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Optical metasurfaces present remarkable opportunities for manipulating wave propagation in unconventional ways, surpassing the capabilities of traditional optical devices. In this work, we introduce and demonstrate a multifunctional dynamic tuning of dielectric metasurfaces containing liquid crystals (LCs) through an effective three-dimensional (3D) control of the molecular orientation. We theoretically and experimentally study the spectral tuning of the electric and magnetic resonances of dielectric metasurfaces, which was enabled by rotating an external magnetic field in 3D. Our approach allows for the independent control of the electric and magnetic resonances of a metasurface, enabling multifunctional operation. The magnetic field tuning approach eliminates the need for the pre-alignment of LCs and is not limited by a finite set of directions in which the LC molecules can be oriented. Our results open new pathways for realizing dynamically reconfigurable metadevices and observing novel physical effects without the usual limitations imposed by the boundary conditions of LC cells and the external voltage.

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We study the propagation dynamics of bright optical vortex solitons in nematic liquid crystals with a nonlocal reorientational nonlinear response. We investigate the role of optical birefringence on the stability of these solitons. In agreement with recent experimental observations, we show that the birefringence-induced astigmatism can eventually destabilize these vortex solitons. However, for low and moderate birefringence, vortex solitons can propagate stably over experimentally relevant distances.

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We study experimentally the interaction of mutually incoherent bright spatial solitons in dye-doped nematic liquid crystals (LCs). The dye-induced light absorption results in a complex nonlinear optical response of the LC having spatially nonlocal focusing and defocusing contributions. The competition between both nonlinearities leads to the separation-dependent soliton interaction with repulsion of distant and attraction of closely placed solitons.

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We study nonlinear propagation of light in colloidal suspension of metallic nanoparticles, in the regime of particles surface plasmon resonance. We show that the propagation exhibits features typical for purely defocusing media and the observed spatial confinement is not a real self-trapping, as for solitons, but rather than is caused by the phase modulation of the beam via nonlocal defocusing nonlinearity. We also show that the light-induced refractive index change in the suspension leads to stabilization of structured light beams. In particular, we demonstrate a stable nonlinear propagation of bright ring beams with complex states of polarization, including practically important radial and azimuthal states.

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We report on the first experimental observation of stable vortex solitons in nematic liquid crystals with nonlocal nonlinear reorientational response. We show how these nonlinear vortex beams can be formed and confined in extraordinary optical waves by employing the cell with no lateral boundary conditions and the application of an external magnetic field that effectively controls the molecular direction and propagation of the self-trapped beams. We also find that these vortex solitons can be generated in certain ranges of the input beam power.

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Among photofunctional materials that can be employed to control the propagation of light by modifying their properties, soft dielectrics such as nematic liquid crystals (NLCs) stand out for their large all-optical response. Through reorientation, the molecular distribution of NLCs can be modified by the electric field of light, permitting functional operations and supporting self-localized light beams or spatial optical solitons. To date, the generation and routing of such solitons have been limited by the boundary conditions employed to tailor the properties of NLCs in planar cells or capillaries. Here we report on spatial solitons in bulk NLCs with no lateral anchoring, where the application of an external magnetic field effectively controls the direction of propagation and the angular steering of the self-trapped wavepackets. Our results entail a completely new approach to the routing of self-localized beams and light-induced waveguides in three dimensions, without the usual limitations imposed by transverse boundary conditions.

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We demonstrate an all-optical fabrication method of quasi-phase matching structures in lithium niobate (LiNbO3) waveguides using a tightly focused femtosecond near-infrared laser beam (wavelength of 800 nm). In contrast to other all-optical schemes that utilize a periodic lowering of the nonlinear coefficient χ(2) by material modification, here the illumination of femtosecond pulses directly reverses the sign of χ(2) through the process of ferroelectric domain inversion. The resulting quasi-phase matching structures, therefore, lead to more efficient nonlinear interactions. As an experimental demonstration, we fabricate a structure with the period of 2.74 µm to frequency double 815 nm light. A maximum conversion efficiency of 17.45% is obtained for a 10 mm long waveguide.

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This work represents experimental demonstration of nonlinear diffraction in an orientation-patterned semiconducting material. By employing a new transverse geometry of interaction, three types of second-order nonlinear diffraction have been identified according to different configurations of quasi-phase matching conditions. Specifically, nonlinear Cerenkov diffraction is defined by the longitudinal quasi-phase matching condition, nonlinear Raman-Nath diffraction satisfies only the transverse quasi-phase matching condition, and nonlinear Bragg diffraction fulfils the full vectorial quasi-phase matching conditions. The study extends the concept of transverse nonlinear parametric interaction toward infrared frequency conversion in semiconductors. It also offers an effective nondestructive method to visualise and diagnose variations of second-order nonlinear coefficients inside semiconductors.

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New forms of electron beams have been intensively investigated recently, including vortex beams carrying orbital angular momentum, as well as Airy beams propagating along a parabolic trajectory. Their traits may be harnessed for applications in materials science, electron microscopy, and interferometry, and so it is important to measure their properties with ease. Here, we show how one may immediately quantify these beams' parameters without need for additional fabrication or nonstandard microscopic tools. Our experimental results are backed by numerical simulations and analytic derivation.

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In this article we compare the results of micromachining of fused silica and silicon with tightly focused scalar (viz., circularly and linearly polarized) and vector (viz., azimuthally and radially polarized) femtosecond laser pulses. We show that drilling with radially polarized pulses produces holes with smoother and better-delineated walls compared with the other polarizations used, whereas linearly polarized pulses can machine 20-nm wide single grooves in fused silica when the electric field of the pulse is aligned perpendicular to the cutting direction. The observed polarization-controlled micromachining is due to the formation of sub-diffraction-limited nanostructures that are optically produced in the multi-pulse irradiation regime.

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We demonstrate experimentally that, in a tight focusing geometry, circularly polarized femtosecond laser vortex pulses ablate material differently depending on the handedness of light. This effect offers an additional degree of freedom to control the shape and size of laser-machined structures on a subwavelength scale.

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We demonstrate that airborne light-absorbing particles can be photophoretically trapped and moved inside an optical lattice formed by multiple-beam interference. This technique allows simultaneous three-dimensional manipulation of multiple micro-objects in gases.

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We demonstrate that micron-sized light-absorbing particles can be trapped and transported photophoretically in air using an optical bottle formed inside the focal volume of a lens with a controlled amount of spherical aberration. This optical fiber-based single beam trap can be used in numerous applications where true 3D manipulation and delivery of airborne micro-objects is required.

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We utilize the interaction of tightly focused ultrashort pulses with transparent media to imprint their local polarization in the focal region. In particular, we demonstrate that this technique allows for a subwavelength resolution diagnostic of complex polarization states including the presence of the longitudinal component of the electric field. Moreover, we demonstrate the first ever material ablation with the longitudinal electric field of femtosecond pulses.

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In this Letter we present the first (to our knowledge) demonstration of material modification using tightly focused single femtosecond laser vortex pulses. Double-charge femtosecond vortices were synthesized with a polarization-singularity beam converter based on light propagation in a uniaxial anisotropic medium and then focused using moderate- and high-NA optics (viz., NA=0.45 and 0.9) to ablate fused silica and soda-lime glass. By controlling the pulse energy, we consistently machine micrometer-size ring-shaped structures with <100nm uniform groove thickness.

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We demonstrate a new principle of optical trapping and manipulation increasing more than 1000 times the manipulation distance by harnessing strong thermal forces while suppressing their stochastic nature with optical vortex beams. Our approach expands optical manipulation of particles into a gas media and provides a full control over trapped particles, including the optical transport and pinpoint positioning of ∼100 µm objects over a meter-scale distance with ±10 µm accuracy.

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We describe an optical beam converter for an efficient transformation of Gaussian femtosecond laser beams to single- or double-charge vortex beams. The device achieves a conversion efficiency of 75% for single- and 50% for double-charge vortex beams and can operate with high-energy broad bandwidth pulses. We also show that the topological charge of a femtosecond vortex beam can be determined by analyzing its intensity distribution in the focal area of a cylindrical lens.

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We describe how the propagation of light through uniaxial crystals can be used as a versatile tool towards the spatial engineering of polarization and phase, thereby providing an all-optical technique for vectorial and scalar singular beam shaping in optics. Besides the prominent role played by the linear birefringence, the influence of circular birefringence (the optical activity) is discussed as well and both the monochromatic and polychromatic singular beam shaping strategies are addressed. Under cylindrically symmetric light-matter interaction, the radially, azimuthally, and spirally polarized eigen-modes for the light field are revealed to be of a fundamental interest to describe the physical mechanisms at work when dealing with scalar and vectorial optical singularities. In addition, we also report on nontrivial effects arising from cylindrical symmetry breaking, e.g. tilting the incident beam with respect to the crystal optical axis.

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We study experimentally the interaction of spatial optical solitons with curved dielectric surfaces in unbiased nematic liquid crystals. We demonstrate that this interaction depends on the curvature of the surface and the walk-off, and it can be employed for efficient routing and control of the soliton trajectories. We also observe a large-angle total internal reflection of the soliton beam from an interface between liquid crystal and air.

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We suggest a new approach for selective trapping of light absorbing particles in gases by multiple optical bottle-beam-like traps created by volume speckle field. We demonstrate stable simultaneous confinement of a few thousand micro-particles in air with a single lowpower laser beam. The size distribution of trapped particles exhibits a narrow peak near the average size of an optical speckle. Thus, the speckleformed traps act as a sieve with the holes selecting particles of a similar size.