RESUMEN
Soil-plant transfer factor (TF) is one of the vital variables employed in assessing plants uptake of radionuclides and their transfer to food chain for predictive ingestion dose and risk evaluation. To further this goal, the TF characteristics of natural 40K, 232Th and 226Ra were thus investigated in some crops (yam, cassava, rice, maize, groundnut, cowpea, okra, pumpkin leaf, banana and pawpaw) cultivated in southwestern part of Nigeria using HPGe gamma spectroscopy. The obtained results of activity concentration (AC) of the radionuclides across all the cultivated soil samples indicated average values that are less than the global average, whereas in the crops, average values of 226Ra and 232Th, were higher than reference values for different crops group. The overall range of the calculated TF of 40K, 232Th and 226Ra across all the crops was 0.05 (in maize and cowpea) to 15.01 (in banana), 0.01 (in pumpkin leaf and groundnut) to 19.80 (in pawpaw), and 0.04 (in cassava) to 21.30 (in cowpea), respectively. Overall arithmetic mean and geometric mean were estimated as 2.66 and 1.60, 1.11 and 0.43, and 1.10 and 0.54 for 40K, 232Th and 226Ra, respectively. TFs mostly correlated negatively with soil radionuclides, while positive correlation was mostly noticeable in the case of crop. Log normal transform of the TFs data indicated a near normal distribution as against the calculated data. The derived results of this study is here presented as a baseline data suggested for possible radiological risk assessment of food chain of the local population.
RESUMEN
Gamma spectrometric measurement of natural radionuclides activity concentrations by HPGe detectors was conducted in 150 agricultural soil samples collected from six states of southwestern Nigeria. The overall activity concentrations of radionuclides ranged from 15.27 to 972.00 Bqkg-1 for 40K, 0.66 to 336.19 Bqkg-1 for 232Th and 1.32 to 123.01 Bqkg-1 for 238U, with mean values of 143.95, 17.02 and 22.92 Bqkg-1, respectively. The overall averages results from this study were generally lower than worldwide average value of 420, 33 and 45 Bqkg-1 for 40K, 238U and 232Th, respectively, thus minimal transfer to plant may be expected. The estimated radiation dose levels of the soil indicated acceptable limits for general public exposure. The radioactivity levels of 40K, 232Th and 238U in the investigated agricultural soil of southwestern Nigeria are within acceptable limits. Therefore, stochastic radiological health effects of radiation exposure by farmers may not be feasible at the current moment.