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1.
Phys Chem Chem Phys ; 26(12): 9534-9545, 2024 Mar 20.
Artículo en Inglés | MEDLINE | ID: mdl-38456242

RESUMEN

Copper zinc tin sulfide (CZTS) thin films were synthesized on soda lime glass using pulsed laser deposition (PLD) at room temperature. Introducing gold nanoparticles (AuNPs) in a sandwich structure led to increased CZTS particle size and a shift in the localized surface plasmon resonance (LSPR) peak of the AuNPs, influenced by different laser energy levels. The absorption measurements revealed intriguing behavior across the visible and near-infrared (NIR) regions, making these films appealing for 1 Sun photodetectors. Furthermore, the presence of AuNPs in the sandwich structure reduced microstrain effects, measuring 1.94 × 10-3 compared to 3.38 × 10-3 in their absence. This reduction directly enhances carrier transport, which is particularly beneficial for accelerating the performance of photodetector devices. This effect of AuNPs also contributed to higher dielectric coefficients, further improving the photodetector performance. Under 1 Sun illumination conditions, this enhancement resulted in a rapid rising time of 95.4 ms, showcasing the potential for faster photodetection.

2.
Heliyon ; 9(12): e22867, 2023 Dec.
Artículo en Inglés | MEDLINE | ID: mdl-38076119

RESUMEN

This computational investigation delves into the electronic and optical attributes of InGaN/GaN nanostructures subjected to both harmonic and anharmonic confinement potentials, coupled with the influence of a nonresonant intense laser field (ILF). The theoretical framework incorporates higher-order anharmonic terms, specifically quartic and sextic terms. The solutions to the Schrödinger equation have been computed employing the finite element method and the effective mass theory. Moreover, linear and third-order nonlinear optical absorption coefficients are derived via a density matrix expansion. Our analysis reveals the feasibility of manipulating electronic and optical properties by adjusting confinement potential parameters, system attributes, and laser field intensity. In addition, the ILF induces remarkable modifications, characterized by reduced resonance peak amplitudes and a blue shift in absorption coefficients. Intriguingly, regardless of potential harmonicity, the impact of incident electromagnetic intensity is notably more pronounced in the absence of the ILF. These findings hold significant promise for advancing theoretical predictions, providing valuable insights into the intricate interplay between confinement potentials, laser fields, and their effects on electronic and optical behaviors within nanostructures.

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