RESUMEN
This paper presents findings on groundwater physiochemical composition and radioactivity levels in households in Bac Lieu province, Vietnam. Through discriminant analysis, it was observed that groundwater quality exhibits spatial variations corresponding to saline intrusion zones. The paired-samples T-tests revealed significantly different ratios of Ra-224, Ra-226, and Ra-228 isotopes between Na-Cl and Ca-Na-HCO3 water types. All three water types had a ratio of Ra-226/Ra-228 of approximately one, indicating the presence of groundwater aquifers beneath the crust and fluvial marine sediment. Furthermore, strong associations between sulfate and calcium suggest that CO2 enrichment in groundwater aquifers indicates anoxic aquatic environments. Twenty-five of the thirty-three evaluated samples exceeded the national technical regulations for domestic water quality with parameters such as chloride, sulfate, sodium, gross alpha, or total dissolved solids. Fifteen samples exceeded gross alpha's allowable contamination threshold of 0.1 Bq/L. The combination of Ra-226 and Ra-228 did not surpass the U.S. Environmental Protection Agency's recommended limit of 0.185 Bq/L. However, nineteen samples exhibited annual committed effective doses of radium isotopes for infants that exceeded the WHO recommendation of 0.1 mSv/year.
Asunto(s)
Agua Subterránea , Radio (Elemento) , Contaminantes Radiactivos del Agua , Vietnam , Agua Subterránea/química , Contaminantes Radiactivos del Agua/análisis , Humanos , Radio (Elemento)/análisis , Monitoreo de Radiación/métodos , Composición Familiar , Sulfatos/análisisRESUMEN
This paper presents information on the concentration of radioactivity and chemicals at 12 water stations that used groundwater as their raw water supply source. The groundwater's radioactivity was higher than the treated, tap, and surface water, but lower than the national and international recommendations. At five stations (41.7%), the gross alpha contents were higher than the levels advised by Vietnam's regulations, but met the WHO and IAEA's recommendations. The mean activity (Bq L-1) gross alpha, gross beta, Ra-224, Ra-226, and Ra-228 were 0.093 ± 0.012, 0.221 ± 0.020, 0.031 ± 0.004, 0.028 ± 0.004, and 0.035 ± 0.001, respectively. The contribution of Ra-226 to the gross alpha was in a range of 23%-60% (r = 0.91, p value <0.001), and the ratio of Ra-226/Ra-228 ranged from 0.49-1.06. For the treated and tap water, each age groups' annual committed effective dose was lower than the international regulations. The concentration of the total dissolved solids, sulfate, chloride, sodium, barium, and manganese met the national regulations. However, during the rainy season, the surface water in the area was affected by saltwater intrusion, with salinity up to 4.1. Discriminant analysis was applied to study the differences among the water groups. As a result, the treated and tap water were separated from the others.
Asunto(s)
Monitoreo de Radiación , Radiactividad , Contaminantes Radiactivos del Agua/análisis , Salud Pública , Vietnam , Abastecimiento de AguaRESUMEN
This paper presents information on the gross alpha and gross beta activity concentrations of two hundred twenty-six groundwater samples collected by gas flow proportional counters in southern Vietnam. The gross alpha results in the water samples ranged from 0.024 to 0.748 Bq L-1 with a mean of 0.183 ± 0.034 Bq L-1, and the gross beta results in the water samples ranged from 0.027-0.632 Bq L-1 with a mean of 0.152 ± 0.015 Bq L-1. The values obtained in this work were compared with those previously published for various regions or countries. Next, untreated and treated groundwater samples were analyzed to assess their influences on the treatment process. The results showed that there were differences in the minimum detection concentrations and the mean activity values between the untreated and treated groundwater samples (The p-value of the mean comparison tests is significant with p < 0.05). In both sample groups, there was a strong positive correlation of the gross alpha versus the gross beta results (r > 0.6). This means that among the radionuclides, the major sources of beta radiation are uranium and thorium decay series radionuclides. Finally, the annual effective dose for adults (>17 years) was calculated based on the assumption that major radionuclides have the highest effective dose conversion factors. In general, the results for Pb-210, Ra-226, and Ra-228 were observed to be lower than the recommended reference values established by the World Health Organization and the International Atomic Energy Agency, except for the value of Po-210.