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1.
Adv Mater ; 33(45): e2104083, 2021 Nov.
Artículo en Inglés | MEDLINE | ID: mdl-34536042

RESUMEN

The occurrence of unconventional superconductivity in cuprates has long motivated the search for manifestations in other layered transition metal oxides. Recently, superconductivity is found in infinite-layer nickelate (Nd,Sr)NiO2 and (Pr,Sr)NiO2 thin films, formed by topotactic reduction from the perovskite precursor phase. A topic of much current interest is whether rare-earth moments are essential for superconductivity in this system. In this study, it is found that with significant materials optimization, substantial portions of the La1- x Srx NiO2 phase diagram can enter the regime of coherent low-temperature transport (x = 0.14 - 0.20), with subsequent superconducting transitions and a maximum onset of ≈9 K at x = 0.20. Additionally, the unexpected indication of a superconducting ground state in undoped LaNiO2 is observed, which likely reflects the self-doped nature of the electronic structure. Combining the results of (La/Pr/Nd)1- x Srx NiO2 reveals a generalized superconducting dome, characterized by systematic shifts in the unit cell volume and in the relative electron-hole populations across the lanthanides.

2.
Nat Nanotechnol ; 16(4): 404-408, 2021 Apr.
Artículo en Inglés | MEDLINE | ID: mdl-33462428

RESUMEN

At non-zero temperatures, superconductors contain excitations known as Bogoliubov quasiparticles (QPs). The mesoscopic dynamics of QPs inform the design of quantum information processors, among other devices. Knowledge of these dynamics stems from experiments in which QPs are injected in a controlled fashion, typically at energies comparable to the pairing energy1-5. Here we perform tunnel spectroscopy of a mesoscopic superconductor under high electric fields. We observe QP injection due to field-emitted electrons with 106 times the pairing energy, an unexplored regime of QP dynamics. Upon application of a gate voltage, the QP injection decreases the critical current and, at sufficiently high electric field, a field-emission current (<0.1 nA in our device) switches the mesoscopic superconductor into the normal state, consistent with earlier observations6. We expect that high-energy injection will be useful for developing QP-tolerant quantum information processors, will allow rapid control of resonator quality factors and will enable the design of electric-field-controlled superconducting devices with new functionality.

3.
Phys Rev Lett ; 125(2): 027001, 2020 Jul 10.
Artículo en Inglés | MEDLINE | ID: mdl-32701320

RESUMEN

We report the phase diagram of Nd_{1-x}Sr_{x}NiO_{2} infinite layer thin films grown on SrTiO_{3}. A superconducting dome spanning 0.125

4.
Nat Commun ; 6: 7682, 2015 Jul 17.
Artículo en Inglés | MEDLINE | ID: mdl-26184854

RESUMEN

The central-spin problem is a widely studied model of quantum decoherence. Dynamic nuclear polarization occurs in central-spin systems when electronic angular momentum is transferred to nuclear spins and is exploited in quantum information processing for coherent spin manipulation. However, the mechanisms limiting this process remain only partially understood. Here we show that spin-orbit coupling can quench dynamic nuclear polarization in a GaAs quantum dot, because spin conservation is violated in the electron-nuclear system, despite weak spin-orbit coupling in GaAs. Using Landau-Zener sweeps to measure static and dynamic properties of the electron spin-flip probability, we observe that the size of the spin-orbit and hyperfine interactions depends on the magnitude and direction of applied magnetic field. We find that dynamic nuclear polarization is quenched when the spin-orbit contribution exceeds the hyperfine, in agreement with a theoretical model. Our results shed light on the surprisingly strong effect of spin-orbit coupling in central-spin systems.

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