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Emission reduction, heat mitigation, and improved access to water and food provision are increasingly critical challenges for urban areas in the context of global climate change adaptation and mitigation. The revival of local agricultural production is often lauded as a potential nature-based solution. However, an expansion of peri-urban agriculture (peri-UA) may entail significant ecosystem trade-offs. This study explores the impacts on the food-water-climate nexus of different scenarios of peri-urban agricultural expansion in a semi-arid, Mediterranean climate, addressing local food provision, freshwater use, local temperature regulation, global climate change mitigation, and the trade-offs thereof. We estimate food provision and irrigation water requirements based on a georeferenced urban metabolism approach along with atmospheric and biosphere models to examine four land-use scenarios in the Metropolitan Area of Barcelona. Our study reveals that a 31 % (+17.27 km2) and 115 % (+64.25 km2) increase in the current peri-UA in the AMB, results in an increase in local food production of 24 % (+16,503 tons year-1) and 86 % (+58,940 tons year-1), and irrigation water requirements by 10.0 % (+3.2 hm3) and 43.5 % (+14.1 hm3), respectively. The expansion of irrigated peri-UA potentially reduces near-surface temperatures by 0.7 °C, albeit temperature reductions in the densest urban areas are minimal. Since the additional peri-UA is achieved by replacing natural non-forested and forest areas, the simulations predict reductions in the net ecosystem productivity of up to 18.5 % and total carbon stocks by 3.3 %. This integrated approach combining urban metabolism and atmospheric modelling to determine the trade-offs appears to be a promising tool for informing land-use decision-making in the context of urban climate adaptation and mitigation.

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Cities face the challenges of supplying food and managing organic municipal solid waste (OMSW) sustainably amid increasing urbanization rates. Urban agriculture (UA) can help with this effort by producing local crops that are fertilized with nutrients recovered from compost generated from OMSW. This research aims to determine the potential of OMSW compost to supply the nitrogen-phosphorus-potassium (NPK) demand of UA and the environmental benefits of replacing mineral fertilizer from a life cycle perspective. The Metropolitan Area of Barcelona (AMB) serves as the case study given its commitment to reuse biowaste according to the Revised Waste Framework Directive and to promote UA as a signing member of the Milan Urban Food Policy Pact. Based on crop requirements and farmer surveys, we find that the annual NPK demands of the agricultural fields of the AMB that cover 5,500 ha and produce 70,000 tons of crops are approximately 769, 113, and 592 tons of NPK, respectively. Spatial material flow analysis and life cycle assessment were applied to found that the current waste management system can potentially substitute 8 % of the total NPK demanded by UA with compost, reduce the impacts by up to 39 % and yield savings in global warming of 130 %. The more ambitious future scenario of 2025 can potentially substitute 21 % of the total NPK demand and reduce environmental impacts up to 1,049 %, depending on the category considered. Avoiding processing of mixed OMSW, mineral fertilizer replacement and cogeneration of electricity from biogas are the major contributors to these environmental savings.

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Urban design is currently promoting the inclusion of plants in buildings. However, plants emit biogenic volatile organic compounds (BVOCs), which alone or in combination with other airborne molecules such as CO2, may result in a general increase in tropospheric pollution. Many studies have documented the effects of biotic and abiotic factors on plant BVOC responses, but few have assessed the contribution of typical CO2 levels found in indoor work and meeting spaces. To answer this question, we monitored CO2 and constitutive (MT-limonene) and induced (LOX-cis-3-hexenal) BVOC emissions of a fully developed tomato crop grown hydroponically inside an integrated rooftop greenhouse (i-RTG) in a Mediterranean climate. Two distinctive CO2 assays were performed at the level of the i-RTG by supplying or not CO2. The impact of CO2 on plant physiological emittance was then assessed, and the resulting BVOC rates were compared with reference to EU-LCI values. MT-limonene was ubiquitous among the assays and the most abundant, while LOX-cis-3-hexenal was detected only under controlled CO2 management. The highest levels detected were below the indicated LCIs and were approximately tenfold lower than the corresponding LCI for MT-limonene (50.88 vs. 5000 µg m-3) and eightfold (6.63 µg m-3) higher than the constitutive emission level for LOX-cis-3-hexenal. Over extended sampling (10 min) findings revealed a general emission decrease and significantly different CO2 concentration between the assays. Despite similar decreasing rates of predicted net photosynthesis (Pn) and stomatal conductance (gs) their correlation with decreasing CO2 under uncontrolled condition indirectly suggested a negative CO2 impact on plant emission activity. Conversely, increasing CO2 under the controlled assay showed a positive correlation with induced emissions but not with constitutive ones. Because of significantly higher levels of relative humidity registered under the uncontrolled condition, this factor was considered to affect more than CO2 the emission response and even its collection. This hypothesis was supported by literature findings and attributed to a common issue related with the sampling in static enclosure. Hence, we suggested a careful monitoring of the sampling conditions or further improvements to avoid bias and underestimation of actual emissions. Based on the main outcomes, we observed no evidence of a hazardous effect of registered CO2 rates on the BVOC emissions of tomato plant. Furthermore, because of the low BVOC levels measured in the i-RTG, we assumed as safe the recirculation of this air along building's indoor environments.

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Heatwaves (HWs) are expected to increase both in duration and intensity in the next decades, but little is known about their synoptic and mesoscalar behavior, which is especially important in mid-latitude regions. Most climate research has focused on temperature analysis to characterize HWs. We propose that a combination of temperature and synoptic patterns is a better way to define and understand HWs because including atmospheric circulation patterns provides information about different HW structures that can irregularly affect the territory, and illustrate this approach at the regional and urban scales using the Iberian Peninsula and the Metropolitan Area of Barcelona as case studies. We first select HW events from 1950 to 2020 and apply a multivariate analysis to identify synoptic patterns based on mean sea level pressure, geopotential height at 500 hPa, and maximum daily 2 m temperature. The results indicate that four synoptic patterns reproduce at least 50% of the variance in HWs, namely, "stationary and stable", "dynamic and advective", "stationary and advective", and "dynamic, advective and undulated". Next, we apply the analysis to the Representative Concentration Pathway future scenarios (RCPs) 4.5 and 8.5 from the Coordinated Regional Climate Downscaling Experiment (CORDEX) to determine how these synoptic trends can change in the future. The analysis shows that the four synoptic patterns continue to explain 55 to 60% of the variance in HWs. Future HW events will be characterized by an increase in geopotential height at 500 hPa due to the northward shift of the anticyclonic ridge. This is especially true for RCP8.5, which simulates business as usual incrementing fossil fuel use and additionally shows an increase in atmospheric dynamism in north advections from all directions in comparison with RCP4.5. These findings point to the importance of considering the geopotential height in HW prediction, as well as the direction of advections. Supplementary Information: The online version contains supplementary material available at 10.1007/s00382-023-06828-1.

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Urban agriculture (UA) activities are increasing in popularity and importance due to greater food demands and reductions in agricultural land, also advocating for greater local food supply and security as well as the social and community cohesion perspective. This activity also has the potential to enhance the circularity of urban flows, repurposing nutrients from waste sources, increasing their self-sufficiency, reducing nutrient loss into the environment, and avoiding environmental cost of nutrient extraction and synthetization. The present work is aimed at defining recovery technologies outlined in the literature to obtain relevant nutrients such as N and P from waste sources in urban areas. Through literature research tools, the waste sources were defined, differentiating two main groups: (1) food, organic, biowaste and (2) wastewater. Up to 7 recovery strategies were identified for food, organic, and biowaste sources, while 11 strategies were defined for wastewater, mainly focusing on the recovery of N and P, which are applicable in UA in different forms. The potential of the recovered nutrients to cover existing and prospective UA sites was further assessed for the metropolitan area of Barcelona. Nutrient recovery from current composting and anaerobic digestion of urban sourced organic matter obtained each year in the area as well as the composting of wastewater sludge, struvite precipitation and ion exchange in wastewater effluent generated yearly in existing WWTPs were assessed. The results show that the requirements for the current and prospective UA in the area can be met 2.7 to 380.2 times for P and 1.7 to 117.5 times for N depending on the recovery strategy. While the present results are promising, current perceptions, legislation and the implementation and production costs compared to existing markets do not facilitate the application of nutrient recovery strategies, although a change is expected in the near future.

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Urban green installations are extensively promoted to increase sustainable and accessible food production and simultaneously improve the environmental performance and liveability of city buildings. In addition to the multiple benefits of plant retrofitting, these installations may lead to a consistent increase in biogenic volatile organic compounds (BVOCs) in the urban environment, especially indoors. Accordingly, health concerns could limit the implementation of building-integrated agriculture. In a building-integrated rooftop greenhouse (i-RTG), throughout the whole hydroponic cycle, green bean emissions were dynamically collected in a static enclosure. Four representative BVOCs, α-pinene (monoterpene), ß-caryophyllene (sesquiterpene), linalool (oxygenated monoterpene) and cis-3-hexenol (LOX derivate), were investigated in the samples collected from two equivalent sections of a static enclosure, one empty and one occupied by the i-RTG plants, to estimate the volatile emission factor (EF). Throughout the season, extremely variable BVOC levels between 0.04 and 5.36 ppb were found with occasional but not significant (P > 0.05) variations between the two sections. The highest emission rates were observed during plant vegetative development, with EFs equivalent to 78.97, 75.85 and 51.34 ng g-1 h-1 for cis-3-hexenol, α-pinene, and linalool, respectively; at plant maturity, all volatiles were either close to the LLOQ (lowest limit of quantitation) or not detected. Consistent with previous studies significant relationships (r ≥ 0.92; P < 0.05) were individuated within volatiles and temperature and relative humidity of the sections. However, correlations were all negative and were mainly attributed to the relevant effect of the enclosure on the final sampling conditions. Overall, levels found were at least 15 folds lower than the given Risk and LCI values of the EU-LCI protocol for indoor environments, suggesting low BVOC exposure in the i-RTG. Statistical outcomes demonstrated the applicability of the static enclosure technique for fast BVOC emissions survey inside green retrofitted spaces. However, providing high sampling performance over entire BVOCs collection is recommended to reduce sampling error and incorrect estimation of the emissions.

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Peri urban agriculture (peri-UA) can supply food locally and potentially more sustainably than far-away conventional agricultural systems. It can also introduce significant environmental impacts depending on the local biophysical conditions and resources required to implement it and, on the crops managing practices, which could vary widely among growers. Sophisticated methods to account for such variability while assessing direct (on-site) and indirect (up/down stream) environmental impacts of peri-UA implementation are thus needed. We implemented an attributional, regionalized, cradle-to-gate life cycle assessment (LCA) for which we derive spatially explicit inventories and calculate 14 impacts due to peri-UA using the ReCiPe method. Further, to show the importance of impact assessment regionalization for the environmental assessment of peri-UA, we regionalize eutrophication impacts characterization. We use the Metropolitan Area of Barcelona (AMB) to illustrate these methodological developments. Vegetables and greenhouses, the prevalent peri-UA land uses, had the largest impacts assessed, of all peri-UA land uses. European NPK mineral fertilizer production to cover N demand of these crops drives all impacts. For fruit crops, on-site N emissions drive marine eutrophication impacts and for irrigated herbaceous crops, phosphate runoff drives freshwater eutrophication impacts. Geographic variability of peri-UA metabolic flows and impacts was displayed. Management practices at the plots, which are linked the land use, are responsible for impacts variability. Regionalization of eutrophication impacts highlights the importance of accounting for the biophysical aspects at the geographic scale at which peri-UA takes place, which is a much finer scale than those implemented in current regionalization of impact assessment methods in LCA. This study provides a fundamental baseline needed to assess transition scenarios of peri-UA at an appropriate geographic level of analysis and gives essential knowledge to guide appropriate circular and sustainability strategies for the sector.

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A paradigm shift is needed in wastewater treatment plants (WWTPs) to progress from traditional pollutant removal to resource recovery. However, whether this transformation produces overall environmental benefits will depend on the efficient and sustainable use of resources by emerging technologies. Given that many of these technologies are still being tested at the pilot scale, there is a lack of environmental assessments quantifying their impacts and benefits. In particular, an integrated approach to energy and nutrient recovery can elucidate the potential configurations for WWTPs. In this study, we conduct a life cycle assessment (LCA) of emergent wastewater treatment technologies aimed at increasing resource circularity in WWTPs. We focus on increasing energy self-sufficiency through biogas upgrades and a more radical circular approach aimed at nutrient recovery. Based on a case-study WWTP, we compare its current configuration with (1) implementing autotrophic nitrogen removal in the mainstream and deriving most of the organic matter for biogas production, which increases the quality and quantity of biogas available for energy production; (2) implementing struvite recovery through enhanced biological phosphorus removal (EBPR) as a radical approach to phosphorus management, offering an alternative to mineral fertilizer; and (3) a combination of both approaches. The results show that incremental changes in biogas production are insufficient for compensating for the environmental investment in infrastructure, although autotrophic nitrogen removal is beneficial for increasing the quality of the effluent. Combined phosphorus and energy recovery reduce the environmental impacts from the avoided use of fertilizers and phosphorus and the nitrogen release into water bodies. An integrated approach to resource management in WWTPs is thus desirable and creates new opportunities toward the implementation of circular strategies with low environmental impact in cities.

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Geographically explicit datasets reflecting local management of crops are needed to help improve direct nitrous oxide (N2O) emission inventories. Yet, the lack of geographically explicit datasets of relevant factors influencing the emissions make it difficult to estimate them in such way. Particularly, for local peri-urban agriculture, spatially explicit datasets of crop type, fertilizer use, irrigation, and emission factors (EFs) are hard to find, yet necessary for evaluating and promoting urban self-sufficiency, resilience, and circularity. We spatially distribute these factors for the peri-urban agriculture in the Metropolitan Area of Barcelona (AMB) and create N2O emissions maps using crop-specific EFs as well as Tier 1 IPCC EFs for comparison. Further, the role of the soil types is qualitatively assessed. When compared to Tier 1 IPCC EFs, we find 15% more emissions (i.e. 7718 kg N2O-N year-1) than those estimated with the crop-specific EFs (i.e. 6533 kg N2O-N year-1) for the entire AMB. Emissions for most rainfed crop areas like cereals (e.g. oat and barley) and non-citric fruits (e.g. cherries and peaches), which cover 24% and 13% of AMB's peri-urban agricultural area respectively, are higher with Tier 1 EF. Conversely, crop-specific EFs estimate higher emissions for irrigated horticultural crops (e.g. tomato, artichoke) which cover 33% of AMB's peri-urban agricultural area and make up 70% of the total N2O emissions (4588 kg N2O-N year-1 using crop-specific EFs). Mapping the emissions helps evaluate spatial variability of key factors such as fertilizer use and irrigation of crops but carry uncertainties due to downscaling regional data to represent urban level data gaps. It also highlighted core emitting areas. Further the usefulness of the outputs on mitigation, sustainability and circularity studies are briefly discussed.

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Urban agriculture (UA) is a means for cities to become more resilient in terms of food sovereignty while shortening the distance between production and consumption. However, intensive soilless UA still depends on the use of fertilizers, which relies on depleting non-renewable resources such as phosphorous (P) and causes both local and global impact for its production and application. With the aim to reduce such impacts and encourage a more efficient use of nutrients, this study assesses the feasibility of using struvite precipitated from an urban wastewater treatment plant as the unique source of P fertilizer. To do so, we apply various quantities of struvite (ranging from 1 to 20 g/plant) to the substrate of a hydroponic Phaseolus vulgaris crop and determine the yield, water flows and P balances. The results show that treatments with more than 5 g of struvite per plant produced a higher yield (maximum of 181.41 g/plant) than the control (134.6 g/plant) with mineral fertilizer (KPO4H2). On the other hand, P concentration in all plant organs was always lower when using struvite than when using chemical fertilizer. Finally, the fact that different amounts of struvite remained undissolved in all treatments denotes the importance to balance between a correct P supply to the plant and a decrease of P lost through the leachates, based on the amount of struvite and the irrigated water. The findings of this study show that it is feasible for UA to efficiently use locally recovered nutrients such as P to produce local food.

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The rise of population in urban areas makes it ever more important to promote urban agriculture (UA) that is efficient in terms of water and nutrients. How to meet the irrigation demand of UA is of particular concern in urban areas where water sources are often limited. With the aim of determining how to reduce water use for irrigation while maintaining productivity and reducing environmental impacts in UA, this study explores the agronomic performance and environmental life cycle impacts and benefits of three different fertigation management practices used in a rooftop greenhouse for tomato crop in Barcelona: 1) open management (OP); 2) recirculation (RC), in which 30% of the drained, unused water is used to irrigate the crop; and 3) the same recirculated management of RC with a further reduction in fresh water input of 15%(RR). Despite the recirculation and reduction of water and nutrients, all three irrigation management practices resulted in similar yields: 16.2, 17.9, and 16.8·kg·m-2 for OP, RC, and RR, respectively. In terms of water-use efficiency, RR management was the most efficient, requiring 48.7·liters·kg-1 of tomato, followed by RC (52.4·L·kg-1) and OP (75.2·L·kg-1). RR presented an improvement of 7% in water-use efficiency. In terms of environmental performance, RC had the best performance in almost all impact categories during the operational phase, especially in regard to marine and freshwater eutrophication, with 44% and 93% fewer impacts than OP due to the recirculation of nutrients and reduced nutrient loss through leachates. In terms of infrastructure, even though recirculation management requires additional equipment, the materials present better performance in the range from 0.2 to 14% depending on the impact category. This study can support evaluation of agricultural projects in the city, through yields and water consumption presented, incentivizing good practices aligned with the sustainability of UA.

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Soilless crop production is a viable way to promote vertical agriculture in urban areas, but it relies extensively on the use of mineral fertilizer. Thus, the benefits of fresher, local food and avoiding the transportation and packaging associated with food import could be counteracted by an increase in nutrient-rich wastewater, which could contribute to freshwater and marine eutrophication. The present study aimed to explore the use of mineral fertilizer substitutes in soilless agriculture. Phaseolus vulgaris (common bean) was fertilized with a combination of slow-releasing fertilizer struvite (a source of N, P, and Mg), which is a byproduct of wastewater treatment plants, and inoculation with Rhizobium (a N2-fixing soil bacteria). The experiment included three bean-production lines: (A) 2 g/plant of struvite and rhizobial inoculation; (B) 5 g/plant of struvite and rhizobial inoculation, both irrigated with a Mg-, P-, and N-free nutrient solution; and (C) a control treatment that consisted of irrigation with a full nutrient solution and no inoculation. Plant growth, development, yields, and nutrient contents were determined at 35, 62, and 84 days after transplanting as well as biological N2 fixation, which was determined using the 15N natural abundance method. Treatments A and B resulted in lower total yields per plant than the control C treatment (e.g., 59.35 ± 26.4 g plant-1 for A, 74.2 ± 23.0 g plant-1 for B, and 147.71 ± 45.3 g plant-1 for C). For A and B, the nodulation and N2 fixation capacities appeared to increase with the amount of initially available struvite, but, over time, deficient levels of Mg were reached as well as nearly deficient levels of P, which could explain the lower yields. Nevertheless, we conclude that the combination of struvite and N2-fixing bacteria covered the N needs of plants throughout the growth cycle. However, further studies are needed to determine the optimal struvite quantities for vertical agriculture systems that can meet the P and Mg requirements throughout the lifetime of the plants.

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BACKGROUND: Urban agriculture contributes to meeting the growing food production demand in cities. In the context of low water availability, it is important to consider alternatives that are able to maintain production. Through a circular economy vision, this study aimed to assess the use of substrates made from local materials as an alternative for urban agriculture in periods of low water availability, due to water supply cuts. The substrates used were coir commercial organic substrate, vegetable compost from urban organic waste and perlite commercial standard substrate; a mixture of the urban compost and perlite (1:1) was used for three consecutive crop cycles of lettuce (Lactuca sativa L. var. crispa). The crop cycles were performed in the spring and summer periods of 2018 to observe the performance during warmer periods of the year in an integrated rooftop greenhouse near Barcelona. Each substrate was assessed under conventional irrigation (0-5 kPa) and temporary water restricted conditions (irrigation stopped until the water tension reached -20 kPa perlite). RESULTS: In terms of yield, our results show that the compost and mixture were similar to those obtained from perlite (11.5% and 3.7% more production under restricted water conditions). Organic substrates increased the crop's resilience to water restriction, in contrast to the perlite. In particular, water loss took longer in coir (one- and two-crop cycle); however, when dryness began, it occurred quickly. CONCLUSION: The vegetable compost and the substrate mixture presented tolerance to temporary water restriction when water restriction reached -20 kPa. © 2021 Society of Chemical Industry.

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Urban agriculture, while being a promising solution to increase food sovereignty in cities, can lead to an unprecedented discharge of nutrient and fertilizer-related emissions into the urban environment. Especially relevant are nitrogen (N) and phosphorus (P), due to their contribution to marine and freshwater eutrophication. Therefore, alternative methods of fertilization need to be put into practice to avoid such impacts to the surrounding environment. Struvite, has been studied as a potential slow releasing fertilizer due to its high P content, while the bacteria rhizobium has been used to fix N directly from the atmosphere. Legumes, like the common bean are N-demanding crops capable of symbiosis with the bacteria rhizobium and have previously shown positive responses to fertilization with struvite. This study aims to analyze the environmental performance of plant production in hydroponic systems combining rhizobium inoculation and struvite (2 g, 5 g, 10 g, 20 g) irrigated with a N and P deficient nutrient solution, using life cycle analysis (LCA). The nutrient content of in- and out-going irrigation was analyzed as well as in plants and beans. The functional unit for the LCA was 1 kg of fresh beans. The results obtained indicate a yield reduction of 60% to 50% in comparison to the control which was irrigated with a full nutrient solution. The impacts from operational stage are less in all impact categories, where most significant reductions up to 69% and 59% are seen in marine-eutrophication and global warming respectively. Although the infrastructure does not change between treatments, its impacts increase due to the lower yields. We determine that below a 10% of the control yield, the alternative systems have more impact than the use of conventional mineral fertilizers in almost all impact categories, thus pointing to the importance of infrastructure to truly reduce environmental impacts for urban agriculture.

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Urban agriculture systems can significantly contribute towards mitigating the impacts of inefficient and complex food supply chains and increase urban food sovereignty. Moreover, improving these urban agriculture systems in terms of nutrient management can lead to a better environmental performance. Based on a rooftop greenhouse in the Barcelona region, we propose a cascade system where the leachates of a tomato cycle from January to July (donor crop) are used as the main irrigation source for five successive lettuce cycles (receiving crop). By determining the agronomic performance and the nutrient metabolism of the system, we aimed to define the potential of these systems to avoid nutrient depletion and mitigate eutrophication, while scaling the system in terms of nutrient supply between the donor and the receiving crops. The results showed that low yields (below 130 g per lettuce plant) are obtained if a cascade system is used during the early stage of the donor crop, as the amount of nutrients in donor's leachates, specially N (62.4 mg irrigated per plant in the first cycle), was not enough to feed the lettuce receiving crop. This effect was also observed in the nutrient content of the lettuce, which increased with every test until equaling the control (4.4% of N content) as the leachates got richer, although too high electrical conductivity values (near 3 dS/m) were reached at the end of the donor crop cycle. Findings on the uptake of the residual nutrient flows showed how the cascade system was able to take advantage of the nutrients to produce local lettuce while mitigating the effect of N and P in the freshwater and marine environments. Considering our case study, we finally quantified the scale between the donor and receiving crops and proposed three major ideas to optimize the nutrient flows while maintaining the yield and quality of the vegetables produced in the receiving crop.

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Urban development and the sprawl of transport infrastructures have disregarded the crucial function of metropolitan landscape in provisioning human well-being and biodiversity. This research aims to contribute to the challenges of Planning for Sustainability by proposing a Socioecological Integrated Analysis (SIA) to support the Land Use Master Plan in the Barcelona Metropolitan Area, to conciliate urban development with the performance of surrounding open spaces. The paper evaluates four different land cover scenarios (current, trending, alternative and potential), and two kinds of agricultural management (conventional and a socioecological transition towards organic agriculture). The results suggest that although there are significant improvements on job provisioning and nutrient-cycling closures (circular economy), certified organic agriculture is not enough to overcome some trends of industrialized agrarian systems such as low energy efficiency or poor improvements in greenhouse gas emissions. The results also show a crossed effect between social metabolism and landscape ecology where changes in the management could affect the landscape functioning while changes in the land covers are particularly affecting the resource use. Then, deeper changes that consider together land use and metabolic flows are required to promote more sustainable agroecological transitions. The SIA model is an important conceptual and methodological step forward that facilitates the transition towards sustainable land use policies.

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Phosphorus (P) resources are decreasing at an alarming rate due to global fertilizer use and insufficient nutrient recovery strategies. Currently, more circular approaches are promoted, such as recovering P from wastewater in the form of struvite. This is especially attractive for urban areas, where there is a growing trend of local crop production and large volumes of wastewater are treated in centralized wastewater treatment plants (WWTPs). This research aims to assess the technical and environmental feasibility of applying a struvite recovery and reuse strategy to meet the P requirements to fertilize the agricultural fields of an urban region. To do so, we analyze the potential P recovery and the environmental impacts of integrating three recovery technologies (REM-NUT®, Ostara® and AirPrex®) in the two biggest WWTPs of the Àrea Metropolitana de Barcelona. The results show that all technologies are able to recover between 5 and 30 times the amount of P required to fertilize the agricultural area of the region annually (36.5 t). As can be expected, including P recovery technologies result in additional impacts per m3 of wastewater due to increased electricity consumption and chemicals required for the struvite precipitation. However, struvite recovery results in less eutrophication potential, especially in the REM-NUT® case, with an average reduction of 5.4 times. On the other hand, Ostara®, that recovers P from the digestate, had the lowest impacts (9 kgCO2eq/kgP), even compared to the production of mineral fertilizer. When we apply our findings to the whole region, we can see that chemical use for struvite precipitation and energy consumption during the wastewater treatment process are the elements with the greatest impact. Thus, choosing the most appropriate technology in the most suitable WWTP is the most efficient strategy to diminish the environmental impacts of the system.

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Cities are rapidly growing and need to look for ways to optimize resource consumption. Metropolises are especially vulnerable in three main systems, often referred to as the FEW (i.e., food, energy, and water) nexus. In this context, urban rooftops are underutilized areas that might be used for the production of these resources. We developed the Roof Mosaic approach, which combines life cycle assessment with two rooftop guidelines, to analyze the technical feasibility and environmental implications of producing food and energy, and harvesting rainwater on rooftops through different combinations at different scales. To illustrate, we apply the Roof Mosaic approach to a densely populated neighborhood in a Mediterranean city. The building-scale results show that integrating rainwater harvesting and food production would avoid relatively insignificant emissions (13.9-18.6 kg CO2 eq/inhabitant/year) in the use stage, but their construction would have low environmental impacts. In contrast, the application of energy systems (photovoltaic or solar thermal systems) combined with rainwater harvesting could potentially avoid higher CO2 eq emissions (177-196 kg CO2 eq/inhabitant/year) but generate higher environmental burdens in the construction phase. When applied at the neighborhood scale, the approach can be optimized to meet between 7% and 50% of FEW demands and avoid up to 157 tons CO2 eq/year. This approach is a useful guide to optimize the FEW nexus providing a range of options for the exploitation of rooftops at the local scale, which can aid cities in becoming self-sufficient, optimizing resources, and reducing CO2 eq emissions.

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Biogas is rich in methane and can be further purified through biogas upgrading technologies, presenting a viable alternative to natural gas. Landfills and anaerobic digestors treating municipal solid waste are a large source of such biogas. They therefore offer an attractive opportunity to tap into this potential source of natural gas while at the same time minimizing the global warming impact resulting from methane emissions in waste management schemes (WMS) and fossil fuel consumption reduction. This study looks at the current municipal solid waste flows of Spain, Italy, and Austria over one year (2009), in order to determine how much biogas is generated. Then it examines how much natural gas could be substituted by using four different biogas upgrading technologies. Based on current waste generation rates, exploratory but realistic WMS were created for each country in order to maximize biogas production and potential for natural gas substitution. It was found that the potential substitution of natural gas by biogas resulting from the current WMS seems rather insignificant: 0.2% for Austria, 0.6% for Italy and 0.3% for Spain. However, if the WMS is redesigned to maximize biogas production, these figures can increase to 0.7% for Austria, 1% for Italy and 2% for Spain. Furthermore, the potential CO2 reduction as a consequence of capturing the biogas and replacing fossil fuel can result in up to a 93% reduction of the annual national waste greenhouse gas emissions of Spain and Italy.

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This article evaluates the life cycle assessment (LCA) of three biogas upgrading technologies. An in-depth study and evaluation was conducted on high pressure water scrubbing (HPWS), as well as alkaline with regeneration (AwR) and bottom ash upgrading (BABIU), which additionally offer carbon storage. AwR and BABIU are two novel technologies that utilize waste from municipal solid waste incinerators - namely bottom ash (BA) and air pollution control residues (APC) - and are able to store CO(2) from biogas through accelerated carbonation processes. These are compared to high pressure water scrubbing (HPWS) which is a widely used technology in Europe. The AwR uses an alkaline solution to remove the CO(2) and then the solution - rich in carbonate and bicarbonate ions - is regenerated through carbonation of APC. The BABIU process directly exposes the gas to the BA to remove and immediately store the CO(2), again by carbonation. It was determined that the AwR process had an 84% higher impact in all LCA categories largely due to the energy intensive production of the alkaline reactants. The BABIU process had the lowest impact in most categories even when compared to five other CO(2) capture technologies on the market. AwR and BABIU have a particularly low impact in the global warming potential category as a result of the immediate storage of the CO(2). For AwR, it was determined that using NaOH instead of KOH improves its environmental performance by 34%. For the BABIU process the use of renewable energies would improve its impact since accounts for 55% of the impact.

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