bandwidth of the calibration results of the proposed method was significantly smaller than that of the mercury-argon lamp method, thus demonstrating a substantial improvement in the calibration accuracy.

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Cavity-enhanced direct frequency comb spectroscopy (CE-DFCS) is widely used as a highly sensitive gas sensing technology in various gas detection fields. For the on-axis coupling incidence scheme, the detection accuracy and stability are seriously affected by the cavity-mode noise, and therefore, stable operation inevitably requires external electronic mode-locking and sweeping devices, substantially increasing system complexity. To address this issue, we propose off-axis cavity-enhanced optical frequency comb spectroscopy from both theoretical and experimental aspects, which is applied to the detection of single- and dual-gas of carbon monoxide (CO) and carbon dioxide (CO2) in the near-infrared. An erbium-doped fiber frequency comb with a repetition frequency of ∼41.709 MHz is coupled into a resonant cavity with a length of ∼360 mm in an off-axis manner, exciting numerous high-order modes to effectively suppress cavity-mode noise. The performance of multiple machine learning models is compared for the inversion of a single/dual gas concentration. A few absorbance spectra are collected to build a sample data set, which is then utilized for model training and learning. The results demonstrate that the Particle Swarm Optimization Support Vector Machine (PSO-SVM) model achieves the highest predictive accuracy for gas concentration and is ultimately applied to the detection system. Based on Allan deviation, the detection limit for CO in single-gas detection can reach 8.247 parts per million by volume (ppmv) by averaging 87 spectra. Meanwhile, for simultaneous CO2/CO measurement with highly overlapping absorbance spectra, the LoD can be reduced to 13.196 and 4.658 ppmv, respectively. The proposed optical gas sensing technique indicates the potential for the development of a field-deployable and intelligent sensor system capable of simultaneous detection of multiple gases.

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A novel method for the generation of an optical frequency comb (OFC) is presented. The proposed approach uses a laser diode with optical feedback and operating at a specific nonlinear dynamic state named periodic window. In this case, the laser spectrum exhibits a feature with a series of discrete, equally spaced frequency components, and the repetition rate can be flexibly adjusted by varying the system parameters (e.g., external cavity length), which can provide many potential applications. As an application example, a dual-OFC system for distance measurement is presented. The results demonstrate the system's ability to achieve target distance detection, underscoring its potential for real-world applications in this field.

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Quantum dots can modify the properties of the whispering gallery mode resonators (WGMRs) used in various potential applications. A deposition of a suitable nanomaterial for the surface functionalization of WGMRs allows for the achievement of high quality (Q) factors. Here, we show that the WGMR surface can be functionalized using quantum dots. We demonstrate that WGMRs covered with thin layers of HgS and PbS quantum dots are suitable for third-harmonic generation due to the high Q factor of the developed microresonators, thus significantly lowering the pumping power required for nonlinear optical interactions.

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Two algorithms of data processing are proposed to shorten the unmeasurable dead-zone close to the zero-position of measurement, i.e., the minimum working distance of a dispersive interferometer using a femtosecond laser, which is a critical issue in millimeter-order short-range absolute distance measurement. After demonstrating the limitation of the conventional data processing algorithm, the principles of the proposed algorithms, namely the spectral fringe algorithm and the combined algorithm that combines the spectral fringe algorithm with the excess fraction method, are presented, together with simulation results for demonstrating the possibility of the proposed algorithms for shortening the dead-zone with high accuracy. An experimental setup of a dispersive interferometer is also constructed for implementing the proposed data processing algorithms over spectral interference signals. Experimental results demonstrate that the dead-zone using the proposed algorithms can be as small as half of that of the conventional algorithm while measurement accuracy can be further improved using the combined algorithm.

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Rapid testing is essential to fighting pandemics such as coronavirus disease 2019 (COVID-19), the disease caused by the severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2). Exhaled human breath contains multiple volatile molecules providing powerful potential for non-invasive diagnosis of diverse medical conditions. We investigated breath detection of SARS-CoV-2 infection using cavity-enhanced direct frequency comb spectroscopy (CE-DFCS), a state-of-the-art laser spectroscopic technique capable of a real-time massive collection of broadband molecular absorption features at ro-vibrational quantum state resolution and at parts-per-trillion volume detection sensitivity. Using a total of 170 individual breath samples (83 positive and 87 negative with SARS-CoV-2 based on reverse transcription polymerase chain reaction tests), we report excellent discrimination capability for SARS-CoV-2 infection with an area under the receiver-operating-characteristics curve of 0.849(4). Our results support the development of CE-DFCS as an alternative, rapid, non-invasive test for COVID-19 and highlight its remarkable potential for optical diagnoses of diverse biological conditions and disease states.

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The present study proposes a terahertz quantum cascade laser frequency comb (THz QCL FC) with a semi-insulated surface plasma waveguide characterized by a low threshold current density, high power and a wide current dynamic range. The gain dispersion value and the nonlinear susceptibility were optimized based on the combination of a hybrid bound-to-continuum active region with a semi-insulated surface plasmon waveguide. Without any extra dispersion compensator, stable frequency comb operation within a current dynamic range of more than 97% of the total was revealed by the intermode beat note map. Additionally, a total comb spectral emission of about 300 GHz centered around 4.6 THz was achieved for a 3 mm long and 150 µm wide device. At 10 K, a maximum output power of 22 mW was obtained with an ultra-low threshold current density of 64.4 A·cm-2.

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Radars can be used as sensors to detect the breathing of victims trapped under layers of building materials in catastrophes like earthquakes or gas explosions. In this contribution, we present the implementation of a novel frequency comb continuous wave (FCCW) bioradar module using a commercial software-defined radio (SDR). The FCCW radar transmits multiple equally spaced frequency components simultaneously. The data acquisition of the received combs is frequency domain-based. Hence, it does not require synchronization between the transmit and receive channels, as time domain-based broadband radars, such as ultra wideband (UWB) pulse radar and frequency-modulated CW (FMCW) radar, do. Since a frequency comb has an instantaneous wide bandwidth, the effective scan rate is much higher than that of a step frequency CW (SFCW) radar. This FCCW radar is particularly suitable for small motion detection. Using inverse fast Fourier transform (IFFT), we can decompose the received frequency comb into different ranges and remove ghost signals and interference of further range intervals. The frequency comb we use in this report has a bandwidth of only 60 MHz, resulting in a range resolution of up to 2.5 m, much larger than respiration-induced chest wall motions. However, we demonstrate that in the centimeter range, motions can be detected and evaluated by processing the received comb signals. We want to integrate the bioradar into an unmanned aircraft system for fast and safe search and rescue operations. As a trade-off between ground penetrability and the size and weight of the antenna and the radar module, we use 1.3 GHz as the center frequency. Field measurements show that the proposed FCCW bioradar can detect an alive person through different nonmetallic building materials.

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Since the turn of the millennium, the development and commercial availability of optical frequency combs has led to a steadily increase of worldwide installed frequency combs and a growing interest in using them for industrial-related metrology applications. Especially, GPS-referenced frequency combs often serve as a "self-calibrating" length standard for laser wavelength calibration in many national metrology institutes with uncertainties better than u = 1 × 10-11. In this contribution, the application of a He-Ne laser source permanently disciplined to a GPS-referenced frequency comb for the interferometric measurements in a nanopositioning machine with a measuring volume of 200 mm × 200 mm × 25 mm (NPMM-200) is discussed. For this purpose, the frequency stability of the GPS-referenced comb is characterized by heterodyning with a diode laser referenced to an ultrastable cavity. Based on this comparison, an uncertainty of u = 9.2 × 10-12 (τ = 8 s, k = 2) for the GPS-referenced comb has been obtained. By stabilizing a tunable He-Ne source to a single comb line, the long-term frequency stability of the comb is transferred onto our gas lasers increasing their long-term stability by three orders of magnitude. Second, short-term fluctuations-related length measurement errors were reduced to a value that falls below the nominal resolving capabilities of our interferometers (ΔL/L = 2.9 × 10-11). Both measures make the influence of frequency distortions on the interferometric length measurement within the NPMM-200 negligible. Furthermore, this approach establishes a permanent link of interferometric length measurements to an atomic clock.

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Generating a coherent optical frequency comb at an arbitrary wavelength is important for fields such as precision spectroscopy and optical communications. Dark solitons which are coherent states of optical frequency combs in normal dispersion microresonators can extend the operating wavelength range of these combs. While the existence and dynamics of dark solitons has been examined extensively, requirements for the modal interaction for accessing the soliton state in the presence of a strong Raman interaction at near visible wavelengths has been less explored. Here, analysis on the parametric and Raman gain in a silica microresonator is performed, revealing that four-wave mixing parametric gain which can be created by a modal-interaction-aided additional frequency shift is able to exceed the Raman gain. The existence range of the dark soliton is analyzed as a function of pump power and detuning for given modal coupling conditions. We anticipate these results will benefit fields requiring optical frequency combs with high efficiency and selectable wavelength such as biosensing applications using silica microcavities that have a strong Raman gain in the normal dispersion regime.

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Cavity-enhanced electro-optic comb generators (CEEOCGs) can provide optical frequency combs with excellent stability and configurability. The existing methods for CEEOCGs spectrum characterization, however, are based on approximations and have suffered from either iterative calculations or limited applicable conditions. In this paper, we show a spectrum characterization method by accumulating the optical electrical field with respect to the count of the round-trip propagation inside of CEEOCGs. The identity transformation and complete analysis of the intracavity phase delay were conducted to eliminate approximations and be applicable to arbitrary conditions, respectively. The calculation efficiency was improved by the noniterative matrix operations. Setting the maximum propagation count as 1000, the spectrum of the center ±300 comb modes can be characterized with merely the truncation error of floating-point numbers within 1.2 s. More importantly, the effects of all CEEOCG parameters were comprehensively characterized for the first time. Accordingly, not only the exact working condition of CEEOCG can be identified for further optimization, but also the power of each comb mode can be predicted accurately and efficiently for applications in optical communications and waveform synthesis.

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The investigation of optical microcavity solitons is in demand both for applications and basic science. Despite the tremendous progress in the study of microresonator solitons, there is still no complete understanding of all features of their nonlinear dynamics in various regimes. Controlling soliton properties is also of great interest. We proposed and investigated experimentally and theoretically a simple and easily reproducible way to generate Raman solitons with controllable spectral width in an anomalous dispersion region in a functionalized silica microsphere with whispering gallery modes (WGMs) driven in a normal dispersion regime. To functionalize the microsphere, coating (TiO2 + graphite powder) was applied at the pole. The coating is used for effective thermalization of the radiation of an auxiliary laser diode launched through the fiber stem holding the microsphere to control detuning of the pump frequency from exact resonance due to the thermo-optical shift of the WGM frequencies. We demonstrated that the thermo-optical control by changing the power of an auxiliary diode makes it possible to switch on/off the generation of Raman solitons and control their spectral width, as well as to switch Raman generation to multimode or single-mode. We also performed a detailed theoretical analysis based on the Raman-modified Lugiato-Lefever equation and explained peculiarities of intracavity nonlinear dynamics of Raman solitons. All experimental and numerically simulated results are in excellent agreement.

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In the future space-borne gravitational wave (GW) detector, the optical transponder scheme, i.e., the phase-locking scheme, will be utilized so as to maintain the signal-to-noise ratio (SNR). In this case, the whole constellation will share one common laser equivalently, which enables the considerable simplification of time delay interferometry (TDI) combinations. Recently, and remarkably, the unique combination of TDI and optical frequency comb (OFC) has shown a bright prospect for the future space-borne missions. When the laser frequency noise and the clock noise are synchronized using OFC as the bridge, the data streams will be reasonably simplified. However, in the optical transponder scheme, the weak-light phase-locking (WLPL) loops could bring additional noises. In this work, we analyze the phase-locking scheme with OFC and transfer characteristics of the noises including the WLPL noise. We show that the WLPL noise can be efficiently reduced by using the specific TDI combination, and the cooperation of phase-locking and frequency combs can greatly simplify the post-processing.

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Photoacoustic spectroscopy (PAS) using two optical combs is a new-born technique, offering appealing features, including broad optical bandwidths, high resolutions, fast acquisition speeds, and wavelength-independent photoacoustic detection, for chemical sensing. However, its further application to, e.g., trace detection, is jeopardized due to the fundamentally and technically limited sensitivity and specificity. Here, we take a different route to comb-enabled PAS with acoustically enhanced sensitivity and nonlinear spectral hole-burning defined resolution. We demonstrate dual-comb quartz-enhanced PAS with two near-infrared electro-optic combs and a quartz tuning fork. Comb-line-resolved multiplexed spectra are acquired for acetylene with a single-pass detection limit at the parts-per-billion level. The technique is further extended to the mid-infrared (for methane), enabling improved sensitivity. More importantly, we measure nonlinear dual-comb photoacoustic spectra for the 12C2H2 ν1 + ν3 band P(17) transition with sub-Doppler pressure-broadening dominated homogeneous linewidths (e.g., 45.8 MHz), hence opening up new opportunities for Doppler-free photoacoustic gas sensing.

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Since the dispersive interferometry (DPI) based on optical frequency combs (OFCs) was proposed, it has been widely used in absolute distance measurements with long-distance and high precision. However, it has a serious problem for the traditional DPI based on the mode-locked OFC. The error of measurements caused by using the fast Fourier transform (FFT) algorithm to process signals cannot be overcome, which is due to the non-uniform sampling intervals in the frequency domain of spectrometers. Therefore, in this paper, we propose a new mathematical model with a simple form of OFC to simulate and analyze various properties of the OFC and the principle of DPI. Moreover, we carry out an experimental verification, in which we adopt the Lomb-Scargle algorithm to improve the accuracy of measurements of DPI. The results show that the Lomb-Scargle algorithm can effectively reduce the error caused by the resolution, and the error of absolute distance measurement is less than 12 µm in the distance of 70 m based on the mode-locked OFC.

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Nanomechanical resonances coupled to microwave cavities can be excited, measured, and controlled simultaneously using electromechanical back-action phenomena. Examples of these effects include sideband cooling and amplification, which are commonly described through linear equations of motion governed by an effective optomechanical Hamiltonian. However, this linear approximation is invalid when the pump-induced cavity microwave field is large enough to trigger optomechanical nonlinearities, resulting in phenomena like frequency combs. Here, we employ a niobium-based superconducting electromechanical device to explore the generation of microwave frequency combs. We observe the formation of combs around a microwave resonant frequency (3.78 GHz) with 8-MHz frequency spacing, equal to the mechanical resonant frequency. We investigate their dynamics for different optomechanical parameters, including detuning, pump powers, and cavity decay rates. Our experimental results show excellent agreement with numerical modeling. These electromechanical frequency combs can be beneficial in nanomechanical sensing applications that require precise electrical tracking of mechanical resonant frequencies.

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Dual-comb multiheterodyne spectroscopy is a well-established technology for the highly sensitive real-time detection and measurement of the optical spectra of samples, including gases and fiber sensors. However, a common drawback of dual-comb spectroscopy is the need for a broadband amplitude-resolved absorption or reflection measurement, which increases the complexity of the dual comb and requires the precise calibration of the optical detection. In the present study, we present an alternative dispersion-based approach applied to fiber Bragg grating sensors in which the dual comb is compacted by a single dual-drive-unit optical modulator, and the fiber sensor is part of a dispersion interferometer. The incident dual comb samples a few points in the spectrum that are sensitive to Bragg wavelength changes through the optical phase. The spectra reading is improved due to the external interferometer and is desensitized to changes in the amplitude of the comb tones. The narrow-band detection of the fiber sensor dispersion changes that we demonstrate enables the compact, cost-effective, high-resolution multiheterodyne interrogation of high-throughput interferometric fiber sensors. These characteristics open its application both to the detection of fast phenomena, such as ultrasound, and to the precise measurement at high speed of chemical-/biological-sensing samples. The results with a low-reflectivity fiber Bragg grating show the detection of dynamic strain in the range of 215 nε with a 30 dB signal to noise ratio and up to 130 kHz (ultrasonic range).

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Frequency combs (FCs)-spectra containing equidistant coherent peaks-have enabled researchers and engineers to measure the frequencies of complex signals with high precision, thereby revolutionising the areas of sensing, metrology and communications and also benefiting the fundamental science. Although mostly optical FCs have found widespread applications thus far, in general FCs can be generated using waves other than light. Here, we review and summarise recent achievements in the emergent field of acoustic frequency combs (AFCs), including phononic FCs and relevant acousto-optical, Brillouin light scattering and Faraday wave-based techniques that have enabled the development of phonon lasers, quantum computers and advanced vibration sensors. In particular, our discussion is centred around potential applications of AFCs in precision measurements in various physical, chemical and biological systems in conditions where using light, and hence optical FCs, faces technical and fundamental limitations, which is, for example, the case in underwater distance measurements and biomedical imaging applications. This review article will also be of interest to readers seeking a discussion of specific theoretical aspects of different classes of AFCs. To that end, we support the mainstream discussion by the results of our original analysis and numerical simulations that can be used to design the spectra of AFCs generated using oscillations of gas bubbles in liquids, vibrations of liquid drops and plasmonic enhancement of Brillouin light scattering in metal nanostructures. We also discuss the application of non-toxic room-temperature liquid-metal alloys in the field of AFC generation.