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1.
Phys Rev Lett ; 132(7): 076202, 2024 Feb 16.
Artículo en Inglés | MEDLINE | ID: mdl-38427866

RESUMEN

We propose a concept of quantum dot based light emitting diode that produces circularly polarized light without magnetic contacts due to the hyperfine interaction at the crossing of the exciton levels in a weak magnetic field. The electroluminescence circular polarization degree can reach 100%. The concept is compatible with the micropillar cavities, which allows for the generation of single circularly polarized photons. Second order photon correlation function includes information about the nuclear spin dynamics in the quantum dot, and the nuclear spin state can be purified by the quantum measurement backaction.

2.
Nat Commun ; 14(1): 6683, 2023 Oct 21.
Artículo en Inglés | MEDLINE | ID: mdl-37865649

RESUMEN

Coherent many-body states are highly promising for robust quantum information processing. While far-reaching theoretical predictions have been made for various implementations, direct experimental evidence of their appealing properties can be challenging. Here, we demonstrate optical manipulation of the nuclear spin ensemble in the lead halide perovskite semiconductor FAPbBr3 (FA = formamidinium), targeting a long-postulated collective dark state that is insensitive to optical pumping after its build-up. Via optical orientation of localized hole spins we drive the nuclear many-body system into this entangled state, requiring a weak magnetic field of only a few milli-Tesla strength at cryogenic temperatures. During its fast establishment, the nuclear polarization along the optical axis remains small, while the transverse nuclear spin fluctuations are strongly reduced, corresponding to spin squeezing as evidenced by a strong violation of the generalized nuclear squeezing-inequality with ξs < 0.5. The dark state corresponds to an ~35-body entanglement between the nuclei. Dark nuclear spin states can be exploited to store quantum information benefiting from their long-lived many-body coherence and to perform quantum measurements with a precision beyond the standard limit.

3.
Nanomaterials (Basel) ; 13(4)2023 Feb 14.
Artículo en Inglés | MEDLINE | ID: mdl-36839097

RESUMEN

Exciton recombination and spin dynamics in (In,Al)As/AlAs quantum dots (QDs) with indirect band gap and type-I band alignment were studied. The negligible (less than 0.2 µeV) value of the anisotropic exchange interaction in these QDs prevents the mixing of the excitonic basis states and makes the formation of spin-polarized bright excitons possible under quasi-resonant, circularly polarized excitation. The recombination and spin dynamics of excitons are controlled by the hyperfine interaction between the electron and nuclear spins. A QD blockade by dark excitons was observed in the magnetic field, that eliminates the impact of nuclear spin fluctuations. A kinetic model which accounts for the population dynamics of the bright and dark exciton states as well as for the spin dynamics was developed to quantitatively describe the experimental data.

4.
Nanoscale ; 14(36): 13284-13291, 2022 Sep 22.
Artículo en Inglés | MEDLINE | ID: mdl-36062980

RESUMEN

We describe theoretically the effects of the quantum back action under the continuous optical measurement of electron spins in quantum dots. We consider the system excitation by elliptically polarized light close to the trion resonance, which allows for simultaneous spin orientation and measurement. We microscopically demonstrate that the nuclei-induced spin relaxation can be both suppressed and accelerated by the continuous spin measurement due to the quantum Zeno and anti-Zeno effects, respectively. Our theoretical predictions can be directly compared with the future experimental results and straightforwardly generalized for pump-probe experiments.

5.
Phys Rev Lett ; 129(7): 077401, 2022 Aug 12.
Artículo en Inglés | MEDLINE | ID: mdl-36018709

RESUMEN

It is known that linear birefringence of the medium essentially hinders measuring the Faraday effect. For this reason, optically anisotropic materials have never been considered as objects of the Faraday-rotation-based spin noise spectroscopy. We show, both theoretically and experimentally, that strong optical anisotropy that may badly suppress the regular Faraday rotation of the medium, practically does not affect the measurement of the spatially uncorrelated spin fluctuations. We also show that the birefringent media provide additional opportunity to measure spatial spin correlations. Results of the experimental measurements of the spin-noise spectra performed on Nd^{3+} ions in the uniaxial crystal matrices well agree with the theory.

6.
Nanoscale Horiz ; 7(7): 752-758, 2022 Jun 27.
Artículo en Inglés | MEDLINE | ID: mdl-35593642

RESUMEN

We put forward a mechanism for the current-induced spin polarization in semiconductor heterostructures, which is based on the complex structure of the valence band. It takes place for a light hole in a quantum dot side-coupled to a quantum wire with heavy holes. In stark contrast with the traditional mechanisms based on the linear in momentum spin-orbit coupling, an exponentially small bias applied to this structure is enough to create the 100% spin polarization in the quantum dot. Microscopically, this effect is related to the formation of the chiral quasi bound states and the spin-dependent tunneling of holes from the quantum wire to the quantum dot. This new concept is equally valid for the GaAs-, Si- and Ge-based nanostructures.

7.
Phys Rev Lett ; 126(21): 216804, 2021 May 28.
Artículo en Inglés | MEDLINE | ID: mdl-34114866

RESUMEN

We obtain a compact analytical solution for the nonlinear equation for the nuclear spin dynamics in the central spin box model in the limit of many nuclear spins. The total nuclear spin component along the external magnetic field is conserved and the two perpendicular components precess or oscillate depending on the electron spin polarization, with the frequency, determined by the nuclear spin polarization. As applications of our solution, we calculate the nuclear spin noise spectrum and describe the effects of nuclear spin squeezing and many body entanglement in the absence of a system excitation.

8.
Phys Rev Lett ; 125(15): 156801, 2020 Oct 09.
Artículo en Inglés | MEDLINE | ID: mdl-33095603

RESUMEN

We suggest a new spin orientation mechanism for localized electrons: dynamic electron spin polarization provided by nuclear spin fluctuations. The detrimental effect of nuclear spin fluctuations can be harnessed and employed to provide angular momentum for the electrons via the hyperfine interaction in a weak magnetic field. For this, the sample is illuminated by an unpolarized light, which directly polarizes neither the electrons nor the nuclei. We predict that, for the electrons bound in localized excitons, 100% spin polarization can be reached in longitudinal magnetic fields of a few millitesla. The proof of principle experiment is performed on momentum-indirect excitons in (In,Al)As/AlAs quantum dots, where in a magnetic field of 17 mT the electron spin polarization of 30% is measured.

9.
Nano Lett ; 20(1): 158-165, 2020 Jan 08.
Artículo en Inglés | MEDLINE | ID: mdl-31756115

RESUMEN

Fascinating optical properties governed by extremely confined excitons have been so far observed in 2D crystals like monolayers of transition metal dichalcogenides. These materials, however, are limited for production by epitaxial methods. Besides, they are not suitable for the development of optoelectronics for the challenging deep-ultraviolet spectral range. Here, we present a single monolayer of GaN in AlN as a heterostructure fabricated by molecular beam epitaxy, which provides extreme 2D confinement of excitons, being ideally suited for light generation in the deep-ultraviolet. Optical studies in the samples, supplemented by a group-theory analysis and first-principle calculations, make evident a giant enhancement of the splitting between the dark and bright excitons due to short-range electron-hole exchange interaction that is a fingerprint of the strongly confined excitons. The practical significance of our results is in the observation of the internal quantum yield of the room-temperature excitonic emission as high as ∼75% at 235 nm.

11.
Phys Rev Lett ; 118(11): 116801, 2017 Mar 17.
Artículo en Inglés | MEDLINE | ID: mdl-28368634

RESUMEN

In disordered systems, the hopping conductivity regime is usually realized at low temperatures where spin-related phenomena differ strongly from the cases of delocalized carriers. We develop the unified microscopic theory of current-induced spin orientation, spin-galvanic, and spin-Hall effects for the two-dimensional hopping regime. We show that the corresponding susceptibilities are proportional to each other and determined by the interplay between the drift and the diffusion spin currents. Estimations are made for realistic semiconductor heterostructures using the percolation theory. We show that the electrical spin polarization in the hopping regime increases exponentially with the increase of the concentration of localization sites and may reach a few percent at the crossover from the hopping to the diffusion conductivity regime.

12.
J Phys Condens Matter ; 24(34): 345302, 2012 Aug 29.
Artículo en Inglés | MEDLINE | ID: mdl-22871901

RESUMEN

A theoretical description of electron spin orientation and detection by short optical pulses is proposed for ensembles of singly charged semiconductor nanocrystals. The complex structure of the valence band in spherical nanocrystals is taken into account. We demonstrate that the direction of electron spin injected by the pump pulse depends on both the pump pulse helicity and the pump pulse power. It is shown that a train of optical pulses can lead to the complete orientation of the resident electron spin. The microscopic theory of the spin Faraday, Kerr and ellipticity effects is developed and the spectral sensitivity of these signals is discussed. We show that under periodic pumping pronounced mode-locking of electron spins takes place and manifests itself as significant spin signals at negative delays between pump and probe pulses.

13.
Neurosci Behav Physiol ; 34(7): 697-701, 2004 Sep.
Artículo en Inglés | MEDLINE | ID: mdl-15526425

RESUMEN

Four episodes of immobilization stress induced a decrease in the sensitivity of rats to glucocorticoid hormones, which was accompanied by anxiogenic behavior, increased MAO-B activity, and a parallel increase in lipid peroxidation (LPO) in brain tissues. There was a simultaneous increase in MAO-B activity in the kidneys and accumulation of LPO products in the liver and kidneys. Administration of Kenalog (2 mg/kg), a pharmacological analog of glucocorticoid hormones, prevented the poststress activation of MAO-B and LPO and decreased the extent of anxiogenic behavioral abnormalities in rats.


Asunto(s)
Conducta Animal/efectos de los fármacos , Glucocorticoides/farmacología , Peroxidación de Lípido/efectos de los fármacos , Monoaminooxidasa/metabolismo , Estrés Fisiológico , Animales , Conducta Animal/fisiología , Encéfalo/efectos de los fármacos , Encéfalo/enzimología , Femenino , Riñón/efectos de los fármacos , Riñón/enzimología , Peroxidación de Lípido/fisiología , Hígado/efectos de los fármacos , Hígado/enzimología , Locomoción/efectos de los fármacos , Locomoción/fisiología , Masculino , Actividad Motora/efectos de los fármacos , Ratas , Restricción Física/métodos , Estadísticas no Paramétricas , Estrés Fisiológico/enzimología , Estrés Fisiológico/fisiopatología , Triamcinolona Acetonida/farmacología
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