RESUMEN
Nuclear and radiological accidents have demonstrated the need for prior planning for exposure assessment as well as guidelines for the implementation of protection and remediation measures of contaminated areas. Typically, the description of the efficiency of the measures in the literature is associated with the reduction of the concentration of the environmental media where they are applied. In order to verify the efficiency related to the reduction in doses, some basic scenarios were established, taking into account aspects of a typical tropical climate, such as building materials (urban areas) and types of crops and farming practices, considering the seasonality and soil type typical of the southeastern region of Brazil. The Integrated System for Emergency (SIEM) program was used to perform the simulations. The results indicate that decision-making processes must be made in accordance with the actual conditions of contamination and use of the affected area. For rural areas, the effectiveness of measures depends on many factors specific to each site, such as seasonality, produced crops, diet habits and degree of subsistence on the items in the diet, which make it unfeasible to develop generic predefined scenarios. The criteria for classification of measurements were defined as: (i) the efficiency in reducing the doses in the first year, in which largest dose rates are observed; (ii) the efficiency in reducing the long-term dose, considering 50 y for adults and (iii) the effect of delay in implementation of the measures on the reduction of doses.
Asunto(s)
Contaminantes del Suelo , Suelo , Agricultura , Brasil , Exposición a Riesgos AmbientalesRESUMEN
In this work the role of organic matter in the potential mobility and bioavailability of 137Cs and 60Co in Brazilian soil was investigated. Radish was cultivated in pots containing the top layer (0-20 cm) of a Histosol, Ferralsol and Nitisol spiked with 137Cs and 60Co. In the case of the Ferralsol and Nitisol samples, besides the control, two different rates of organic amendments were used. In these soils, a sequential extraction protocol was used to identify the main soil compartments that could be responsible for the variation of transfer factor values. Our results indicate that organic amendment could be suggested as a practical countermeasure for 137Cs and 60Co contamination, since it reduces bioavailability of radionuclides and, consequently, soil to plant transfer factor values by almost one order of magnitude in a short period of time.
Asunto(s)
Radioisótopos de Cesio/metabolismo , Radioisótopos de Cobalto/metabolismo , Fertilizantes , Raphanus/metabolismo , Contaminantes Radiactivos del Suelo/metabolismo , Suelo , Agricultura/métodos , BrasilRESUMEN
In this study, soil to plant transfer factor values were determined for 137Cs and 60Co in radish (Raphanus sativus), maize (Zea mays L.) and cabbage (Brassica oleracea L. var. capitata) growing in gibbsite-, kaolinite- and iron-oxide-rich soils. After 3 years of experiment in lysimeters it was possible to identify the main soil properties able to modify the soil to plant transfer processes, e.g. exchangeable K and pH, for 137Cs, and organic matter for 60Co. Results of sequential chemical extraction were coherent with root uptake and allowed the recognition of the role of iron oxides on 137Cs behaviour and of Mn oxides on 60Co behaviour. This information should provide support for adequate choices of countermeasures to be applied on tropical soils in case of accident or for remediation purposes.
Asunto(s)
Brassica/metabolismo , Radioisótopos de Cesio/metabolismo , Radioisótopos de Cobalto/metabolismo , Raphanus/metabolismo , Contaminantes Radiactivos del Suelo/metabolismo , Zea mays/metabolismo , Compuestos Férricos , Caolín , Hojas de la Planta/metabolismo , SueloRESUMEN
The housing features in a country depend much on its climate. Dwellings in warm countries are much lighter constructions than in cold ones, which will reflect on the amount of shielding against radiation they provide. In addition to that, wealth is another factor that influences the building's finishing. Great effort has been taken to determine parameters to more accurately estimate dose to a population in case of a radioactive or nuclear accident. Nevertheless, most available data are concerned with typical housing in cold climate countries. This study aims to determine shielding factors for typical building materials used in the southeast of Brazil, a warm area, due to radioactive material deposited on the surrounding field, walls and ceiling of the external surfaces. The shielding factors determination was performed by simulation with the MCNP5 Monte Carlo computer code. The air kerma indoors for the 300, 662 and 3000 keV photon energies have been determined for three different housing patterns, ranging from the very simple to a very complex structure. The shielding factor, defined as the ratio of the air kerma indoor to the air kerma in open field, for the most simple house type and 300 keV photon energy was found to be twice of the best finished one for the same energy.
Asunto(s)
Contaminación del Aire Interior/análisis , Materiales de Construcción/análisis , Rayos gamma , Vivienda , Monitoreo de Radiación/métodos , Protección Radiológica/instrumentación , Radioisótopos/análisis , Brasil , Exposición a Riesgos Ambientales/análisis , Dosis de Radiación , Protección Radiológica/métodosRESUMEN
This study discusses the methodology for measuring and assessing the radon concentration in indoor and outdoor environments. A research study was developed to investigate the long-term behavior of the diurnal and seasonal fluctuations of radon (222)Rn EEC (Equilibrium-Equivalent Concentration) and the influence of temperature and other climatic aspects on this behavior. The study was performed by means of both integrated and instantaneous measurements of radon and its short-lived daughter products for a period of 1 year in an indoor environment in Rio de Janeiro city, Brazil (reference environment), with continuous measurement, using a radon monitor with an alpha spectrometry detector. For a single day, a variability of about 50% could be observed in the (222)Rn EEC values measured on a hourly basis, with a maximum occurring early in the morning and a minimum in the afternoon. For the long-term period, seasonality is responsible for a two order of magnitude variability, with a maximum of 50 Bq.m(-3) in winter (dry season) and a minimum of 0.5 Bq.m(-3) in the summer months (wet season), outdoors. A negative correlation with temperature was observed. The conclusions of this experiment led to a survey of radon gas concentration in dwellings in Rio de Janeiro city, Brazil, in urban area with nearly 7 million inhabitants, through integrated sampling methods, using a Solid State Nuclear Track Detectors Technique (SSNTD). The study was conducted in different geomorphological locations in town. The radon gas concentration in Rio de Janeiro dwellings ranged from 5 Bq.m(-3) to 200 Bq.m(-3). A good correlation between indoor radon gas concentration and location of dwellings was observed. The seashore areas presented the lowest levels of indoor radon concentration, whereas the highest levels were found close to the mountains.
Asunto(s)
Contaminantes Radiactivos del Aire/análisis , Contaminación del Aire Interior/análisis , Radón/análisis , Brasil , Monitoreo del Ambiente , Geografía , Humanos , Estaciones del AñoRESUMEN
Two niobium mining facilities located at two different geological settings were selected as case studies for assessing the radiological impacts associated with mining and milling activities. The impacts were assessed both for operational and post-operational (future unrestricted use of the area) scenarios. The work methodology encompassed sampling and analysis of different materials along the operational process, including wastes, effluents and by-products, mass balance calculations, and dose assessment. The exposure scenario considered during the operational phase included the land use by hypothetical groups of members of the general public. In the case of post-operational phase the possible occupation of contaminated areas was considered. The results pointed out that during the operational phase of the investigated industries no relevant impacts could be attributed to them. However, in the case of the potential occupation of the contaminated areas where the wastes are being deposited, the unrestricted use of these areas cannot be accepted in terms of the relevant radiation protection requirements.
Asunto(s)
Niobio/análisis , Radioisótopos/análisis , Eliminación de Residuos/métodos , Exposición a Riesgos Ambientales , Monitoreo del Ambiente/métodos , Dosis de Radiación , TiempoRESUMEN
The concentrations of the naturally occurring radionuclides 232Th, 238U, 210Pb, 226Ra and 238Ra were determined in the vegetables (leafy vegetables, fruit, root, bean and rice) and derived products (sugar, coffee, manioc flour, wheat flour, corn flour and pasta) consumed most by the adult inhabitants of Rio de Janeiro City. A total of 88 samples from 26 different vegetables and derived products were analyzed. The highest contribution to radionuclide intake arises from bean, wheat flour, manioc flour, carrot, rice, tomato and potato consumption. The estimated daily intakes due to the consumption of vegetables and derived products are 1.9 mBq of 232Th (0.47 microg), 2.0 mBq of 238U (0.17 microg), 19 mBq of 236Ra, 26 mBq of 210Pb and 47 mBq of 228Ra. The estimated annual effective dose due to the ingestion of vegetables and their derived products with the long-lived natural radionuclides is 14.5 microSv. Taking into account literature data for water and milk from Rio de Janeiro the dose value increases to 29 microSv, with vegetables and derived products responsible for 50% of the dose and water for 48%. 210Pb (62%) and 228Ra (24%) were found to be the main sources for internal irradiation.
Asunto(s)
Exposición a Riesgos Ambientales , Contaminación de Alimentos , Radioisótopos/farmacocinética , Verduras , Brasil , Monitoreo del Ambiente , Humanos , Radioisótopos/análisis , Población UrbanaRESUMEN
Niobium, phosphate, coal and gold mining facilities have been selected as case studies with the aim of identifying possible sources of radiological impact during and after cessation of industrial operations. The results have shown that acid drainage, as well as chemical processing of mineral ores, constitute relevant impact indicators for present-day and future scenarios. The possible use of solid wastes abandoned at the end of the operations represents a long-term radiological concern. Therefore, it is necessary that Brazilian legislation for environmental licensing be revised taking into account the potential environmental and radiological impacts caused by these industries and establishing remedial procedures for waste storage areas in the existing sites. The indicators developed and procedures carried out can be used in screening for decisions on the adoption of regulatory requirements for practices at such types of installations.
Asunto(s)
Ambiente , Minería , Contaminantes Radiactivos , Brasil , Carbón Mineral , Monitoreo del Ambiente , Predicción , Oro , Niobio , Fosfatos , Eliminación de Residuos Líquidos , Movimientos del AguaRESUMEN
The uncertainties in the exposure predictions after contamination of an urban area due to the variabilities in environmental transfer parameters and in dose conversion factors have been estimated. This was done using the "Latin Hypercube" sampling scheme and the computer codes PRISM and PARATI. For the scenario 'urban contamination by 137Cs' and the population groups considered, the main sources contributing to the uncertainty in the resulting exposures are the limited knowledge of the initial deposition and retention, the weathering processes, the actual urban environments, and the characteristics and habits of the population. The effect of the parameter uncertainties on the variability of the dose is almost constant over time.
Asunto(s)
Simulación por Computador , Exposición a Riesgos Ambientales , Contaminantes Radiactivos , Población Urbana , Radioisótopos de Cesio , Materiales de Construcción , Vivienda , Humanos , Medición de Riesgo , Salud UrbanaRESUMEN
After a large-scale contamination of an urban area with gamma-ray emitting radionuclides (e.g. caesium isotopes) decision makers will need guidance as to its potential radiological consequences and to optimum means of mitigation. To provide such information, a dynamic radioecological model PARATI has been developed and used to simulate the contamination of realistic urban environments in a computer model and to estimate the various radiation fields in such environments. In this study, the computer-simulated realistic behaviour and movements of individuals and populations in such radiation fields are described, and the resulting radiation exposures and their variabilities are estimated. For the scenarios considered, the doses of individuals in the same contaminated environment may vary by more than one order of magnitude. Studies on population habits and on the behaviour of radionuclides on important urban surfaces even a long time after the contamination might reduce the uncertainty considerably.
Asunto(s)
Simulación por Computador , Ecosistema , Exposición a Riesgos Ambientales , Rayos gamma , Modelos Biológicos , Salud Urbana , Adolescente , Adulto , Distribución por Edad , Anciano , Niño , Preescolar , Relación Dosis-Respuesta en la Radiación , Estudios de Evaluación como Asunto , Humanos , Lactante , Recién Nacido , Persona de Mediana EdadRESUMEN
The structure and mathematical model of PARATI, a detailed computer programme developed for the assessment of the radiological consequences of an accidental contamination of urban areas, is described with respect to the scenarios used for the estimation of exposure fields in a village or town, the models for the initial and secondary contamination with the radionuclide 137Cs, the concepts for calculating the resulting radiation exposures and the changes with time of the contamination and radiation fields. Kerma rates at various locations in tropical urban areas are given, and the contribution of different contaminated surfaces to these rates after dry or wet deposition are discussed.
Asunto(s)
Liberación de Radiactividad Peligrosa , Contaminantes Radiactivos/análisis , Animales , Simulación por Computador , Contaminación de Alimentos , HumanosRESUMEN
In September 1987, a powder radioactive source was removed from a teletherapy machine in Goiânia, Brazil. Subsequently, it was ruptured in a residential garden causing the dissemination of 137Cs throughout the city. Soil resuspension processes and burial of contaminated house waste in unused gardens were the major contributors to the Cs dissemination in soils at the secondary contaminated sites. Only locations within a radius of 50 m from the primary contaminated sites presented the need for remedial action. The radiation dose-rate measurements and the soil profiles were good indicators of the extent of the secondary contamination and were fundamental for the decisions taken regarding decontamination procedures. In cases of surface contamination, 60% on average of the total activity remained in the upper 1.5-cm layer over the first 5 mo after the accident, and topsoil removal proved to be an effective procedure for decontamination.