RESUMEN
Aerosol-CCN characteristics and dynamics during a pre-monsoon dust storm (April 6-11, 2015) over a high-altitude site ((17.92°N, 73.66°E, and 1348 m above mean sea level (MSL)) in Western Ghats, India, has been studied using ground-based observations, satellite, and reanalysis datasets. Spatial distribution of dust surface mass concentration along with the back trajectory analysis showed the Arabian Desert area (Rub-Al-khali desert) as the source region and strong westerly winds transported the dust particles toward the Indian subcontinent. High values noticed in the surface PM10 (PM2.5), i.e., ~ 450 (~ 130) µg m-3, MODIS AOD550nm (0.6), and MERRA 2 dust surface mass concentration (5 × 10-7 kg m-3) along MODIS true color images confirmed the dust storm event on April 6, 2015 over the observational site. Size-segregated aerosol number concentration measured from ground-based observations showed the dominance of Aitken, accumulation, and coarse mode particles during dust period. CCN concentrations at 0.1, 0.3, 0.5, 0.7, and 0.9% SS were analyzed. A low value of CCN concentration and activation fraction (~ 0.3) near surface was noticed during dust storm day, suggesting insoluble mineral dust particle being transported. Analyzed vertical velocity during pre-dust period showed downdraft between 900 and 750 hPa, suggesting dust transport from upper altitudes toward the observational site. WRF-Chem model simulation also captured the dust storm event, and the results are in good agreement with the observation with a significance of 95% confidence level.
Asunto(s)
Contaminantes Atmosféricos , Contaminantes Atmosféricos/análisis , Altitud , Polvo/análisis , Viento , Aerosoles/análisis , India , Monitoreo del AmbienteRESUMEN
The characteristics of black carbon (BC) aerosols, their sources, and their impact on atmospheric radiative forcing were extensively studied during the COVID-19 lockdown (28th March-31st May 2020) at a high-altitude rural site over the Western Ghats in southwest India. BC concentration and the contribution of BC originating from biomass burning (BCbb) estimated from the aethalometer model during the lockdown period were compared with the same periods in 2017 and 2018 and with the pre-lockdown period (1st February to March 20, 2020). BC concentrations were 44, 19, and 17% lower during the lockdown period compared with the pre-lockdown periods of 2020 and similar periods (28th March to 31st May) of 2017 and 2018, respectively. BCbb contributed â¼50% to total BC during the lockdown period of 2020 and compensated for the decrease in BC concentration due to lower traffic emissions. The characteristics of light-absorbing organic carbon (brown carbon; BrC) absorption at 370 nm were evaluated during the lockdown and the pre-lockdown periods of 2020, 2017, and 2018. The BrC was estimated to be the highest during the lockdown period of 2020. Finally, atmospheric radiative forcing was calculated using the mean BC concentration during the pre-lockdown, lockdown, and similar periods (28th March to 31st May) of 2017 and 2018.
RESUMEN
The temporal variability of the planetary boundary layer height (PBLH) over Mahabaleshwar was studied for a period of 1 year from 1 December 2015 to 30 November 2016 using microwave radiometer (MWR) observations. The PBLH over Mahabaleshwar was found to be the highest during the pre-monsoon (March-May) season and lowest during the winter (December-February) season. The seasonal mean of PBLH was estimated to be 339±88 m during winter, 485±70 m during pre-monsoon, 99±153 m during monsoon, and 438±24 m during post-monsoon season. Frequency distribution analysis of PBLH during pre-monsoon season revealed that the formation of turbulence internal boundary layer (TIBL) is evident. In contrast, cold and moist air mass during the monsoon season enhances the wind shear with lower buoyancy term which results in lowering of PBLH. The comparison of PBLH between MWR and radiosonde observations shows a good correlation (r2 = 0.66, p=0.001). The growth rate was observed to be 388 m/h during pre-monsoon, 206 m/h during winter, 57 m/h during monsoon, and 167 m/h during post-monsoon season. The seasonal mean concentration of PM2.5 was found to be 42.3±4.6 µg/m3during winter, 33.4±8.7 µg/m3 during pre-monsoon, 6.6±2.2 µg/m3 during monsoon, and 26.1±1.7 µg/m3during post-monsoon season. The effect of higher loading of scattering-type aerosol (dust particle) was also investigated as a case study. The analysis reveals the inverse relationship between the PBL height variability and the particulate loading indicating the importance of aerosol direct effect. Analysis of the ventilation coefficient (Vc) revealed that the dissipation potential was higher (1736 m2/s) during pre-monsoon season as compared to (1191 m2/s, 455m2/s, and 1580 m2/s) winter, monsoon, and post-monsoon seasons.