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1.
Chemosphere ; 364: 143154, 2024 Aug 21.
Artículo en Inglés | MEDLINE | ID: mdl-39173835

RESUMEN

As climate change induces changes in water quality and available water quantity of drinking water supply sources, the final product water quality changes in terms of trace organics including disinfection byproducts (DBPs) formed during water treatment. In this study, the seasonal variability and speciation of DBPs across nine sample sites within a drinking water distribution system serving ∼400k people over a one-year period was investigated considering the governing parameters of water quality and treatment/transport/storage of finished water. The system considered treats surface water from a river and practices aquifer storage and recovery to address seasons water availability changes. Eighty-eight (88) sample sets were collected and held for 6-months in the laboratory to simulate extended storage scenarios associated with ASR operations, and each was analyzed at 9 different timesteps for concentration and speciation of chlorinated DBPs. Samples from groundwater influenced sites exhibited significantly lower total organic carbon (TOC) compared to other sites from the river source, and also were observed to have the lowest DBP formation. Three sites exceeded the Maximum Contaminant Level (MCL) for four total trihalomethanes (THM4) within 30-60 days of storage. Chloroform was the predominant THM4 species, even in groundwater-influenced locations, whereas di- and tri-chloroacetic acid (DCA and TCA) were the most prevalent haloacetic acids (HAA5). Extended water age at one site, coupled with low initial chlorine concentrations exhibited higher initial THM4 concentrations and flat DBP formation curves. The study results provide new insights into DBP occurrence and fate in drinking water distribution systems which consider water storage such as in ASR.

2.
Water Environ Res ; 92(11): 1922-1934, 2020 Nov.
Artículo en Inglés | MEDLINE | ID: mdl-32319709

RESUMEN

An innovative approach to treat centrate for rapid nitrogen load discharge reduction was investigated and applied at the Truckee Meadows Water Reclamation Facility (TMWRF) in Reno, NV. This process allowed TMWRF to circumvent an anticipated exceedance of the individual waste load allocation in 2018. Existing infrastructure and equipment were re-purposed in a full-scale suspended growth biological centrate treatment system, attaining simultaneous nitrification, and denitrification with no additional capital investment. Functioning within a few days of start-up, the average ammonia reduction was 81% (1,106 kg/day) and the average total nitrogen reduction in the sidestream was 53% (757 kg/day) using primary effluent as carbon source. Alkalinity and carbon limitations were both anticipated and observed; however, adaptive operations allowed for balancing of nitrification and denitrification processes, providing pH stability and success in meeting treatment goals. Immediately after the sidestream treatment system was placed into service, nitrogen in the mainstream facility was measured at concentrations significantly lower than typical and was sustained at historically low concentrations throughout the operation. This translated into a significant methanol cost savings of $1,500 per day (USD). The system has become a critical supplemental treatment process during upcoming rehabilitation projects to address aging infrastructure of existing nitrogen treatment facilities. PRACTITIONER POINTS: Full scale demonstration of sidestream N removal using a hybrid process. Integration of the sidestream N process to reduce N effluent load without alkalinity or supplementary carbon augmentation. Operational solution to reduce operating costs without new infrastructure.


Asunto(s)
Carbono , Eliminación de Residuos Líquidos , Reactores Biológicos , Desnitrificación , Nitrificación , Nitrógeno , Aguas del Alcantarillado , Aguas Residuales
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