RESUMEN
We have observed electromagnetically induced transparency in a Doppler broadened molecular cascade system using fluorescence detection. We demonstrate that the power-dependent splitting of lines in the upper-level fluorescence excitation spectrum can be used as a new spectroscopic tool for the measurement of molecular transition dipole moment functions.
RESUMEN
The nonlinear behavior of a frustrated-total-reflection (FTR) optical cavity containing a nonlinear Kerr medium is considered. It is shown that optical bistability may occur at lower incident power than in the nonlinear interface system. Other potential advantages of the resonant FTR configuration over other geometries are also briefly discussed.
RESUMEN
Nonlinear absorption coefficients have been calculated for certain direct-bandgap semiconductors at 0.694-microm, 1.06-microm, 1.318-microm, and 10.6-microm wavelengths and compared with experimental results. The second- order perturbation theories of Braunstein and Basov yield underestimates and overestimates, respectively, of the nonlinear absorption constants. The numerical values are dependent upon the use of appropriate effective band masses, dielectric constants, and electron spin degeneracy factors. However, the Keldysh model gives second-order absorption constants that are intermediate between the two perturbation calculations. Although the Keldysh model often underestimates the value, in general, it yields the estimate of the magnitude of the two-photon absorption coefficient. The one-photon band-edge absorption in GaAs and InSb is predicted surprisingly well by the Keldysh model.